Current status of single-molecule spectroscopy: Theoretical aspects

Journal of Chemical Physics

Volumn 117, Issue 24, 2002, Pages 10980-10995

  Jung, YounJoon ^a   Barkai, Eli ^a,b   Silbey, Robert J ^a  

^a MASSACHUSETTS INSTITUTE OF TECHNOLOGY   (United States)

^b UNIVERSITY OF NOTRE DAME   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

BIOMOLECULES; FLUORESCENCE INTENSITY FLUCTUATIONS; PAULI MATRIX; QUANTUM JUMP METHOD; SINGLE MOLECULE REACTION DYNAMICS; SINGLE-MOLECULE SPECTROSCOPY; TIME DEPENDENT LINE SHAPE FLUCTUATIONS;

CHROMOPHORES; FLUORESCENCE; GROUND STATE; HAMILTONIANS; MATRIX ALGEBRA; MOLECULES; PHOTONS; PROBABILITY DENSITY FUNCTION; PROBABILITY DISTRIBUTIONS; RELAXATION PROCESSES; STATISTICAL METHODS; TEMPERATURE;

SPECTROSCOPY;

EID: 0037461515     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1521157     Document Type: Article

References (120)

1. W. E. Moerner and L. Kador, Phys. Rev. Lett. 62, 2535 (1989).
2. M. Orrit and J. Bernard, Phys. Rev. Lett. 65, 2716 (1990).
3. Single-Molecule Optical Detection, Imaging, and Spectroscopy, edited by T. Basché, W. E. Moerner, M. Orrit, and U. P. Wild (VCH, Berlin, 1996).
4. T. Plakhotnik, E. A. Donley, and U. P. Wild, Annu. Rev. Phys. Chem. 48, 181 (1997).
5. X. S. Xie and J. K. Trautman, Annu. Rev. Phys. Chem. 49, 441 (1998).
6. W. E. Moerner and M. Orrit, Science 283, 1670 (1999).
7. S. Weiss, Science 283, 1676 (1999).
8. P. Tamarat, A. Maali, B. Lounis, and M. Orrit, J. Phys. Chem. A 104, 1 (2000).
9. W. E. Moerner, J. Phys. Chem. B 106, 910 (2002).
10. E. Geva and J. L. Skinner, J. Phys. Chem. B 101, 8920 (1997).
11. E. Barkai, R. Silbey, and G. Zumofen, Phys. Rev. Lett. 84, 5339 (2000).
12. E. Barkai, Y. Jung, and R. J. Silbey, Phys. Rev. Lett. 87, 207403 (2001).
13. Y. Jung, E. Barkai, and R. J. Silbey, Adv. Chem. Phys. 123, 199 (2002).
14. H. P. Lu, L. Y. Xun, and X. S. Xie, Science 282, 1877 (1998).
15. X. Zhuang, L. E. Bartley, H. P. Babcock, R. Russell, T. Ha, D. Herschlag, and S. Chu, Science 288, 2048 (2000).
16. L. Kador, T. Latychevskaia, A. Renn, and U. P. Wild, J. Chem. Phys. 111, 8755 (1999).
17. W. P. Ambrose, T. Basché, and W. E. Moerner, J. Chem. Phys. 95, 7150 (1991).
18. L. Fleury, A. Zumbusch, M. Orrit, R. Brown, and J. Bernard, J. Lumin. 56, 15 (1993).
19. A.-M. Boiron, Ph. Tamarat, B. Lounis, R. Brown, and M. Orrit, Chem. Phys. 247, 119 (1999).
20. A. V. Naumov, Y. G. Vainer, M. Bauer, S. Zilker, and L. Kador, Phys. Rev. B 63, 212302 (2001).
21. L. Mandel and E. Wolf, Optical Coherence and Quantum Optics (Cambridge University Press, New York, 1995).
22. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, Oxford, 1995).
23. L. R. Narasimhan, K. A. Littau, D. W. Pack, Y. Bai, A. Elschner, and M. D. Fayer, Chem. Rev. 90, 439 (1990).
24. J. Bernard, L. Fleury, H. Talon, and M. Orrit, J. Chem. Phys. 98, 850 (1993).
25. T. Basché, S. Kummer, and C. Bräuchle, Nature (London) 373, 132 (1995).
26. A. C. J. Brouwer, E. J. J. Groenen, and J. Schmidt, Phys. Rev. Lett. 80, 3944 (1998).
27. T. Ha, T. Enderle, D. F. Ogletree, D. S. Chemla, P. R. Selvin, and S. Weiss, Proc. Natl. Acad. Sci. (USA) 93, 6264 (1996).
28. D. A. Vanden Bout, W. Yip, D. Hu, D. Fu, T. M. Swager, and P. F. Barbara, Science 277, 1074 (1997).
29. W. Yip, D. Hu, J. Yu, D. A. Vanden Bout, and P. F. Barbara, J. Phys. Chem. A 102, 7564 (1998).
30. H. Bach, A. Renn, G. Zumofen, and U. P. Wild, Phys. Rev. Lett. 82, 2195 (1999).
31. J. Wang and P. G. Wolynes, Phys. Rev. Lett. 74, 4317 (1995).
32. V. Chernyak, M. Schulz, and S. Mukamel, J. Chem. Phys. 111, 7416 (1999)
33. A. M. Berezhkovskii, A. Szabo, and G. H. Weiss, J. Phys. Chem. B 104, 3776 (2000).
34. G. K. Schenter, H. P. Lu, and X. S. Xie, J. Phys. Chem. A 103, 10477 (1999).
35. N. Agmon, J. Phys. Chem. B 104, 7830 (2000).
36. J. Cao, Chem. Phys. Lett. 327, 38 (2000).
37. S. Yang and J. Cao, J. Phys. Chem. B 105, 6536 (2001).
38. T. Ha, T. Enderle, D. S. Chemla, P. R. Selvin, and S. Weiss, Phys. Rev. Lett. 77, 3979 (1996).
39. T. Ha, J. Glass, T. Enderle, D. S. Chemla, and S. Weiss, Phys. Rev. Lett. 80, 2093 (1998).
40. L. Edman, J. Phys. Chem. A 104, 6165 (2000).
41. W. P. Ambrose and W. E. Moerner, Nature (London) 349, 225 (1991).
42. A. Zumbusch, L. Fleury, R. Brown, J. Bernard, and M. Orrit, Phys. Rev. Lett. 70, 3584 (1993).
43. C. Cohen-Tannoudji, J. Dupon-Roc, and G. Grynberg, Atom Photon Interaction (Wiley, New York, 1993).
44. R. Loudon, The Quantum Theory of Light, 2nd ed. (Oxford University Press, Oxford, 1983).
45. K. D. Weston, P. J. Carson, H. Metiu, and S. K. Buratto, J. Chem. Phys. 109, 7474 (1998).
46. I. S. Osad'ko, J. Exp. Theor. Phys. 86, 875 (1998).
47. I. S. Osad'ko, J. Exp. Theor. Phys. 89, 513 (1999).
48. L. Fleury, J.-M. Segura, G. Zumofen, B. Hecht, and U. P. Wild, Phys. Rev. Lett. 84, 1148 (2000).
49. R. Short and L. Mandel, Phys. Rev. Lett. 51, 384 (1983).
50. M. S. Kim and P. L. Knight, Phys. Rev. A 36, 5265 (1987).
51. Tunneling Systems in Amorphous and Crystalline Solids, edited by P. Esquinazi (Springer, Berlin, 1998).
52. P. W. Anderson, B. I. Halperin, and C. M. Varma, Philos. Mag. 25, 1 (1971).
53. W. A. Phillips, J. Low Temp. Phys. 7, 351 (1972).
54. A. Heuer and R. Silbey, Phys. Rev. Lett. 70, 3911 (1993).
55. B. Kozankiewicz, J. Bernard, and M. Orrit, J. Chem. Phys. 101, 9377 (1994).
56. M. Vacha, Y. Liu, H. Nakatsuka, and T. Tani, J. Chem. Phys. 106, 8324 (1997).
57. F. L. H. Brown and R. J. Silbey, J. Chem. Phys. 108, 7434 (1998).
58. P. D. Reilly and J. L. Skinner, J. Chem. Phys. 101, 959 (1994).
59. P. W. Anderson, J. Phys. Soc. Jpn. 9, 316 (1954).
60. R. Kubo, J. Phys. Soc. Jpn. 9, 935 (1954).
61. T. Plakhotnik, J. Lumin. 83-4, 221 (1999).
62. W. Pfleugl, F. L. H. Brown, and R. J. Silbey, J. Chem. Phys. 108, 6876 (1998).
63. E. Barkai, R. Silbey, and G. Zumofen, J. Chem. Phys. 113, 5853 (2000).
64. J.-P. Bouchaud and A. Georges, Phys. Rep. 4-5, 127 (1990).
65. E. A. Donley, H. Bach, W. P. Wild, and T. Plakhotnik, J. Phys. Chem. A 103, 2282 (1999).
66. E. A. Donley and T. Plakhotnik, J. Chem. Phys. 114, 9993 (2001).
67. P. D. Reilly and J. L. Skinner, Phys. Rev. Lett. 71, 4257 (1993).
68. T. Basché, W. E. Moerner, M. Orrit, and H. Talon, Phys. Rev. Lett. 69, 1516 (1992).
69. T. Plakhotnik and D. Walser, Phys. Rev. Lett. 80, 4064 (1998).
70. T. Plakhotnik, Phys. Rev. B 59, 4658 (1999).
71. R. Kubo, in Fluctuation, Relaxation, and Resonance in Magnetic Systems, Scottish Universities Summer School, edited by D. T. Haar (Oliver and Boyd, Edinburgh and London, 1962).
72. A. Suárez and R. Silbey, Chem. Phys. Lett. 218, 445 (1994).
73. R. M. Dickson, A. B. Cubitt, R. Y. Tsien, and W. E. Moerner, Nature (London) 388, 355 (1997).
74. M. Nirmal, B. O. Dabbousi, M. G. Bawendi, J. J. Macklin, J. K. Trautman, T. D. Harris, and L. E. Brus, Nature (London) 383, 802 (1996).
75. M. Kuno, D. P. Fromm, H. F. Hamann, A. Gallagher, and D. J. Nesbitt, J. Chem. Phys. 112, 3117 (2000).
76. K. Shimizu, R. G. Neuhauser, C. A. Leatherdale, S. A. Empedocles, W.-K. Woo, and M. G. Bawendi, Phys. Rev. B 63, 205316 (2001).
77. G. Messin, J. P. Hermier, E. Giacobino, P. Desbiolles, and M. Dahan, Opt. Lett. 26, 1891 (2001).
78. J. Hofkens, M. Maus, T. Gensch, T. Vosch, M. Cotlet, F. Kohn, A. Herrmann, and K. Mullen, J. Am. Chem. Soc. 122, 9278 (2000).
79. J. D. White, J. H. Hsu, S. C. Yang, W. S. Fann, G. Y. Pern, and S. A. Chen, J. Chem. Phys. 114, 3848 (2001).
80. R. Brown, J. Wrachtrup, M. Orrit, J. Bernard, and C. von Borczyskowski, J. Chem. Phys. 100, 7182 (1994).
81. I. S. Osad'ko and L. B. Yershova, J. Chem. Phys. 112, 9645 (2000).
82. A. Molski, J. Hofkens, T. Gensch, N. Boens, and F. de Schryver, Chem. Phys. Lett. 318, 325 (2000).
83. S. Kummer, S. Mais, and T. Basché, J. Phys. Chem. 99, 17078 (1995).
84. B. Lounis, H. A. Bechtel, D. Gerion, A. P. Alivisatos, and W. E. Moerner, Chem. Phys. Lett. 329, 399 (2000).
85. P. Michler, A. Imamoglu, M. D. Mason, P. J. Carson, G. F. Strouse, and S. K. Buratto, Nature (London) 406, 968 (2000).
86. Y. Jung, E. Barkai, and R. J. Silbey, Chem. Phys. 284, 181 (2002).
87. G. Zumofen and J. Klafter, Phys. Rev. E 47, 851 (1993).
88. (2)(τ) is obtained from the time average, instead of the ensemble average, as done in Ref. 79, Eq. (2.10) yields a result consistent with the experiments.
89. U. Banin, M. Bruchez, A. P. Alivisatos, T. Ha, S. Weiss, and D. S. Chemla, J. Chem. Phys. 110, 1195 (1999).
90. E. L. Efros and M. Rosen, Phys. Rev. Lett. 78, 1110 (1997).
91. G. H. Weiss, Aspects and Applications of the Random Walks (North-Holland, Amsterdam, 1994).
92. L. Edman, U. Mets, and R. Rigler, Proc. Natl. Acad. Sci (USA) 93, 6710 (1996).
93. S. Wennmalm, L. Edman, and R. Rigler, Proc. Natl. Acad. Sci (USA) 94, 10641 (1997).
94. Y. Jia, A. Sytnik, L. Li, S. Vladimirov, B. S. Cooperman, and R. M. Hochstrasser, Proc. Natl. Acad. Sci. (USA) 94, 7932 (1997).
95. E. Geva and J. L. Skinner, Chem. Phys. Lett. 288, 225 (1998).
96. A. M. Berezhkovskii, A. Szabo, and G. H. Weiss, J. Chem. Phys. 110, 9145 (1999).
97. R. Zwanzig, Acc. Chem. Res. 23, 148 (1990).
98. H. Frauenfelder, S. G. Sligar, and P. G. Wolynes, Science 254, 1598 (1991).
99. J. Wang and P. Wolynes, J. Chem. Phys. 110, 4812 (1999).
100. J. Onuchic, J. Wang, and P. G. Wolynes, Chem. Phys. 247, 175 (1999).
101. M. Boguñá, A. M. Berezhkovskii, and G. H. Weiss, Physica A 282, 475 (2000).
102. M. Boguñá and G. H. Weiss, Physica A 282, 486 (2000).
103. M. Boguñá, J. Masoliver, and G. H. Weiss, Physica A 284, 13 (2000).
104. K. Blum, Density Matrix Theory and Applications (Plenum, New York, 1996).
105. M. B. Plenio and P. L. Knight, Rev. Mod. Phys. 70, 101 (1998).
106. J. Dalibard, Y. Castin, and K. Møllmer, Phys. Rev. Lett. 68, 580 (1992).
107. K. Møllmer, Y. Castin, and J. Dalibard, J. Opt. Soc. Am. B 10, 524 (1993).
108. H. Carmichael, An Open Systems Approach to Quantum Optics, Vol. m18, in Lecture Notes in Physics (Springer-Verlag, Berlin, New York, 1993).
109. D. E. Makarov and H. Metiu, J. Chem. Phys. 111, 10126 (1999).
110. D. E. Makarov and H. Metiu, J. Chem. Phys. 111, 10137 (1999).
111. C. Brunel, B. Lounis, P. Tamarat, and M. Orrit, Phys. Rev. Lett. 83, 2722 (1999).
112. B. Lounis and W. E. Moerner, Nature (London) 407, 491 (2000).
113. D. E. Makarov and H. Metiu, J. Chem. Phys. 115, 5989 (2001).
114. A. M. van Oijen, M. Ketelaars, J. Kohler, T. J. Aartsma, and J. Schmidt, Science 285, 400 (1999).
115. M. Ketelaars, A. M. van Oijen, M. Matsushita, J. Kohler, J. Schmidt, and T. J. Aartsma, Biophys. J. 80, 1591 (2001).
116. M. Matsushita, M. Ketelaars, A. M. van Oijen, J. Kohler, T. J. Aartsma, and J. Schmidt, Biophys. J. 80, 1604 (2001).
117. M. V. Mostovoy and J. Knoester, J. Phys. Chem. B 104, 12355 (2000).
118. S. E. Dempster, S. Jang, and R. J. Silbey, J. Chem. Phys. 114, 10015 (2001).
119. S. Jang, S. E. Dempster, and R. J. Silbey, J. Phys. Chem. B 105, 6655 (2001).
120. J. M. Caruge and M. Orrit, Phys. Rev. B 64, 205202 (2001).