Nuclear magnetic resonance and dielectric noise study of spectral densities and correlation functions in the glass forming monoalcohol 2-ethyl-1-hexanol

Journal of Chemical Physics

Volumn 135, Issue 17, 2011, Pages

  Schildmann, S ^a   Reiser, A ^b   Gainaru, R ^a   Gainaru, C ^a   Bohmer R ^a  

^a TU DORTMUND UNIVERSITY   (Germany)

^b UNIVERSITY OF HEIDELBERG   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

2-ETHYL-1-HEXANOL; CORRELATION FUNCTION; DEBYE PROCESS; ELECTRICAL FIELD; GLASS FORMER; GLASS-FORMING; MONOHYDROXY ALCOHOLS; NMR TECHNIQUES; NOISE SPECTROSCOPY; ORIENTATIONAL FLUCTUATIONS; TRANSLATIONAL CORRELATIONS; VOLTAGE FLUCTUATIONS;

ALCOHOLS; DEUTERIUM; GLASS; INTERNET PROTOCOLS; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; RESONANCE; SPECTRAL DENSITY; STRUCTURAL DYNAMICS; STRUCTURAL RELAXATION;

NUCLEAR MAGNETIC RESONANCE;

EID: 80855156834     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.3647954     Document Type: Article

References (103)

1. J. C. Dyre, Rev. Mod. Phys. 78, 953 (2006). 10.1103/RevModPhys.78.953 (Pubitemid 44496728)
2. R. O. Davies and G. O. Jones, Proc. R. Soc. London 217, 26 (1953); 10.1098/rspa.1953.0044
3. R. O. Davies and G. O. Jones, Adv. Phys. 2, 370 (1953). 10.1080/00018735300101252
4. P. Lunkenheimer, R. Wehn, U. Schneider, and A. Loidl, Phys. Rev. Lett. 95, 055702 (2005). 10.1103/PhysRevLett.95.055702 (Pubitemid 41509222)
5. C. Gainaru and R. Bhmer, J. Non-Cryst. Solids 356, 542 (2010). 10.1016/j.jnoncrysol.2009.07.030
6. P. Debije, Verh. Dtsch. Phys. Ges. 15, 777 (1913).
7. D. C. Davidson and R. H. Cole, J. Chem. Phys. 19, 1484 (1951). 10.1063/1.1748105
8. C. Hansen, F. Stickel, T. Berger, R. Richert, and E. W. Fischer, J. Chem. Phys. 107, 1086 (1997). 10.1063/1.474456
9. T. Lyon and T. A. Litovitz, J. Appl. Phys. 27, 179 (1956). 10.1063/1.1722331
10. R. Kono, T. A. Litovitz, and G. E. McDuffie, J. Chem. Phys. 45, 1790 (1966). 10.1063/1.1727831
11. B. Jakobsen, C. Maggi, T. Christensen, and J. C. Dyre, J. Chem. Phys. 129, 184502 (2008). 10.1063/1.3007988
12. V. Crupi, S. Magaz, G. Maisano, D. Majolino, and P. Migliardo, J. Phys.: Condens. Matter 5, 6819 (1993); 10.1088/0953-8984/5/37/003
13. Y. Takagi, T. Yano, M. Mikami, and S. Kojima, Physica B 263-264, 306 (1999). 10.1016/S0921-4526(98)01229-0
14. H. Huth, L.-M. Wang, C. Schick, and R. Richert, J. Chem. Phys. 126, 104503 (2007). 10.1063/1.2539105 (Pubitemid 46440091)
15. G. Power, M. Nagaraj, J. K. Vij, and G. P. Johari, J. Chem. Phys. 134, 044525 (2011). 10.1063/1.3543713
16. S. S. N. Murthy and M. Tyagi, J. Chem. Phys. 117, 3837 (2002). 10.1063/1.1494428 (Pubitemid 35000309)
17. R. Coelho and D. K. Manh, C. R. Acad. Sci. Paris 264, 641 (1967).
18. J. Crossley and G. Williams, J. Chem. Soc., Faraday Trans. 2 73, 1906 (1977). 10.1039/f29777301906
19. M. Maroncelli and G. R. Fleming, J. Chem. Phys. 86, 6221 (1987); 10.1063/1.452460
20. H. Wendt and R. Richert, J. Phys. Chem. A 102, 5775 (1998). 10.1021/jp981613p
21. Dielectric noise spectroscopy as a tool to study the dynamics of small-molecule liquids has been utilized, e.g., in N. E. Israeloff, Phys. Rev. B 53, R11913 (1996); 10.1103/PhysRevB.53.R11913
22. M. Lucchesi, A. Dominjon, S. Capaccioli, D. Prevosto, and P. A. Rolla, J. Non-Cryst. Solids 352, 4920 (2006). 10.1016/j.jnoncrysol.2006.02.153 (Pubitemid 44647059)
23. R. Wemelle, C. R. Acad. Sci. Paris 244, 775 (1957).
24. S. S. N. Murthy, J. Phys. Chem. 100, 8508 (1996). 10.1021/jp953596z
25. L.-M. Wang and R. Richert, J. Chem. Phys. 120, 11082 (2004). 10.1063/1.1751393
26. L.-M. Wang and R. Richert, J. Chem. Phys. 121, 11170 (2004). 10.1063/1.1811072 (Pubitemid 40025619)
27. C. Gainaru, S. Kastner, F. Mayr, P. Lunkenheimer, S. Schildmann, H. J. Weber, W. Hiller, A. Loidl, and R. Bhmer, Phys. Rev. Lett. 107, 118304 (2011). 10.1103/PhysRevLett.107.118304
28. D. Kruk, A. Herrmann, and E. A. Rssler, Field-cycling NMR relaxometry of viscous liquids and polymers, Prog. Nucl. Magn. Reson. Spectrosc. (in press).
29. C. Gainaru, R. Meier, S. Schildmann, C. Lederle, W. Hiller, E. A. Rssler, and R. Bhmer, Phys. Rev. Lett. 105, 258303 (2010). 10.1103/PhysRevLett.105. 258303
30. B. M. Fung and T. W. McGaughy, J. Chem. Phys. 65, 2970 (1976). 10.1063/1.433533
31. H. Nadolny, A. Volmari, and H. Weingrtner, Ber. Bunsenges. Phys. Chem. 102, 866 (1998).
32. M. Butsch and H. Sillescu, private communication (March 2006).
33. H. Versmold, Ber. Bunsenges. Phys. Chem. 78, 1318 (1974);
34. H. G. Hertz, T. Wild, and H. Weingrtner, Z. Phys. Chem. 140, 71 (1984); 10.1524/zpch.1984.140.1.071
35. R. Ludwig, M. D. Zeidler, and T. C. Farrar, Z. Phys. Chem. 189, 19 (1995). 10.1524/zpch.1995.189.Part-1.019
36. M. Pschl and H. G. Hertz, J. Phys. Chem. 98, 8195 (1994). 10.1021/j100084a043
37. M. Pschl, G. Althoff, S. Killie, E. Wenning, and H. G. Hertz, Ber. Bunsenges. Phys. Chem. 95, 1084 (1991).
38. T. Frech and H. G. Hertz, Ber. Bunsenges. Phys. Chem. 89, 948 (1985).
39. C. Lederle, W. Hiller, C. Gainaru, and R. Bhmer, J. Chem. Phys. 134, 064512 (2011). 10.1063/1.3549123
40. An NMR study of 1-octanol is K. Hu, Y. Zhou, J. Shen, Z. Ji, and G. Cheng, J. Phys. Chem. B 111, 10160 (2007). 10.1021/jp072847o (Pubitemid 47388019)
41. An excellent review of this subject is given by G. Williams, Chem. Soc. Rev. 7, 89 (1978). 10.1039/cs9780700089
42. K. Schmidt-Rohr and H. W. Spiess, Multidimensional Solid-State NMR and Polymers (Academic, London, 1994).
43. R. Bhmer, G. Diezemann, G. Hinze, and E. Rssler, Prog. Nucl. Magn. Reson. Spectrosc. 39, 191 (2001). 10.1016/S0079-6565(01)00036-X (Pubitemid 33005848)
44. Including the shear viscosity of 2E1H, see CRC-Handbook of Chemistry and Physics, 85 th ed., edited by, D. R. Lide, (CRC, Boca Raton, Florida, 2002).
45. D. W. McCall and D. C. Douglass, J. Chem. Phys. 32, 1876 (1960); 10.1063/1.1731042
46. M. Iwahashi, Y. Ohbu, T. Kato, Y. Suzuki, and K. Yamauchi, Bull. Chem. Soc. Jpn. 59, 3771 (1986); 10.1246/bcsj.59.3771
47. R. L. Hurle, A. J. Easteal, and L. A. Woolf, J. Chem. Soc. Faraday Trans. 1 81, 769 (1985); 10.1039/f19858100769
48. S. Meckl and M. D. Zeidler, Mol. Phys. 63, 85 (1988). 10.1080/00268978800100081
49. N. Shaker-Gaafar, N. Karger, S. Wappmann, and H. D. Ldemann, Ber. Bunsenges. Phys. Chem. 97, 805 (1993);
50. N. Karger, S. Wappmann, N. Shaker-Gaafar, and H. D. Ldemann, J. Mol. Liq. 64, 211 (1995). 10.1016/0167-7322(95)00810-W
51. C. M. Roland, S. Hensel-Bielowka, M. Paluch, and R. Casalini, Rep. Prog. Phys. 68, 1405 (2005). 10.1088/0034-4885/68/6/R03 (Pubitemid 40906221)
52. D. Fragiadakis, C. M. Roland, and R. Casalini, J. Chem. Phys. 132, 144505 (2010). 10.1063/1.3374820
53. A. Reiser, G. Kasper, C. Gainaru, and R. Bhmer, J. Chem. Phys. 132, 181101 (2010). 10.1063/1.3421555
54. S. Pawlus, M. Paluch, and A. Grzybowski, J. Chem. Phys. 134, 041103 (2011). 10.1063/1.3540636
55. J. L. MacCallum and D. P. Tieleman, J. Am. Chem. Soc. 124, 5085 (2002). 10.1021/ja027422o (Pubitemid 36014117)
56. B. Geil, Concepts Magn. Reson. 10, 299 (1998). 10.1002/(SICI)1099- 0534(1998)10:5299::AID-CMR33.0.CO;2-S
57. M. Holz, S. R. Heil, and A. Sacco, Phys. Chem. Chem. Phys. 2, 4740 (2000). 10.1039/b005319h
58. J. Schindele, A. Reiser, and C. Enss, Phys. Rev. Lett. 107, 095701 (2011). 10.1103/PhysRevLett.107.095701
59. See, e.g., R. Mller, Rauschen (Springer, Berlin, 1990);
60. S. Kogan, Electronic Noise and Fluctuations in Solids (Cambidge University Press, Cambridge, 1996).
61. J. B. Johnson, Phys. Rev. 32, 97 (1928); 10.1103/PhysRev.32.97
62. H. Nyquist, Phys. Rev. 32, 110 (1928). 10.1103/PhysRev.32.110
63. C. Schmidt, K. J. Kuhn, and H. W. Spiess, Prog. Colloid Polym. Sci. 71, 71 (1985). 10.1007/BFb0114006
64. N. Bloembergen, E. M. Purcell, and R. V. Pound, Phys. Rev. 73, 679 (1948). 10.1103/PhysRev.73.679
65. See, e.g., G. Diezemann and H. Sillescu, J. Chem. Phys. 103, 6385 (1995). 10.1063/1.470418
66. P. A. Beckmann, Phys. Rep. 171, 86 (1988). 10.1016/0370-1573(88)90073-7
67. Th. Dries, F. Fujara, M. Kiebel, E. Rssler, and H. Sillescu, J. Chem. Phys. 88, 2139 (1988); 10.1063/1.454047
68. Th. Dries, F. Fujara, M. Kiebel, E. Rssler, and H. Sillescu, J. Chem. Phys. 90, 7613 (1990); 10.1063/1.456708
69. W. Schnauss, F. Fujara, and H. Sillescu, J. Chem. Phys. 97, 1378 (1992). 10.1063/1.463264
70. E. Rssler and H. Sillescu, Chem. Phys. Lett. 112, 94 (1984). 10.1016/0009-2614(84)87048-7
71. A. Kudlik, Ph.D. dissertation, Universitt Bayreuth, 1997.
72. I. Chang, F. Fujara, B. Geil, G. Heuberger, T. Mangel, and H. Sillescu, J. Non-Cryst. Solids 172-174, 248 (1994); 10.1016/0022-3093(94)90443-X
73. B. Geil, F. Fujara, and H. Sillescu, J. Magn. Reson. 130, 18 (1998); 10.1006/jmre.1997.1284
74. G. Hinze, Phys. Rev. E 57, 2010 (1998); 10.1103/PhysRevE.57.2010
75. R. Bhmer and G. Hinze, J. Chem. Phys. 109, 241 (1998); see also Ref.. 10.1063/1.476557 (Pubitemid 128678822)
76. F. Qi, R. Bhmer, and H. Sillescu, Phys. Chem. Chem. Phys. 3, 4022 (2001). 10.1039/b102391h (Pubitemid 32911690)
77. M. Vogel and E. Rssler, J. Chem. Phys. 115, 10883 (2001). 10.1063/1.1415495 (Pubitemid 34063673)
78. An informative review on Johari-Goldstein relaxations also in monohydroxy alcohols was recently published by J. K. Vij and G. Power, J. Non-Cryst. Solids 357, 783 (2011). 10.1016/j.jnoncrysol.2010.07.067
79. G. Fleischer and F. Fujara, in NMR-Basic Principles and Progress, edited by, P. Diehl, E. Fluck, H. Gnther, R. Kosfeld, and, J. Seelig, (Springer, Berlin, 1994), Vol. 30, pp. 159-207, see their Fig..
80. I. Chang and H. Sillescu, J. Phys. Chem. B 101, 8794 (1997). 10.1021/jp9640989
81. J. T. Edward, J. Chem. Educ. 47, 261 (1970). 10.1021/ed047p261
82. M. A. Floriano and C. A. Angell, J. Chem. Phys. 91, 2537 (1989). 10.1063/1.457013
83. A few examples are K. S. Vahvaselk, R. Serimaa, and M. Torkkeli, J. Appl. Cryst. 28, 189 (1995); 10.1107/S0021889894010149
84. M. Tomsic, A. Jamnik, G. Fritz-Popovski, O. Glatter, and L. Vlcek, J. Phys. Chem. B 111, 1738 (2007) and references cited therein. 10.1021/jp066139z (Pubitemid 46384267)
85. A few examples are G. Oster and J. G. Kirkwood, J. Chem. Phys. 11, 175 (1943); 10.1063/1.1723823
86. W. Dannhauser and R. H. Cole, J. Chem. Phys. 23, 1762 (1955); 10.1063/1.1740576
87. R. Minami, K. Itoh, H. Takahashi, and K. Higasi, J. Chem. Phys. 73, 3396 (1980). 10.1063/1.440536
88. Recent examples are L. Zoranik, F. Sokolic, and A. Perera, J. Chem. Phys. 127, 024502 (2007); 10.1063/1.2753482 (Pubitemid 47130428)
89. S. K. Stephenson, R. D. Offeman, G. H. Robertson, and W. J. Orts, Chem. Eng. Sci. 62, 3019 (2007); 10.1016/j.ces.2007.03.007 (Pubitemid 46653866)
90. J. Lehtola, M. Hakala, and K. Hmlinen, J. Phys. Chem. B 114, 6426 (2010); see also Ref.. 10.1021/jp909894y
91. See, e.g., M. E. Baur and H. Stockmayer, J. Chem. Phys. 43, 4319 (1965). 10.1063/1.1696691
92. See, e.g., J. A. Saxton, R. A. Bond, G. T. Coats, and R. M. Dickinson, J. Chem. Phys. 37, 2132 (1962). 10.1063/1.1733434
93. F. C. Hagemeister, C. J. Gruenloh, and T. S. Zwier, J. Phys. Chem. A 102, 82 (1998). 10.1021/jp963763a
94. M. A. Czarnecki and K. Orzechowski, J. Phys. Chem. A 107, 1119 (2003). 10.1021/jp026384s
95. H. Jansson and J. Swenson, J. Chem. Phys. 134, 104504 (2011). 10.1063/1.3563630
96. C. Gainaru, S. Schildmann, and R. Bhmer, Surface and confinement effects on the dielectric relaxation of a monohydroxy alcohol., J. Chem. Phys. 135, 174510 (2011). 10.1063/1.3655356
97. C. Dalle-Ferrier, C. Thibierge, C. Alba-Simionesco, L. Berthier, G. Biroli, J.-P. Bouchaud, F. Ladieu, D. L'Hte, and G. Tarjus, Phys. Rev. E 76, 041510 (2007). 10.1103/PhysRevE.76.041510 (Pubitemid 350023311)
98. g the number of correlated 2E1H molecules is of the order of 20. See C. Maggi, Presentation at the International Workshop on Fragility of Viscous Liquids: Cause(s) and Consequences, Copenhagen, 8-10 October 2008 (http://glass.ruc.dk/fragility/ proceedings/Maggi.pdf) and Ref..
99. C. Gainaru, W. Hiller, and R. Bhmer, Macromolecules 43, 1907 (2010). 10.1021/ma9026383
100. W. Huang and R. Richert, J. Chem. Phys. 130, 194509 (2009). 10.1063/1.3139519
101. T. Matsuo, H. Suga, and S. Seki, Bull. Chem. Soc. Jpn. 39, 1827 (1966); 10.1246/bcsj.39.1827
102. T. Matsuo, H. Suga, and S. Seki, J. Phys. Soc. Jpn. 22, 677 (1967); 10.1143/JPSJ.22.677
103. J. L. Green, K. Ito, K. Xu, and C. A. Angell, J. Phys. Chem. B 103, 3991 (1999). 10.1021/jp983927i