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2 ions followed by annealing to 400°C for 1 min. The sample was then transferred into the precooled 5TM, and Mn atoms were subsequently evaporated onto the surface.
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Mn was transferred to the tip from either the CuN or bare Cu surface by moving the tip into point contact with the atom and then withdrawing the tip while applying +2 V. The atom was then transferred to the CuN by repeating this procedure with -0.5 V. Mn atoms can bind to the CuN atop either a Cu or N atom, with the Cu site being more stable.
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The conductance steps at low fields on Mn atoms and trimers are too narrow to resolve the flat bottom that clearly differentiates an IETS line shape from the Fano line shape that characterizes the Kondo effect (15, 16). Because this flat bottom is seen on longer chains, we consider the Kondo interpretation to be unlikely for the shorter chains as well.
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A and N. We therefore limited our calculations to N ≤ 6.
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note
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STM topographic images were processed using WSxM (www.nanotec.es). We thank D. M. Eigler for mentoring and stimulating discussions; B. J. Melior for expert technical assistance; and C.-Y. Lin and B. A. Jones for stimulating discussions.
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