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The disparity in yield for the 5- and 27-ps time regimes may suggest that the dynamics involve bifurcation with two types of trajectories: those that are direct and lead to a large c-axis structural change (low yield) and those that concurrently involve expansion and lattice relaxation (high yield) (33).
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The disparity in yield for the 5- and 27-ps time regimes may suggest that the dynamics involve bifurcation with two types of trajectories: those that are direct and lead to a large c-axis structural change (low yield) and those that concurrently involve expansion and lattice relaxation (high yield) (33).
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The anisotropy of expansion has been addressed in detail in (21). In this case, the sample is free to expand along the surface normal direction, whereas in a-b planes, the laser-excited region is constrained by the surrounding unexcited region. Moreover, for in-plane charge transfer, the Coulomb repulsion is mainly interplanar, which results in a substantial expansion along the c axis with essentially no lattice change in the a-b planes.
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This work was supported at Caltech by the Gordon and Betty Moore Foundation and NSF and at BNL by the U.S. Department of Energy contract number MA-509-MACA, We thank P. Baum in the UEC laboratory and P. Cao in J. Heath's group at Caltech for AFM imaging; V. Butko, C. Deville-Cavelin, and L. Howald at BNL for XRD, AFM, and transport measurements; and Z. Radovic and N. Bozovic at BNL for the cohesive energy calculations
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This work was supported at Caltech by the Gordon and Betty Moore Foundation and NSF and at BNL by the U.S. Department of Energy (contract number MA-509-MACA). We thank P. Baum in the UEC laboratory and P. Cao in J. Heath's group at Caltech for AFM imaging; V. Butko, C. Deville-Cavelin, and L. Howald at BNL for XRD, AFM, and transport measurements; and Z. Radovic and N. Bozovic at BNL for the cohesive energy calculations.
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