Synthesis and characterization of siloxy, aminoxy, and oxo complexes from the reaction of a tantalum amide silyl complex with oxygen

Inorganic Chemistry

Volumn 48, Issue 7, 2009, Pages 3073-3079

  Qiu, He ^a,b,c,d,e,f   Chen, Shu Jian ^a,b,c,d,e,f   Wang, Chang Sheng ^a,b,c,d,e   Wu, Yun Dong ^a,b,c,d,e   Guzei, Ilia A ^a,b,c,d,e,g   Chen, Xue Tai ^a,b,c,d,e   Xue, Zi Ling ^a,b,c,d,e,f  

^a UNIVERSITY OF TENNESSEE   (United States)

^b HONG KONG UNIVERSITY OF SCIENCE AND TECHNOLOGY   (Hong Kong)

^c LIAONING NORMAL UNIVERSITY   (China)

^d UNIVERSITY OF WISCONSIN MADISON   (United States)

^e NANJING UNIVERSITY   (China)

^f UNIVERSITY OF TENNESSEE   (United States)

^g UNIVERSITY OF WISCONSIN   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

AMIDE; ORGANOMETALLIC COMPOUND; ORGANOSILICON DERIVATIVE; OXIDE; OXYGEN; TANTALUM;

ARTICLE; CHEMICAL STRUCTURE; CHEMISTRY; SYNTHESIS; X RAY CRYSTALLOGRAPHY;

AMIDES; CRYSTALLOGRAPHY, X-RAY; MODELS, MOLECULAR; ORGANOMETALLIC COMPOUNDS; ORGANOSILICON COMPOUNDS; OXIDES; OXYGEN; TANTALUM;

EID: 64349089492     PISSN: 00201669     EISSN: None     Source Type: Journal    
DOI: 10.1021/ic802380u     Document Type: Article

References (84)

1. (a) Feig, A. L.; Lippard, S. J. Chem. Rev. 1994, 94, 759.
2. (b) Klotz. I. M.; Kurtz, D. M. Chem. Rev. 1994, 94, 567.
3. (c) Theopold, K. H.; Reinaud, O. M.; Blanchard, S.; Leelasubeharoen, S.; Hess, A.: Thyagarajan, S. ACS Symp. Ser. 2002, 823, 75.
4. (d) Kopp, D. A.; Lippard, S. J. Curr. Opin. Chem. Biol. 2002, 6, 568.
5. (e) Que, L., Jr.: Tolman, W. B. Angew. Chem., Int. Ed. 2002, 41, 1114.
6. (f) Brown. S. N.; Mayer, J. M. Inorg. Chem. 1992, 31, 4091.
7. (g) Balch, A. L.; Cornman, C. R.; Olmstead, M. M. J. Am. Chem. Soc. 1990, 112, 2963.
8. Advances in Catalytic Activation of Dioxygen by Metal Complexes: Simándi, L. I., Ed.; Kluwer: Boston, 2003.
9. The Activation of Dioxygen and Homogeneous Catalytic Oxidation: Barton, D. H. R., Martell, A. E., Sawyer, D. T., Eds.; Plenum: New York, 1993.
10. (a) Labinger, J. A.; Hart, D. W.; Seibert, W. E.; Schwartz, J. J. Am. Chem. Soc. 1975, 97, 3851.
11. (b) Blackburn, T. F.; Labinger, J. A.; Schwartz, J. Tetrahedron Lett. 1975, 16, 3041.
12. (a) Lubben, T. V.; Wolczanski, P. T. J. Am. Chem. Soc. 1985, 107, 701.
13. (b) Lubben, T. V.; Wolczanski, P. T. J. Am. Chem. Soc. 1987, 109, 424.
14. Brindley, P. B.; Scotton, M. J. J. Chem. Soc., Perkin Trans. 1981, 419.
15. Tilley, T. D. Organometallics 1985, 4, 1452.
16. Wang, R.; Folting, K.; Huffman, J. C.; Chamberlain, L. R.; Rothwell, I. P. Inorg. Chim. Acta 1986, 120, 81.
17. Gibson, V. C.; Redshaw, C.; Walker, G. L. P.; Howard, J. A. K.; Hoy, V. J.; Cole, J. M.; Kuzmina, L. G.; De Silva, D. S. J. Chem. Soc., Dalton Trans. 1999, 161.
18. Brindley, P. B.; Hodgson, J. C. J. Organomet. Chem. 1974, 65, 57.
19. (a) Van Asselt, A.; Trimmer, M. S.; Healing, L. M.; Bercaw, J. E. J. Am. Chem. Soc. 1988, 110, 8254.
20. (b) Coughlin, E. B.; Bercaw, J. E. Organometallics 1992, 11, 465.
21. Gibson, T. Organometallics 1987, 6, 918.
22. Kim, S.-J.; Jung, I. N.; Yoo, B. R.; Cho, S.; Ko, J.; Kim, S. H.; Kang, S. O. Organometallics 2001, 20, 1501.
23. (a) Wallace, R. M.; Wilk, G. D. Crit. Rev. Solid State Mater. Sci. 2003, 28, 231.
24. (b) Smith, R. C.; Ma, T.; Hoilien, N.; Tsung, L. Y.; Bevan, M. J.; Colombo, L.; Roberts, J.; Campbell, S. A.; Gladfelter, W. L. Adv. Mater. Opt. Electron. 2000, 10, 105.
25. (c) Kelly, P. V. Adv. Mater. Opt. Electron. 2000, 10, 115.
26. (d) Senzaki, Y.; Hochberg, A. K.; Norman, J. A. T. Adv. Mater. Opt. Electron. 2000, 10, 93.
27. 2 and High-κ Materials for ULSI Gate Dielectrics).
28. (a) Bastianini, A.; Battiston, G. A.; Gerbasi, R.; Porchia, M.; Daolio, S. J. Phys. IV 1995, 5, C5-525.
29. (b) Ohshita, Y.; Ogura, A.; Hoshino, A.; Hiiro, S.; Machida, H. J. Cryst. Growth 2001, 233, 292.
30. (c) Hendrix, B. C.; Borovik, A. S.; Xu, C.; Roeder, J. F.; Baum, T. H.; Bevan, M. J.; Visokay, M. R.; Chambers, J. J.; Rotondaro, A. L. P.; Bu, H.; Colombo, L. Appl. Phys. Lett. 2002, 80, 2362.
31. (d) Schlom, D. G.; Guha, S.; Datta, S. MRS Bull. 2008, 33, 1017.
32. Son, K.-A.; Mao, A. Y.; Sun, Y.-M.; Kim, B. Y.; Liu, F.; Kamath, A.; White, J. M.; Kwong, D. L.; Roberts, D. A.; Vrtis, R. N. Appl. Phys. Lett. 1998, 72, 1187.
33. (a) Miyazaki, S. J. Vac. Sci. Technol. 2001, B19, 2212.
34. (b) Yu, J. J.; Boyd, I. W. Phys. Status Solidi A 2006, 203, R9.
35. (a) Robertson, J.; Chen, C. W. Appl. Phys. Lett. 1999, 74, 1168.
36. (b) Robertson, J. J. Vac. Sci. Technol. 2000, B18, 1785.
37. (c) Robertson, J. J. Non-Cryst. Solids 2002, 303, 94.
38. Wang, R.-T.; Zhang, X.-H.; Chen, S.-J.; Yu, X.-H.; Wang, C.-S.; Beach, D. B.; Wu, Y.-D.; Xue, Z.-L. J. Am. Chem. Soc. 2005, 127, 5204.
39. Chen, S.-J.; Zhang, X.-H.; Yu, X.; Qiu, H.; Yap, G. P. A.; Guzei, I. A.; Lin, Z.; Wu, Y.-D.; Xue, Z.-L. J. Am. Chem. Soc. 2007, 129, 14408.
40. Wu, Z.-Z.; Cai, H.; Yu, X.-H.; Blanton, J. R.; Diminnie, J. B.; Pan, H.-J.; Xue, Z.-L. Organometallics 2002, 21, 3973.
41. (a) Chen, T.-N.; Wu, Z.-Z.; Li, L.-T.; Sorasaenee, K. R.; Diminnie, J. B.; Pan, H.-J.; Guzei, I. A.; Rheingold, A. L.; Xue, Z.-L. J. Am. Chem. Soc. 1998, 120, 13519.
42. (b) Chen, T.-N.; Zhang, X.-H.; Wang, C.-S.; Chen, S.-J.; Wu, Z.-Z.; Li, L.-T.; Sorasaenee, K. R.; Diminnie, J. B.; Pan, H.-J.; Guzei, I. A.; Rheingold, A. L.; Wu, Y.-D.; Xue, Z.-L. Organometallics 2005, 24, 1214.
43. For metal silyl and related chemistry, see, e.g. ,(a) Tilley, T. D. In The Silicon-Heteroatom Bond; Patai, S., Rappoport, Z.; Eds.; Wiley: New York, 1991; Chapters 9 and 10.
44. (b) Eisen, M. S. In The Chemistry of Organic Silicon Compounds Vol. 2; Rappoport, Z.; Apeloig, Y., Eds.; Wiley: New York, 1998,Pt. 3, p 2037.
45. (c) Corey, J. Y. In Advances in Silicon Chemistry; Larson, G., Ed.; JAI Press: Greenwich, CT, 1991; Vol. 1, p 327.
46. (d) Gauvin, F.; Harrod, J. F.; Woo, H. G. Adv. Organomet. Chem. 1998, 42, 363.
47. (e) Sharma, H. K.; Pannell, K. H. Chem. Rev. 1995, 95, 1351.
48. (f) Campion, B. K.; Falk, J.; Tilley, T. D. J. Am. Chem. Soc. 1987, 109, 2049.
49. (g) Procopio, L. J.; Carroll, P. J.; Berry, D. H. Polyhedron 1995, 14, 45.
50. (h) Nikonov, G. I. J. Organomet. Chem. 2001, 635, 24.
51. (i) Nikonov, G. I.; Mountford, P.; Ignatov, S. K.; Green, J. C.; Leech, M. A.; Kuzmina, L. G.; Razuvaev, A. G.; Rees, N. H.; Blake, A. J.; Howard, J. A. K.; Lemenovskii, D. A. J. Chem. Soc., Dalton Trans. 2001, 2903.
52. (j) Spaltenstein, E.; Palma, P.; Kreutzer, K. A.; Willoughby, C. A.; Davis, W. M.; Buchwald, S. L. J. Am. Chem. Soc. 1994, 116, 10308.
53. 0 silyl complexes, see, e.g. ,(a) Xue, Z.; Li, L.; Hoyt, L. K.; Diminnie, J. B.; Pollitte, J. L. J. Am. Chem. Soc. 1994, 116, 2169.
54. (b) McAlexander, L. H.; Hung, M.; Li, L.; Diminnie, J. B.; Xue, Z.; Yap, G. P. A.; Rheingold, A. L. Organometallics 1996, 15, 5231.
55. (c) Diminnie, J. B.; Hall, H. D.; Xue, Z. Chem. Commun. 1996, 2383.
56. (d) Li, L.; Diminnie, J. B.; Liu, X.; Pollitte, J. L.; Xue, Z. Organometallics 1996, 15, 3520.
57. (e) Diminnie, J. B.; Xue, Z. J. Am. Chem. Soc. 1997, 119, 12657.
58. (f) Wu, Z.; Diminnie, J. B.; Xue, Z. Organometallics 1998, 17, 2917.
59. (g) Wu, Z.; McAlexander, L. H.; Diminnie, J. B.; Xue, Z. Organometallics 1998, 17, 4853.
60. (h) Liu, X.-Z.; Li, L.-T.; Diminnie, J. B.; Yap, G. P. A.; Rheingold, A. L.; Xue, Z.-L. Organometallics 1998, 17, 4597.
61. (i) Wu, Z.-Z.; Diminnie, J. B.; Xue, Z.-L. Organometallics 1999, 18, 1002.
62. (j) Wu, Z.-Z.; Diminnie, J. B.; Xue, Z.-L. J. Am. Chem. Soc. 1999, 121, 4300.
63. (k) Choi, S.-H.; Lin, Z.-Y.; Xue, Z.-L. Organometallics 1999, 18, 5488.
64. (l) Wu, Z.-Z.; Xue, Z-L. Organometallics 2000, 19, 4191.
65. (m) Blanton, J. R.; Diminnie, J. B.; Chen, T.-N.; Wiltz, A. M.; Xue, Z.-L. Organometallics 2001, 20, 5542.
66. (n) Blanton, J. R.; Chen, T.-N.; Diminnie, J. B.; Cai, H.; Wu, Z.-Z.; Li, L.-T.; Sorasaenee, K. R.: Quisenberry, K. T.; Pan, H.-J.; Wang, C.-S.; Choi, S.-H.; Wu, Y.-D.; Lin, Z.-Y.; Guzei, I. A.; Rheingold, A. L.; Xue, Z.-L. J. Mol. Catal. A Chem. 2002, 190, 101.
67. (o) Chen, T.-N.; Sorasaenee, K. R.; Wu, Z.-Z.; Diminnie, J. B.; Xue, Z.-L. Inorg. Chim. Acta 2003, 345, 113.
68. (p) Yu, X.-H.; Cai, H.; Guzei, I. A.; Xue, Z.-L. J. Am. Chem. Soc. 2004, 126, 4472.
69. (q) Yu, X.-H.; Bi, S.-W.; Guzei, I. A.; Lin, Z.-Y.; Xue, Z.-L. Inorg. Chem. 2004, 43, 7111.
70. (r) Yu, X.-H.; Xue, Z.-L. Organometallics 2005, 24, 4190.
71. (s) Woods, J. B.; Yu, X.-H.; Chen, T.-N.; Xue, Z.-L. Organometallics 2004, 23, 5910.
72. (t) Qiu, H.; Cai, H.; Woods, J. B.; Wu, Z.-Z.; Chen, T.-N.; Yu, X.-H.; Xue, Z.-L. Organometallics 2005, 24, 4190.
73. (u) Qiu, H.; Chen, S.-J.; Xue, Z.-L. Inorg. Chem. 2007, 46, 6178.
74. (v) Cai, H.; Yu, X.; Chen, S.; Qiu, H.; Guzei, I. A.; Xue, Z.-L. Inorg. Chem. 2007, 46, 8071.
75. (a) Yu, X.-H.; Morton, L. A.; Xue, Z.-L. Organometallics 2004, 23, 2210.
76. (b) Xue, Z.-L. Comments Inorg. Chem. 1996, 18, 223.
77. (c) Chen. T.-N.; Xue, Z.-L. Chin. J. Inorg. Chem. 1999, 15, 413.
78. Jones, T. C; Nielson, A. J.; Rickard, E. F. Chem. Commun. 1984. 205.
79. (a) Chisholm, M. H.; Tan, L.-S.; Huffman, J. C. J. Am. Chem. Soc. 1982, 104, 4879.
80. (b) Chisholm, M. H.; Huffman, J. C; Tan, L.-S. Inorg. Chem. 1981, 20, 1859.
81. Zhang, X.-H.; Chen, S.-J.; Cai, H.; Im, H.-J.; Chen, T.; Yu, X.; Chen, X.; Lin, Z.; Wu, Y.-D.; Xue, Z.-L. Organometallics 2008, 27, 1338.
82. Campion, B. K.; Heyn, R. H.; Tilley, T. D. Organometallics 1993. 12, 2584.
83. (a) Sheldrick, G. M. SADABS, A Program for Empirical Absorption Correction of Area Detector Data; University of Göttingen: Göttingen, Germany, 2000.
84. (b) Sheldrick, G. M. SHELXL-97, A Program for the Refinement of Crystal Structures; University of Göttingen: Göttingen, Germany, 1997.