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Volumn 91, Issue 4, 2015, Pages

Impact of quantized vibrations on the efficiency of interfacial charge separation in photovoltaic devices

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EID: 84921048025     PISSN: 10980121     EISSN: 1550235X     Source Type: Journal    
DOI: 10.1103/PhysRevB.91.041107     Document Type: Article
Times cited : (30)

References (37)
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    • Thermally activated hopping, not captured by the present approach, is anyway not relevant in the regime of moderate electron-phonon coupling (Equation presented) studied here [see, e.g., ()]. PRLTAO 0031-9007 10.1103/PhysRevLett.91.256403
    • Thermally activated hopping, not captured by the present approach, is anyway not relevant in the regime of moderate electron-phonon coupling (Equation presented) studied here [see, e.g., S. Fratini and S. Ciuchi, Phys. Rev. Lett. 91, 256403 (2003)]. PRLTAO 0031-9007 10.1103/PhysRevLett.91.256403
    • (2003) Phys. Rev. Lett. , vol.91 , pp. 256403
    • Fratini, S.1    Ciuchi, S.2
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    • This quantity is related, but not equal, to the internal quantum efficiency commonly extracted from experiments: One cannot directly relate the injection energy (Equation presented) in Eq. (1) to the incoming photon frequency, because a continuum of possible initial electronic states is generated in the highest occupied molecular orbital (HOMO)-lowest unoccupied molecular orbital (LUMO) bands upon absorption of light.
    • This quantity is related, but not equal, to the internal quantum efficiency commonly extracted from experiments: One cannot directly relate the injection energy (Equation presented) in Eq. (1) to the incoming photon frequency, because a continuum of possible initial electronic states is generated in the highest occupied molecular orbital (HOMO)-lowest unoccupied molecular orbital (LUMO) bands upon absorption of light.


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