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4 moieties as reported in ref 23. Considering the standard set-up of XRD measurement and observed monoclinic unit structure (dihedral angles: 90° in axes a-b and b-c), such head-to-tail type interactions mainly occur in the internal structure. The XRD pattern and detail structures based on the results of the paper in ref 23 are shown in Supporting Information S4.
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4 moieties as reported in ref 23. Considering the standard set-up of XRD measurement and observed monoclinic unit structure (dihedral angles: 90° in axes a-b and b-c), such head-to-tail type interactions mainly occur in the internal structure. The XRD pattern and detail structures based on the results of the paper in ref 23 are shown in Supporting Information S4.
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The difference between ?S and ?T may be dependent on the freedom degree of exciton motion of excited singlet or triplet state in the crystalline structures. Although in the short-lived singlet state, excitons move freely within the crystalline structure (free excitons), excitons are likely trapped by some defects because of its relatively long lifetime in the triplet state (trapped excitons). Yokoi and Ohba reported that T-T annihilation between free and trapped triplet excitons occurs much faster due to the long-range interaction comparing to the one between two free excitons. Careful screening of the difference in our system is currently underway. See the reference paper: Yokoi, K.; Ohba, Y. J. Chem. Phys. 1987, 86, 3318.
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The difference between ?S and ?T may be dependent on the freedom degree of exciton motion of excited singlet or triplet state in the crystalline structures. Although in the short-lived singlet state, excitons move freely within the crystalline structure (free excitons), excitons are likely trapped by some defects because of its relatively long lifetime in the triplet state (trapped excitons). Yokoi and Ohba reported that T-T annihilation between free and trapped triplet excitons occurs much faster due to the long-range interaction comparing to the one between two free excitons. Careful screening of the difference in our system is currently underway. See the reference paper: Yokoi, K.; Ohba, Y. J. Chem. Phys. 1987, 86, 3318.
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