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Measurements of electron bunch length and energy spread as they evolve through the SLAC linac are in good agreement with the particle tracking codes used to predict 80-fs bunches. Measurements by interferometric autocorrelation of the coherent transition radiation from the electron bunches are also consistent with 80-fs electron bunches. These independent measurements provide strong evidence that our estimates of the x-ray pulse duration as well as the pulse shape at optimal compression are accurate.
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The measured time constants are in good agreement with the average of the time constants extracted from each image. By comparing our measurements with independent measurements of the electron-bunch arrival time, we estimate that the relative timing of laser and x-rays from shot to shot can be determined to better than 60 fs by spatially recording the midpoint of the sudden drop in diffracted intensity (28).
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Portions of this research were supported by the U.S. Department of Energy, Office of Basic Energy Science, through direct support for the SPPS and individual investigators and through the Stanford Synchrotron Radiation Laboratory, a national user facility operated by Stanford University. Additional support for the construction of SPPS was provided in part by Uppsala University and the Swedish Research CounciL K.S.-T., D.V.D.L., and S.T. gratefully acknowledge financial support by the Deutsche Forschungsgemeinschaft. J.L., O.S., T.N.H., K.S.-T., and D.V.D.L. acknowledge the support of the European Commission through the FAMTO, X-RAY FEL PUMP-PROBE, and XPOSE projects. J.L. acknowledges the support from Wallenberg Research Link and the Swedish Foundation for Strategic Research. R.W.F. acknowledges support from the U.S. Department of Energy through the High Energy Density Science Grants Program and through a collaboration with Chemistry and Materials Science at Lawrence Livermore National Laboratory. A.M.L. thanks D. Moncton for useful conversations.
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