The detection of nocturnal N2O5 as HNO3by alkali- and aqueous-denuder techniques

Atmospheric Measurement Techniques

Volumn 6, Issue 2, 2013, Pages 231-237

  Phillips, G J ^a   Makkonen, U ^b   Schuster, G ^a   Sobanski, N ^a   Hakola, H ^b   Crowley, J N ^a  

^a MAX PLANCK INSTITUTE FOR CHEMISTRY   (Germany)

^b FINNISH METEOROLOGICAL INSTITUTE   (Finland)

Author keywords

[No Author keywords available]

Indexed keywords

ANTHROPOGENIC EFFECT; CONCENTRATION (COMPOSITION); DETECTION METHOD; MEASUREMENT METHOD; MONITORING; NITRIC ACID; NITROGEN CYCLE; OXIDATION; OXIDE;

EID: 84882638066     PISSN: 18671381     EISSN: 18678548     Source Type: Journal    
DOI: 10.5194/amt-6-231-2013     Document Type: Article

References (42)

1. Aan de Brugh, J. M. J., Henzing, J. S., Schaap, M., Morgan, W. T., van Heerwaarden, C. C., Weijers, E. P., Coe, H., and Krol, M. C.: Modelling the partitioning of ammonium nitrate in the convective boundary layer, Atmos. Chem. Phys., 12, 3005-3023, doi:10.5194/acp-12-3005-2012, 2012.
2. Aas, W., Tsyro, S., Bieber, E., Bergström, R., Ceburnis, D., Ellermann, T., Fagerli, H., Frölich, M., Gehrig, R., Makkonen, U., Nemitz, E., Otjes, R., Perez, N., Perrino, C., Prévôt, A. S. H., Putaud, J.-P., Simpson, D., Spindler, G., Vana, M., and Yttri, K. E.: Lessons learnt from the first EMEP intensive measurement periods, Atmos. Chem. Phys., 12, 8073-8094, doi:10.5194/acp-12-8073-2012, 2012.
3. 5 near Fairbanks, Alaska, J. Geophys. Res.-Atmos., 111, D14309, doi:10.1029/2006JD007070, 2006.
4. 5 reactivity on ambient aerosol particles, Geophys. Res. Lett., 36, L19803, doi:10.1029/2009GL040248, 2009.
5. Brown, S. S. and Stutz, J.: Nighttime radical observations and chemistry, Chem. Soc. Rev., 41, 6405-6447, doi:10.1039/c2cs35181a, 2012.
6. 5 via cavity ring-down spectroscopy, Geophys. Res. Lett., 28, 3227-3230, 2001.
7. 3, J. Geophys. Res.-Atmos., 108, 4299, doi:10.1029/2002JD002917, 2003.
8. 5 through the nocturnal boundary layer, Atmos. Chem. Phys., 7, 139-149, doi:10.5194/acp-7-139-2007, 2007.
9. 3) concentrations, The Scientific World Journal, 1, 815-822, 2001.
10. 5: A review, Aerosol. Sci. Tech., 45, 655-685, 2011.
11. Cowen, K., Hanft, E., Kelly, T., Dindal, A., and McKernan, J.: Environmental technology verification report, ETV advanced monitoring systems center, Applikon MARGA semi-continuous ambient air monitoring system, Battelle, 2011.
12. Crowley, J. N., Ammann, M., Cox, R. A., Hynes, R. G., Jenkin, M. E., Mellouki, A., Rossi, M. J., Troe, J., and Wallington, T. J.: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume V - heterogeneous reactions on solid substrates, Atmos. Chem. Phys., 10, 9059-9223, doi:10.5194/acp-10-9059-2010, 2010a.
13. Crowley, J. N., Schuster, G., Pouvesle, N., Parchatka, U., Fischer, H., Bonn, B., Bingemer, H., and Lelieveld, J.: Nocturnal nitrogen oxides at a rural mountain-site in south-western Germany, Atmos. Chem. Phys., 10, 2795-2812, doi:10.5194/acp-10-2795-2010, 2010b.
14. Dong, H.-B., Zeng, L.-M., Hu, M., Wu, Y.-S., Zhang, Y.-H., Slanina, J., Zheng, M., Wang, Z.-F., and Jansen, R.: Technical Note: The application of an improved gas and aerosol collector for ambient air pollutants in China, Atmos. Chem. Phys., 12, 10519-10533, doi:10.5194/acp-12-10519-2012, 2012.
15. Finlayson-Pitts, B. J., Ezell, M. J., and Pitts, J. N. J.: Formation of chemically active chlorine compounds by reactions of atmospheric nacl particles with gaseous N2O5 and ClONO2, Nature, 337, 241-244, 1989. (Pubitemid 19303781)
16. Finlayson-Pitts, B. J. and Pitts, J. N.: Tropospheric air pollution: Ozone, airborne toxics, polycyclic aromatic hydrocarbons, and particles, Science, 276, 1045-1052, 1997.
17. Flechard, C. R., Nemitz, E., Smith, R. I., Fowler, D., Vermeulen, A. T., Bleeker, A., Erisman, J. W., Simpson, D., Zhang, L., Tang, Y. S., and Sutton, M. A.: Dry deposition of reactive nitrogen to European ecosystems: a comparison of inferential models across the NitroEurope network, Atmos. Chem. Phys., 11, 2703-2728, doi:10.5194/acp-11-2703-2011, 2011.
18. Fowler, D., Ashmore, M., Cape, J. N., Derwent, R. G., Dore, C., Dore, A., Emmett, B., Grennfelt, P., Hall, J., Malcolm, H., Monteith, D., and Smith, R.: Review of transboundary air pollution (RoTAP): Acidification, eutrophication, ground level ozone and heavy metals in the uk, Centre for Ecology and Hydrology, Contract Report to the Department for Environment, Food and Rural Affairs, 2012.
19. Handisides, G. M.: The influence of peroxy radicals on ozone production, Fachbereich Geowissenschaften, Johann Wolfgang Goethe Universität, Frankfurt am Main, 2001.
20. Huebert, B. J. and Robert, C. H.: The dry deposition of nitric acid to grass, J. Geophys. Res.-Atmos., 90, 2085-2090, doi:10.1029/JD090iD01p02085, 1985. (Pubitemid 15463541)
21. Makkonen, U., Virkkula, A., Mäntykenttä, J., Hakola, H., Keronen, P., Vakkari, V., and Aalto, P. P.: Semi-continuous gas and inorganic aerosol measurements at a Finnish urban site: comparisons with filters, nitrogen in aerosol and gas phases, and aerosol acidity, Atmos. Chem. Phys., 12, 5617-5631, doi:10.5194/acp-12-5617-2012, 2012.
22. Markovic, M. Z., VandenBoer, T. C., and Murphy, J. G.: Characterization and optimization of an online system for the simultaneous measurement of atmospheric water-soluble constituents in the gas and particle phases, J. Environ. Monitor., 14, 1872-1884, doi:10.1039/c2em00004k, 2012.
23. 5 in the urban atmosphere by thermal decomposition/laser-induced fluorescence technique, Atmos. Environ., 39, 6802-6811, 2005.
24. 2 in a mid-continental urban environment, Environ. Sci. Technol., 45, 8889-8896, doi:10.1021/es201955u, 2011.
25. 5 in the marine boundary layer during New England air quality study - intercontinental transport and chemical transformation 2004, J. Geophys. Res.-Atmos., 111, D23S14, doi:10.1029/ 2006JD007593, 2006.
26. Osthoff, H. D., Roberts, J. M., Ravishankara, A. R., Williams, E. J., Lerner, B. M., Sommariva, R., Bates, T. S., Coffman, D., Quinn, P. K., Dibb, J. E., Stark, H., Burkholder, J. B., Talukdar, R. K., Meagher, J., Fehsenfeld, F. C., and Brown, S. S.: High levels of nitryl chloride in the polluted subtropical marine boundary layer, Nat. Geosci., 1, 324-328, 2008.
27. Phillips, G. J., Tang, M. J., Thieser, J., Brickwedde, B., Schuster, G., Bohn, B., Lelieveld, J., and Crowley, J. N.: Significant concentrations of nitryl chloride observed in rural continental europe associated with the influence of sea salt chloride and anthropogenic emissions, Geophys. Res. Lett., 39, L10811, doi:10.1029/2012GL051912, 2012.
28. Riedel, T. P., Bertram, T. H., Crisp, T. A., Williams, E. J., Lerner, B. M., Vlasenko, A., Li, S.-M., Gilman, J., de Gouw, J., Bon, D. M., Wagner, N. L., Brown, S. S., and Thornton, J. A.: Nitryl chloride and molecular chlorine in the coastal marine boundary layer, Environ. Sci. Technol., 46, 10463-10470, doi:10.1021/es204632r, 2012.
29. 5 on chemistry and nitrate aerosol formation in the lower troposphere under photosmog conditions, J. Geophys. Res.-Atmos., 108, 4144, doi:10.1029/2002JD002436, 2003.
30. Rinne, J., Markkanen, T., Ruuskanen, T. M., Petäjä, T., Keronen, P., Tang, M. J., Crowley, J. N., Rannik, Ü., and Vesala, T.: Effect of chemical degradation on fluxes of reactive compounds - a study with a stochastic Lagrangian transport model, Atmos. Chem. Phys., 12, 4843-4854, doi:10.5194/acp-12-4843-2012, 2012.
31. Schaap, M., Otjes, R. P., and Weijers, E. P.: Illustrating the benefit of using hourly monitoring data on secondary inorganic aerosol and its precursors for model evaluation, Atmos. Chem. Phys., 11, 11041-11053, doi:10.5194/acp-11- 11041-2011, 2011.
32. 5, Atmos. Meas. Tech., 2, 1-13, doi:10.5194/amt-2-1- 2009, 2009.
33. 5), Rev. Sci. Instrum., 74, 3442-3452, 2003.
34. Sutton, M. A., Howard, C. M., Erisman, J. W., Billen, G., Bleeker, A., Grennfelt, P., van Grinsven, H., and Grizzetti, B.: The European nitrogen assessment. Sources, effects and policy perspectives, Cambridge University Press, 2011.
35. Tang, Y. S., Simmons, I., van Dijk, N., Di Marco, C., Nemitz, E., Daemmgen, U., Gilke, K., Djuricic, V., Vidic, S., Gliha, Z., Borovecki, D., Mitosinkova, M., Hanssen, J. E., Uggerud, T. H., Sanz, M. J., Sanz, P., Chorda, J. V., Flechard, C. R., Fauvel, Y., Ferm, M., Perrino, C., and Sutton, M. A.: European scale application of atmospheric reactive nitrogen measurements in a low-cost approach to infer dry deposition fluxes, Agr. Ecosyst. Environ., 133, 183-195, doi:10.1016/j.agee.2009.04.027, 2009.
36. ten Brink, H., Otjes, R., Jongejan, P., and Kos, G.: Monitoring of the ratio of nitrate to sulphate in size-segregated submicron aerosol in the Netherlands, Atmos. Res., 92, 270-276, doi:10.1016/j.atmosres.2008.12.003, 2009.
37. Thomas, R. M., Trebs, I., Otjes, R., Jongejan, P. A. C., Ten Brink, H., Phillips, G., Kortner, M., Meixner, F. X., and Nemitz, E.: An automated analyzer to measure surface-atmosphere exchange fluxes of water soluble inorganic aerosol compounds and reactive trace gases, Environ. Sci. Technol., 43, 1412-1418, doi:10.1021/es8019403, 2009.
38. Thornton, J. A., Kercher, J. P., Riedel, T. P., Wagner, N. L., Cozic, J., Holloway, J. S., Dube, W. P., Wolfe, G. M., Quinn, P. K., Middlebrook, A. M., Alexander, B., and Brown, S. S.: A large atomic chlorine source inferred from mid-continental reactive nitrogen chemistry, Nature, 464, 271-274, doi:10.1038/nature08905, 2010.
39. Twigg, M. M., House, E., Thomas, R., Whitehead, J., Phillips, G. J., Famulari, D., Fowler, D., Gallagher, M. W., Cape, J. N., Sutton, M. A., and Nemitz, E.: Surface/atmosphere exchange and chemical interactions of reactive nitrogen compounds above a manured grassland, Agr. Forest Meteorol., 151, 1488-1503, doi:10.1016/j.agrformet.2011.06.005, 2011.
40. Wexler, A. S. and Seinfeld, J. H.: Analysis of aerosol ammonium nitrate - departures from equlibrium during SCAQS, Atmos. Environ. A Gen., 26, 579-591, doi:10.1016/0960-1686(92)90171-g, 1992.
41. Yvon, S. A., Saltzman, E. S., Cooper, D. J., Bates, T. S., and Thomson, A. M.: Atmospheric sulfur cycling in the tropical pacific marine boundary layer (12°S, 135°W): A comparison of field data and model results 1. Dimethylsulfide, J. Geophys. Res., 101, 6899-6909, 1996.
42. Zhang, L., Jacob, D. J., Knipping, E. M., Kumar, N., Munger, J. W., Carouge, C. C., van Donkelaar, A., Wang, Y. X., and Chen, D.: Nitrogen deposition to the United States: distribution, sources, and processes, Atmos. Chem. Phys., 12, 4539-4554, doi:10.5194/acp-12-4539-2012, 2012.