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While it is likely that the (111) plane defined by the locations of the fourfold coordinated adsorption sites remains a boundary of one twin crystallite, this is not obvious for the other twin crystallite boundary starting out as a (100) plane. From the STM topographs it appears that the width of the defective area between the two crystallites stays limited to several nanometer even for the thickest deposited films. Thus, the initial (100) facet probably does not stay in this orientation for thicker films.
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While it is likely that the (111) plane defined by the locations of the fourfold coordinated adsorption sites remains a boundary of one twin crystallite, this is not obvious for the other twin crystallite boundary starting out as a (100) plane. From the STM topographs it appears that the width of the defective area between the two crystallites stays limited to several nanometer even for the thickest deposited films. Thus, the initial (100) facet probably does not stay in this orientation for thicker films.
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