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1Py* occurred in our experimental conditions where the ranges of CMP and TMP concentration are 0-0.1 M. For the photoinduced electron-transfer reduction of dC and dT by 7,8,9,10-tetrahydrobenzo[a]pyrene, see: (1) (a) Netzel, T. L.; Zhao, M.; Nafisi, K.; Headrick, J.; Sigman, M. S.; Eaton, B. E. J. Am. Chem. Soc. 1995, 117, 9119.
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(e) Shafirovich, V. Y.; Levin, P. P.; Kuzmin, V. A.; Thorgeirsson, T. E.; Kliger, D. S.; Geacintov, N. E. J. Am. Chem. Soc. 1994, 116, 63.
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105
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18144371974
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note
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10a,40
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106
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18144383870
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note
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28
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107
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0029797271
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Fujita, M.; Ishida, A.; Takamuku, S.; Fukuzumi, S. J. Am. Chem. Soc. 1996, 118, 8566.
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Fujita, M.1
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108
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18144397460
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note
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In the case of triphenylene, photoinduced electron transfer should also occur from all types of DNA bases to the singlet excited state of triphenylene judging from the exothermicity of the electron transfer. However, the absence of absorbance at 355 nm of tripehnylene has precluded the confirmation of the occurrence of photoinduced electron transfer from all types of DNA to the singlet excited state of triphenylene by using our laser system.
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109
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0000419654
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+. See: Kikuchi, K.; Sato, C.; Watabe, M.; Ikeda, H.; Takahashi, Y.; Miyashi, T. J. Am. Chem. Soc. 1993, 115, 5180.
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Kikuchi, K.1
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0028513696
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51b See: O'Connor, D.; Shafirovich, V. Y.; Geacintov, N. E. J. Phys. Chem. 1994, 98, 9831.
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O'Connor, D.1
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116
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18144375220
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note
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1Py*-GMP. Similar transient absorption has been reported in ref 30.
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117
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0011607722
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Transient absorption spectra of a pyrene solution were measured with low-power laser irradiation (1.0 mJ/pulse). When high-power laser irradiation (> 10 mJ/pulse) is employed, the pyrene radical cation and the radical anion are also produced. See: Watkins, A. R. J. Phys. Chem. 1976, 80, 713.
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Watkins, A.R.1
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118
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18144401659
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note
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max = 430 nm) was observed in the absence of nucleotides in Tris/HCl buffer at pH 7.0.
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119
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18144374155
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note
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3+ are also only slightly slower than those of the single-stranded oligonucleotide; see ref 32a.
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