An investigation of the effects of two level system coupling on single molecule lineshapes in low temperature glasses

Journal of Chemical Physics

Volumn 108, Issue 17, 1998, Pages 7434-7450

  Brown, Frank L H ^a   Silbey, Robert J ^a  

^a MASSACHUSETTS INSTITUTE OF TECHNOLOGY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 0001057526     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.476164     Document Type: Article

References (52)

1. L. Allen and J. Eberly, Optical Resonance and Two-Level Atoms (Dover, New York, 1987).
2. R. M. Macfarlane and R. M. Shelby, J. Lumin. 7, 179 (1987).
3. W. E. Moerner, Persistent Spectral Hole Burning: Science and Applications (Springer, Berlin, 1988).
4. B. M. Kharlamov, R. I. Personov, and L. A. Bykovskaya, Opt. Commun. 12, 191 (1974).
5. D. Harrer and R. Silbey, Physics Today 43. 58 (1990).
6. N. A. Kumit, I. D. Abella, and S. R. Hartmann, Phys. Rev. Lett. 13. 567 (1964).
7. L. R. Narasimhan, Y. S. Bai, M. A. Dugan, and M. D. Fayer, Chem. Phys. Lett. 176, 335 (1991).
8. H. C. Meijers and D. A. Wiersma, Phys. Rev. Lett. 68. 381 (1992).
9. S. Asaka, H. Nakatsuka, M. Fujiwara, and M. Matsuoka, Phys. Rev. A 29, 2286 (1984).
10. N. Morita and T. Yajima, Phys. Rev. A 30, 2525 (1984).
11. R. Beach and R. Hartmann, Phys. Rev. Lett. 53, 663 (1984).
12. W. H. Hesselink and D A. Wiersma, Phys. Rev. Lett. 43, 1991 (1979).
13. W. H. Hesselink and D. A. Wiersma, J. Chem. Phys 75, 4192 (1981).
14. L. Fleury, A. Zumbusch, R. Brown, and J. Bernard, J. Lumin, 56, 1 (1993).
15. B. Kozankiewicz, J. Bernard, and M. Orrit, J. Chem. Phys. 101, 9377 (1994).
16. R. Kettner, J. Tittel, T. Basche, and C. Brauchle, J. Phys. Chem. 98, 6671 (1994).
17. J. Tittel, R. Kenner, T. Basche, C. Brauchle, H. Quante, and K. Mullen, J. Lumin. 64. 1 (1995).
18. E. Geva, P. D. Reilly, and J. L Skinner, Acc. Chem. Res. 29, 579 (1996).
19. P. D. Reilly and J. L. Skinner, J. Chem. Phys. 101, 959 (1994).
20. E. Geva and J. L. Skinner, J. Phys Chem. B 101, 8920 (1997).
21. R. W. Anderson, B. I. Halperin, and C. M. Vanna, Philos, Mag. 25, 1 (1971).
22. W. A. Phillips, J. Low Temp Phys. 7. 351 (1972).
23. R. Kubo, J. Phys. Soc. Jpn. 9, 935 (1954).
24. R. Kubo, in Fluctuation, Relaxation, Resonance in Magnetic Systems, edited by D. TerHaar (Oliver and Boyd, Edinbury, 1962).
25. R. Kubo, Adv. Chem. Phys. 15, 101 (1969).
26. P. W. Anderson, J. Phys. Soc Jpn. 9, 316 (1954).
27. R. C. Zeller and R. O Pohl. Phys. Rev. B 4, 2029 (1971).
28. R. O. Pool, in Amorphous Solids: Low Temperature Properties, edited by W. Phillips (Springer, Berlin, 1981).
29. J. L. Black and B. I. Halperin, Phys. Rev. B 16, 2879 (1977).
30. Y. Tanimura, H. Takano, and J. Klafter, J. Chem. Phys. 108, 1851 (1998).
31. R. Silbey and K. Kassner, J. Lumin. 36, 283 (1987).
32. R. Silbey, in Relaxation Processes in Molecular Excited States, edited by J. Funfschilling (Kluwer Academic, Dordercht, 1989).
33. K. Blum, Density Matrix Theory and Applications (Plenum, New York, 1981).
34. W. H. Louisell, Quantum Statistical Properties of Radiation (Wiley, New York, 1973).
35. D. L. Huber, J. Lumin. 36, 307 (1987).
36. A. Suarez and R. Silbey, J. Phys. Chem. 98, 7329 (1994).
37. K. Kassner and R. Silbey, J. Phys.: Condens. Matter 1, 4599 (1989).
38. P. Reineker and K. Kassner, in Optical Spectroscopy of Glasses, edited by I. Zschokke (Reidel, Dordrecht, 1986).
39. R. G. Gordon, Adv. Magn. Reson. 3, 1 (1968).
40. O. Terzidis and A. Wurger, J. Phys.: Condens. Matter 8, 7303 (1996).
41. J. Joffrin and A. Levelut, J. Phys. (France) 36, 81 (1975).
42. Of course there will be elements of R which couple nondiagonal to nondiagonal, but these elements will not be of interest to us because they are involved in a set of equations uncoupled to ours.
43. H. P. H. Thijssen, R. van den Berg, and S. Volker, Chem. Phys. Lett. 91, 295 (1983).
44. H. P. H. Thijssen, R. van den Berg, and S. Volker, Chem. Phys. Left. 113, 23 (1983).
45. S. Volker, Annu. Rev. Phys. Chem. 40, 499 (1989).
46. A. Heuer and R. Silbey, Phys. Rev. Lett. 70, 3911 (1993); Phys. Rev. B 49, 1441 (1994); 53, 1 (1996).
47. A. Heuer and R. Silbey, Phys. Rev. Lett. 70, 3911 (1993); Phys. Rev. B 49, 1441 (1994); 53, 1 (1996).
48. A. Heuer and R. Silbey, Phys. Rev. Lett. 70, 3911 (1993); Phys. Rev. B 49, 1441 (1994); 53, 1 (1996).
49. J. F. Berret and M. Meissner, Z. Phys. B 70, 65 (1988).
50. W. Pfluegl, F. L. H. Brown, and R. J. Silbey, J. Chem. Phys. 108, 6876 (1998).
51. F. U. H. Brown, Ph.D. thesis, Massachusetts Institute of Technology, 1998.
52. W. E. Moerner, T. Plakhotnik, and T. Irngartinger, J. Phys Chem 98, 7382 (1994).