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The remarkable difference in fluorescence quenching relates to the different fluorescence lifetimes that [BPyPDI] 3 and (Ru(CO)Pc] 2 exhibit.
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Despite the large driving force for charge separation, especially evolving from photoexcited [BPyPDI], no additional emission that might be attributable to a charge transfer is seen in the recorded range of up to 900 nm.
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Considering, however, that the [BPyPDIl triplet excited state lifetime is intrinsically shorter than that of the corresponding radical ion pair state, it might be populated but would be spectroscopically invisible to us.
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107
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33845294247
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The [Ru(CO)Pc] triplet excited state is approximated as 1.14 eV, when considering the same singlet-triplet energy gap in ZnPc, but accounting tor a [Ru(CO)Pc] singlet excited state (1.87 eV) that is 007 eV higher than that of ZnPc (see ref 11h).
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