From conventional to phase-sensitive vibrational sum frequency generation spectroscopy: Probing water organization at aqueous interfaces

Journal of Physical Chemistry Letters

Volumn 3, Issue 20, 2012, Pages 3012-3028

  Verreault, Dominique ^a   Hua, Wei ^a   Allen, Heather C ^a  

^a OHIO STATE UNIVERSITY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

AQUEOUS INTERFACES; DETECTION MODE; EXPERIMENTAL METHODS; INTERFACIAL SYSTEMS; PHASE-SENSITIVE; STRUCTURAL INFORMATION; VIBRATIONAL SUM-FREQUENCY GENERATIONS;

CHEMISTRY; PHYSICAL CHEMISTRY;

PHASE INTERFACES;

EID: 84867630039     PISSN: None     EISSN: 19487185     Source Type: Journal    
DOI: 10.1021/jz301179g     Document Type: Review

References (215)

1. 2O: A Biography of Water; Weidenfeld & Nicolson: London, 1999.
2. Finney, J. L. Water? What's so Special About it? Philos. Trans. R. Soc. London, Ser. B 2004, 359, 1145-1165 (Pubitemid 39123209)
3. Ball, P. Water as an Active Constituent in Cell Biology Chem. Rev. 2008, 108, 74-108 (Pubitemid 351187472)
4. Brovchenko, I.; Oleinikova, A. Interfacial and Confined Water; Elsevier Science: New York, 2008.
5. Fayer, M. D.; Levinger, N. E. Analysis of Water in Confined Geometries and at Interfaces Annu. Rev. Anal. Chem. 2010, 3, 89-107
6. Fayer, M. D. Dynamics of Water Interacting with Interfaces, Molecules, and Ions Acc. Chem. Res. 2012, 45, 3-14
7. Lang, E. W.; Ludemann, H. D. The Anomalous Properties of Liquid Water Angew. Chem., Int. Ed. 1982, 21, 315-388
8. Brovchenko, I.; Oleinikova, A. Multiple Phases of Liquid Water ChemPhysChem 2008, 9, 2660-2675
9. Cheng, L.; Fenter, P.; Nagy, K. L.; Schlegel, M. L.; Sturchio, N. C. Molecular-Scale Density Oscillations in Water Adjacent to a Mica Surface Phys. Rev. Lett. 2001, 87, 156103/1-156103/4 (Pubitemid 33006404)
10. Teschke, O.; Ceotto, G.; de Souza, G. F. Interfacial Water Dielectric-Permittivity-Profile Measurements using Atomic Force Microscopy Phys. Rev. E 2001, 64, 011605/1-011605/10 (Pubitemid 32693834)
11. Bonthuis, D. J.; Gekle, S.; Netz, R. R. Profile of the Static Permittivity Tensor of Water at Interfaces: Consequences for Capacitance, Hydration Interaction and Ion Adsorption Langmuir 2012, 28, 7679-7694
12. Goertz, M. P.; Houston, J. E.; Zhu, X. Y. Hydrophilicity and the Viscosity of Interfacial Water Langmuir 2007, 23, 5491-5497 (Pubitemid 46826498)
13. Vargaftik, N. B.; Volkov, B. N.; Voljak, L. D. International Tables of the Surface Tension of Water J. Phys. Chem. Ref. Data 1983, 12, 817-820
14. Sokhan, V. P.; Tildesley, D. J. The Free Surface of Water: Molecular Orientation, Surface Potential and Nonlinear Susceptibility Mol. Phys. 1997, 92, 625-640 (Pubitemid 127477497)
15. Paluch, M. Electrical Properties of Free Surface of Water and Aqueous Solutions Adv. Colloid Interface Sci. 2000, 84, 27-45 (Pubitemid 30526522)
16. Parfenyuk, V. I. Surface Potential at the Gas-Aqueous Solution Interface Colloid J. 2002, 64, 588-595 (Pubitemid 35384894)
17. Kathmann, S. M.; Kuo, I.-F. W.; Mundy, C. J.; Schenter, G. K. Understanding the Surface Potential of Water J. Phys. Chem. B 2011, 115, 4369-4377
18. Vácha, R.; Marsalek, O.; Willard, A. P.; Bonthuis, D. J.; Netz, R. R.; Jungwirth, P. Charge Transfer between Water Molecules as the Possible Origin of the Observed Charging at the Surface of Pure Water J. Phys. Chem. Lett. 2012, 3, 107-111
19. Vácha, R.; Buch, V.; Milet, A.; Devlin, J. P.; Jungwirth, P. Autoionization at the Surface of Neat Water: Is the Top Layer pH Neutral, Basic, or Acidic? Phys. Chem. Chem. Phys. 2007, 9, 4736-4747
20. Gray-Weale, A.; Beattie, J. K. An Explanation for the Charge on Water's Surface Phys. Chem. Chem. Phys. 2009, 11, 10994-11005
21. Zimmermann, R.; Freudenberg, U.; Schweia, R.; Küttner, D.; Werner, C. Hydroxide and Hydronium Ion Adsorption - A Survey Curr. Opin. Colloid Interface Sci. 2010, 15, 196-202
22. Petersen, P. B.; Saykally, R. J. Is the Liquid Water Surface Basic or Acidic? Macroscopic vs. Molecular-Scale Investigations Chem. Phys. Lett. 2008, 458, 255-261
23. Jungwirth, P.; Winter, B. Ions at Aqueous Interfaces: From Water Surface to Hydrated Proteins Annu. Rev. Phys. Chem. 2008, 59, 343-366 (Pubitemid 351703390)
24. Jubb, A. M.; Hua, W.; Allen, H. C. Organization of Water and Atmospherically Relevant Ions and Solutes: Vibrational Sum Frequency Spectroscopy at the Vapor/Liquid and Liquid/Solid Interfaces Acc. Chem. Res. 2012, 45, 110-119
25. Jubb, A. M.; Hua, W.; Allen, H. C. Environmental Chemistry at Vapor/Water Interfaces: Insights from Vibrational Sum Frequency Generation Spectroscopy Annu. Rev. Phys. Chem. 2012, 63, 107-130
26. Netz, R. R.; Horinek, D. Progress in Modeling of Ion Effects at the Vapor/Water Interface Annu. Rev. Anal. Chem. 2012, 63, 401-418
27. Onsager, L.; Samaras, N. N. T. The Surface Tension of Debye-Hückel Electrolytes J. Chem. Phys. 1934, 2, 528-536
28. Chang, T. M.; Dang, L. X. Recent Advances in Molecular Simulations of Ion Solvation at Liquid Interfaces Chem. Rev. 2006, 106, 1305-1322 (Pubitemid 43676511)
29. Jungwirth, P.; Tobias, D. J. Specific Ion Effects at the Air/Water Interface Chem. Rev. 2006, 106, 1259-1281 (Pubitemid 43676510)
30. Gopalakrishnan, S.; Liu, D. F.; Allen, H. C.; Kuo, M.; Shultz, M. J. Vibrational Spectroscopic Studies of Aqueous Interfaces: Salts, Acids, Bases, and Nanodrops Chem. Rev. 2006, 106, 1155-1175 (Pubitemid 43676507)
31. Winter, B.; Faubel, M. Photoemission from Liquid Aqueous Solutions Chem. Rev. 2006, 106, 1176-1211 (Pubitemid 43676508)
32. Marcus, Y. Effect of Ions on the Structure of Water: Structure Making and Breaking Chem. Rev. 2009, 109, 1346-1370
33. Collins, K. D.; Neilson, G. W.; Enderby, J. E. Ions in Water: Characterizing the Forces that Control Chemical Processes and Biological Structure Biophys. Chem. 2007, 128, 95-104 (Pubitemid 46843439)
34. Stuart, S. J.; Berne, B. J. Surface Curvature Effects in the Aqueous Ionic Solvation of the Chloride Ion J. Phys. Chem. A 1999, 103, 10300-10307 (Pubitemid 129571314)
35. Noah-Vanhoucke, J.; Geissler, P. L. Liquids and Structural Glasses Special Feature: On the Fluctuations that Drive Small Ions Toward, and Away from, Interfaces between Polar Liquids and Their Vapors Proc. Natl. Acad. Sci. U.S.A. 2009, 106, 15125-15130
36. Otten, D. E.; Shaffer, P. R.; Geissler, P. L.; Saykally, R. J. Elucidating the Mechanism of Selective Ion Adsorption to the Liquid Water Surface Proc. Natl. Acad. Sci. U.S.A. 2012, 109, 701-705
37. Peslherbe, G. H.; Ladanyi, B. M.; Hynes, J. T. Structure of NaI Ion Pairs in Water Clusters Chem. Phys. 2000, 258, 201-224
38. Herce, D. H.; Perera, L.; Darden, T. A.; Sagui, C. Surface Solvation for an Ion in a Water Cluster J. Chem. Phys. 2005, 122, 024513/1-024513/10
39. Archontis, G.; Leontidis, E.; Andreou, G. Attraction of Iodide Ions by the Free Water Surface, Revealed by Simulations with a Polarizable Force Field Based on Drude Oscillators J. Phys. Chem. 2005, 109, 17957-17966 (Pubitemid 41445335)
40. Wick, C. D.; Xantheas, S. S. Computational Investigation of the First Solvation Shell Structure of Interfacial and Bulk Aqueous Chloride and Iodide Ions J. Phys. Chem. B 2009, 113, 4141-4146
41. Jungwirth, P.; Tobias, D. J. Molecular Structure of Salt Solutions: A New View of the Interface with Implications for Heterogeneous Atmospheric Chemistry J. Phys. Chem. B 2001, 105, 10468-10472 (Pubitemid 35338534)
42. Jungwirth, P.; Tobias, D. J. Ions at the Air/Water Interface J. Phys. Chem. B 2002, 106, 6361-6373 (Pubitemid 35281769)
43. Pegram, L. M.; Record, M. T. Partitioning of Atmospherically Relevant Ions Between Bulk Water and the Water/Vapor Interface Proc. Natl. Acad. Sci. U.S.A. 2006, 103, 14278-14281 (Pubitemid 44484740)
44. Arslanargin, A.; Beck, T. L. Free Energy Partitioning Analysis of the Driving Forces that Determine Ion Density Profiles Near the Water Liquid-Vapor Interface J. Chem. Phys. 2012, 136, 104503/1-104503/12
45. Baer, M. D.; Stern, A. C.; Levin, Y.; Tobias, D. J.; Mundy, C. J. Electrochemical Surface Potential Due to Classical Point Charge Models Drives Anion Adsorption to the Air-Water Interface J. Phys. Chem. Lett. 2012, 3, 1565-1570
46. Cheng, J.; Vecitis, C. D.; Hoffmann, M. R.; Colussi, A. J. Experimental Anion Affinities for the Air/Water Interface J. Phys. Chem. B 2006, 110, 25598-25602 (Pubitemid 46133262)
47. Wren, S. N.; Donaldson, D. J. Glancing-Angle Raman Spectroscopic Probe for Reaction Kinetics at Water Surfaces Phys. Chem. Chem. Phys. 2010, 12, 2648-2654
48. Wren, S. N.; Donaldson, D. J. Exclusion of Nitrate to the Air-Ice Interface During Freezing J. Phys. Chem. Lett. 2011, 2, 1967-1971
49. x =2-5Ar Cluster Ions for M = Li, Na, K, and Cs J. Am. Chem. Soc. 2008, 130, 15381-15392
50. Asmis, K. R.; Neumark, D. M. Vibrational Spectroscopy of Microhydrated Conjugate Base Anions Acc. Chem. Res. 2012, 45, 43-52
51. Padmanabhan, V.; Daillant, J.; Belloni, L.; Mora, S.; Alba, M.; Konovalov, O. Specific Ion Adsorption and Short-Range Interactions at the Air Aqueous Solution Interface Phys. Rev. Lett. 2007, 99, 086105/1-086105/4
52. Ghosal, S.; Hemminger, J. C.; Bluhm, H.; Mun, S. M.; Hebenstreit, E. L. D.; Ketteler, G.; Ogletree, D. F.; Requejo, F. G.; Salmeron, M. Electron Spectroscopy of Aqueous Solution Interfaces Reveals Surface Enhancement of Halides Science 2005, 307, 563-566 (Pubitemid 40165676)
53. Eisenthal, K. B. Liquid Interfaces Probed by Second-Harmonic and Sum-Frequency Spectroscopy Chem. Rev. 1996, 96, 1343-1360 (Pubitemid 126639358)
54. Eisenthal, K. B. Second Harmonic Spectroscopy of Aqueous Nano- and Microparticle Interfaces Chem. Rev. 2006, 106, 1462-1477
55. Petersen, P. B.; Saykally, R. J. On the Nature of Ions at the Liquid Water Surface Annu. Rev. Phys. Chem. 2006, 57, 333-364
56. Schrödle, S.; Richmond, G. L. In Situ Non-Linear Spectroscopic Approaches to Understanding Adsorption at Mineral-Water Interfaces J. Phys. D: Appl. Phys. 2008, 41, 033001/1-033001/14
57. Allen, H. C.; Casillas-Ituarte, N. N.; Sierra-Hernandez, M. R.; Chen, X. K.; Tang, C. Y. Shedding Light on Water Structure at Air-Aqueous Interfaces: Ions, Lipids, and Hydration Phys. Chem. Chem. Phys. 2009, 11, 5538-5549
58. Petersen, P. B.; Johnson, J. C.; Knutsen, K. P.; Saykally, R. J. Confirmation of Enhanced Anion Concentration at the Liquid Water Surface Chem. Phys. Lett. 2004, 397, 51-55
59. Onorato, R. M.; Otten, D. E.; Saykally, R. J. Measurement of Bromide Ion Affinities for the Air/Water and Dodecanol/Water Interfaces at Molar Concentrations by UV Second Harmonic Generation Spectroscopy J. Phys. Chem. C 2010, 114, 13746-13751
60. Viswanath, P.; Motschmann, H. Oriented Thiocyanate Anions at the Air-Electrolyte Interface and Its Implications on Interfacial Water - A Vibrational Sum Frequency Spectroscopy Study J. Phys. Chem. C 2007, 111, 4484-4486 (Pubitemid 46573482)
61. Viswanath, P.; Motschmann, H. Effect of Interfacial Presence of Oriented Thiocyanate on Water Structure J. Phys. Chem. C 2008, 112, 2099-2103 (Pubitemid 351322084)
62. Xu, M; Tang, C. Y.; Jubb, A. M.; Chen, X. K.; Allen, H. C. Nitrate Anions and Ion Pairing at the Air-Aqueous Interface J. Phys. Chem. C 2009, 113, 2082-2087
63. Tian, C.; Byrnes, S. J.; Han, H.-L.; Shen, Y. R. Surface Propensities of Atmospherically Relevant Ions in Salt Solutions Revealed by Phase-Sensitive Sum Frequency Vibrational Spectroscopy J. Phys. Chem. Lett. 2011, 2, 1946-1949
64. 2 and NaCl at the Air/Aqueous Interface Revealed by Heterodyne Detected Phase-Sensitive Sum Frequency J. Phys. Chem. Lett. 2011, 2, 2515-2520
65. Heinz, T. F. Second-Order Nonlinear Optical Effects at Surfaces and Interfaces. In Nonlinear Surface Electromagnetic Phenomena; Ponath, H.-E.; Stegemen, G. I., Eds.; North-Holland: Amsterdam, The Netherlands, 1991.
66. Shen, Y. R. Surface Spectroscopy by Nonlinear Optics. In Frontiers in Laser Spectroscopy: Proceedings of the International School of Physics "Enrico Fermi", Course CXX; Hänsch, T. W.; Ignuscio, M., Eds.; North-Holland: Amsterdam, The Netherlands, 1994.
67. Hunt, J. H.; Guyot-Sionnest, P.; Shen, Y. R. Observation of C-H Stretch Vibrations of Monolayers of Molecules Optical Sum-Frequency Generation Chem. Phys. Lett. 1987, 133, 189-192
68. Zhu, X. D.; Suhr, H.; Shen, Y. R. Surface Vibrational Spectroscopy by Infrared-Visible Sum Frequency Generation Phys. Rev. B 1987, 35, 3047-3050
69. Guyot-Sionnest, P.; Hunt, J. H.; Shen, Y. R. Sum-Frequency Vibrational Spectroscopy of a Langmuir Film: Study of Molecular Orientation of a Two-Dimensional System Phys. Rev. Lett. 1987, 59, 1597-1600
70. Zhuang, X.; Miranda, P. B.; Kim, D.; Shen, Y. R. Mapping Molecular Orientation and Conformation at Interfaces by Surface Nonlinear Optics Phys. Rev. B 1999, 59, 12632-12640
71. Bain, C. D.; Davies, P. B.; Ong, T. H.; Ward, R. N.; Brown, M. A. Quantitative Analysis of Monolayer Composition by Sum-Frequency Vibrational Spectroscopy Langmuir 1991, 7, 1563-1566 (Pubitemid 21737622)
72. Feng, R.-r.; Guo, Y.; Lü, R.; Velarde, L.; Wang, H.-f. Consistency in the Sum Frequency Generation Intensity and Phase Vibrational Spectra of the Air/Neat Water Interface J. Phys. Chem. A 2011, 115, 6015-6027
73. Busson, B.; Tadjeddine, A. Non-Uniqueness of Parameters Extracted from Resonant Second-Order Nonlinear Optical Spectroscopies J. Phys. Chem. C 2009, 113, 21895-21902
74. Sovago, M.; Vartiainen, E.; Bonn, M. Determining Absolute Molecular Orientation at Interfaces: A Phase Retrieval Approach for Sum Frequency Generation Spectroscopy J. Phys. Chem. C 2009, 113, 6100-6106
75. Sovago, M.; Vartiainen, E.; Bonn, M. Observation of Buried Water Molecules in Phospholipid Membranes by Surface Sum-Frequency Generation Spectroscopy J. Chem. Phys. 2009, 131, 161107/1-161107/4
76. Sovago, M.; Vartiainen, E.; Bonn, M. Erratum: Observation of Buried Water Molecules in Phospholipid Membranes by Surface Sum-Frequency Generation Spectroscopy J. Chem. Phys. 2010, 133, 229901/1-229901/2
77. de Beer, A. G. F.; Samson, J.-S.; Hua, W.; Huang, Z.; Chen, X.; Allen, H. C.; Roke, S. Direct Comparison of Phase-Sensitive Vibrational Sum Frequency Generation with Maximum Entropy Method: Case Study of Water J. Chem. Phys. 2011, 135, 224701/1-224701/9
78. Superfine, R.; Huang, J. Y.; Shen, Y. R. Phase Measurement for Surface Infrared-Visible Sum-Frequency Generation Opt. Lett. 1990, 15, 1276-1278
79. Superfine, R.; Huang, J. Y.; Shen, Y. R. Experimental Determination of the Sign of Molecular Dipole Moment Derivatives: An Infrared-Visible Sum Frequency Generation Absolute Phase Measurement Study Chem. Phys. Lett. 1990, 172, 303-306
80. Ostroverkhov, V.; Waychunas, G. A.; Shen, Y. R. New Information on Water Interfacial Structure Revealed by Phase-Sensitive Surface Spectroscopy Phys. Rev. Lett. 2005, 94, 046102/1-046102/4
81. Ji, N.; Ostroverkhov, V.; Chen, C.-Y.; Shen, Y.-R. Phase-Sensitive Sum-Frequency Vibrational Spectroscopy and Its Application to Studies of Interfacial Alkyl Chains J. Am. Chem. Soc. 2007, 129, 10056-10057 (Pubitemid 47312924)
82. Stiopkin, I. V.; Jayathilake, H. D.; Bordenyuk, A. N.; Benderskii, A. V. Heterodyne-Detected Vibrational Sum Frequency Generation Spectroscopy J. Am. Chem. Soc. 2008, 130, 2271-2275 (Pubitemid 351288004)
83. Yamaguchi, S.; Tahara, T. Heterodyne-Detected Electronic Sum Frequency Generation: "Up" versus "Down" Alignment of Interfacial Molecules J. Chem. Phys. 2008, 129, 101102/1-101102/4
84. Nihonyanagi, S.; Yamaguchi, S.; Tahara, T. Direct Evidence for Orientational Flip-Flop of Water Molecules at Charged Interfaces: A Heterodyne-Detected Vibrational Sum Frequency Generation Study J. Chem. Phys. 2009, 130, 204704/1-204704/5
85. Pool, R. E.; Versluis, J.; Backus, E. H. G.; Bonn, M. Comparative Study of Direct and Phase-Specific Vibrational Sum-Frequency Generation Spectroscopy: Advantages and Limitations J. Phys. Chem. B 2011, 115, 15362-15369
86. Bloembergen, N.; Pershan, P. S. Light Waves at the Boundary of Nonlinear Media Phys. Rev. 1962, 128, 606-622
87. Lü, R.; Rao, Y.; Zhang, W.-k.; Wang, H.-f. Phase Measurement in Nonlinear Optics of Molecules at Air/Water Interface with Femtosecond Laser Pulses Proc. SPIE Nonlinear Spectrosc. 2002, 4812-15, 115-124
88. Jungwirth, P.; Finlayson-Pitts, B. J.; Tobias, D. J. Introduction: Structure and Chemistry at Aqueous Interfaces Chem. Rev. 2006, 106, 1137-1139 (Pubitemid 43676506)
89. Shultz, M. J.; Baldelli, S.; Schnitzer, C.; Simonelli, D. Aqueous Solution/Air Interfaces Probed with Sum Frequency Generation Spectroscopy J. Phys. Chem. B 2002, 106, 5313-5324 (Pubitemid 35281892)
90. Shen, Y. R.; Ostroverkhov, V. Sum-Frequency Vibrational Spectroscopy on Water Interfaces: Polar Orientation of Water Molecules at Interfaces Chem. Rev. 2006, 106, 1140-1154
91. Morita, A.; Ishiyama, T. Recent Progress in Theoretical Analysis of Vibrational Sum Frequency Generation Spectroscopy Phys. Chem. Chem. Phys. 2008, 10, 5801-5816
92. Skinner, J. L.; Pieniazek, P. A.; Gruenbaum, S. M. Vibrational Spectroscopy of Water at Interfaces Acc. Chem. Res. 2012, 45, 93-100
93. Du, Q.; Superfine, R.; Freysz, E.; Shen, Y. R. Vibrational Spectroscopy of Water at the Vapor/Water Interface Phys. Rev. Lett. 1993, 70, 2313-2316
94. Ji, N.; Ostroverkhov, V.; Tian, C. S.; Shen, Y. R. Characterization of Vibrational Resonances of Water-Vapor Interfaces by Phase-Sensitive Sum-Frequency Spectroscopy Phys. Rev. Lett. 2008, 100, 096102/1-096102/4
95. Sovago, M.; Kramer Campen, R.; Wurpel, G. W. H.; Müller, M.; Bakker, H. J.; Bonn, M. Vibrational Response of Hydrogen-Bonded Interfacial Water is Dominated by Intramolecular Coupling Phys. Rev. Lett. 2008, 100, 173901/1-173901/4
96. Sovago, M.; Kramer Campen, R.; Wurpel, G. W. H.; Müller, M.; Bakker, H. J.; Bonn, M. Sovago et al. Reply Phys. Rev. Lett. 2008, 101, 139402/1
97. Tian, C. S.; Shen, Y. R. Sum-Frequency Vibrational Spectroscopic Studies of Water/Vapor Interfaces Chem. Phys. Lett. 2009, 470, 1-6
98. Pieniazek, P. A.; Tainter, C. J.; Skinner, J. L. Interpretation of the Water Surface Vibrational Sum-Frequency Spectrum J. Chem. Phys. 2011, 135, 044701/1-044701/12
99. (2) Spectra of an Isotopically Diluted Water Surface J. Am. Chem. Soc. 2011, 133, 16875-16880
100. Tian, C.; Ji, N.; Waychunas, G. A.; Shen, Y. R. Interfacial Structures of Acidic and Basic Aqueous Solutions J. Am. Chem. Soc. 2008, 130, 13033-13039
101. Tian, C.-S.; Shen, Y. R. Isotopic Dilution Study of the Water/Vapor Interface by Phase-Sensitive Sum-Frequency Vibrational Spectroscopy J. Am. Chem. Soc. 2009, 131, 2790-2791
102. Morita, A.; Hynes, J. T. A Theoretical Analysis of the Sum Frequency Generation Spectrum of the Water Surface Chem. Phys. 2000, 258, 371-390
103. Morita, A.; Hynes, J. T. A Theoretical Analysis of the Sum Frequency Generation Spectrum of the Water Surface. II. Time-Dependent Approach J. Phys. Chem. B 2002, 106, 673-685 (Pubitemid 35276186)
104. Perry, A.; Ahlborn, H.; Space, B.; Moore, P. B. A Combined Time Correlation Function and Instantaneous Normal Mode Study of the Sum Frequency Generation Spectroscopy of the Water/Vapor Interface J. Chem. Phys. 2003, 118, 8411/1-144705/9
105. Buch, V. Molecular Structure and OH-Stretch Spectra of Liquid Water Surface J. Phys. Chem. B 2005, 109, 17771-17774 (Pubitemid 41445308)
106. Perry, A.; Neipert, C.; Ridley Kasprzyk, C.; Green, T.; Space, B.; Moore, P. B. A Theoretical Description of the Polarization Dependence of the Sum Frequency Generation Spectroscopy of the Water/Vapor Interface J. Chem. Phys. 2005, 123, 144705/1-144705/11
107. Morita, A. Improved Computation of Sum Frequency Generation Spectrum of the Surface of Water J. Phys. Chem. B 2006, 110, 3158-3163
108. Perry, A.; Neipert, C.; Space, B.; Moore, P. B. Theoretical Modeling of Interface Specific Vibrational Spectroscopy: Methods and Applications to Aqueous Interfaces Chem. Rev. 2006, 106, 1234-1258
109. Buch, V.; Tarbuck, T.; Richmond, G. L.; Groenzin, H.; Li, I.; Shultz, M. J. Sum Frequency Generation Surface Spectra of Ice, Water, and Acid Solution Investigated by an Exciton Model J. Chem. Phys. 2007, 127, 204710/1-204710/15
110. 2O J. Chem. Phys. 2008, 129, 214705/1-214705/14
111. Auer, B. M.; Skinner, J. L. Vibrational Sum-Frequency Spectroscopy of the Water Liquid/Vapor Interface J. Phys. Chem. B 2009, 113, 4125-4130
112. Fan, Y.; Chen, X.; Yang, L.; Cremer, P. S.; Gao, Y. Q. On the Structure of Water at the Aqueous/Air Interface J. Phys. Chem. B 2009, 113, 11672-11679
113. Ishiyama, T.; Morita, A. Vibrational Spectroscopic Response of Intermolecular Orientational Correlation at the Water Surface J. Phys. Chem. C 2009, 113, 16299-16302
114. Pieniazek, P. A.; Tainter, C. J.; Skinner, J. L. Surface of Liquid Water: Three-Body Interactions and Vibrational Sum-Frequency Spectroscopy J. Am. Chem. Soc. 2011, 133, 10360-10363
115. Finlayson-Pitts, B. J.; Pitts, J. N., Jr. Chemistry of the Upper and Lower Atmosphere: Theory, Experiments, and Applications; Academic Press: San Diego, CA, 2000.
116. Finlayson-Pitts, B. Reactions at Surfaces in the Atmosphere: Integration of Experiments and Theory as Necessary (but not Necessarily Sufficient) for Predicting the Physical Chemistry of Aerosols Phys. Chem. Chem. Phys. 2009, 11, 7760-7779
117. 2 and BrCl in Surface Ozone Destruction at Polar Sunrise Science 2001, 291, 471-474 (Pubitemid 32097068)
118. Spicer, C. W.; Plastridge, R. A.; Foster, K. L.; Finlayson-Pitts, B. J.; Bottenheim, J. W.; Grannas, A. M.; Shepson, P. B. Molecular Halogens Before and During Ozone Depletion Events in the Arctic at Polar Sunrise: Concentrations and Sources Atmos. Environ. 2002, 36, 2721-2731 (Pubitemid 34628362)
119. Finlayson-Pitts, B. J. Halogens in the Troposphere Anal. Chem. 2010, 82, 770-776
120. Hunt, S. W.; Roeselova, M.; Wang, W.; Wingen, L. M.; Knipping, E. M.; Tobias, D. J.; Dabdub, D.; Finlayson-Pitts, B. J. Formation of Molecular Bromine from the Reaction of Ozone with Deliquesced NaBr Aerosol: Evidence for Interface Chemistry J. Phys. Chem. A 2004, 108, 11559-11572
121. Clifford, D.; Donaldson, D. J. Direct Experimental Evidence for a Heterogeneous Reaction of Ozone with Bromide at the Air-Aqueous Interface J. Phys. Chem. A 2007, 111, 9809-9814 (Pubitemid 47598287)
122. Shultz, M. J.; Schnitzer, C.; Simonelli, D.; Baldelli, S. Sum Frequency Generation Spectroscopy of the Aqueous Interface: Ionic and Soluble Molecular Solutions Int. Rev. Phys. Chem. 2000, 19, 123-153
123. Baldelli, S.; Schnitzer, C.; Shultz, M. J. The Structure of Water on HCl Solutions Studied with Sum Frequency Generation Chem. Phys. Lett. 1999, 302, 157-163 (Pubitemid 129549432)
124. 4 Aqueous Solutions J. Phys. Chem. B 2000, 104, 585-590
125. Liu, D.; Ma, G.; Levering, L. M.; Allen, H. C. Vibrational Spectroscopy of Aqueous Sodium Halide Solutions and Air-Liquid Interfaces: Observation of Increased Interfacial Depth J. Phys. Chem. B 2004, 108, 2252-2260
126. Raymond, E. A.; Richmond, G. L. Probing the Molecular Structure and Bonding of the Surface of Aqueous Salt Solutions J. Phys. Chem. B 2004, 108, 5051-5059
127. Tarbuck, T. L.; Ota, S. T.; Richmond, G. L. Spectroscopic Studies of Solvated Hydrogen and Hydroxide Ions at Aqueous Surfaces J. Am. Chem. Soc. 2006, 128, 14519-14527 (Pubitemid 44749851)
128. Levering, L. M.; Sierra-Hernández, M. R.; Allen, H. C. Observation of Hydronium Ions at the Air-Aqueous Acid Interface: Vibrational Spectroscopic Studies of Aqueous HCl, HBr, and HI J. Phys. Chem. C 2007, 111, 8814-8826 (Pubitemid 47152590)
129. Mucha, M.; Frigato, T.; Levering, L. M.; Allen, H. C.; Tobias, D. J.; Dang, L. X.; Jungwirth, P. Unified Molecular Picture of the Surfaces of Aqueous Acid, Base, and Salt Solutions J. Phys. Chem. B 2005, 109, 7617-7623 (Pubitemid 40643977)
130. Ishiyama, T.; Morita, A. Molecular Dynamics Analysis of Interfacial Structures and Sum Frequency Generation Spectra of Aqueous Hydrogen Halide Solutions J. Phys. Chem. A 2007, 111, 9277-9285 (Pubitemid 47548316)
131. Bian, H.-t.; Feng, R.-r.; Xu, Y.-y.; Guo, Y.; Wang, H.-f. Increased Interfacial Thickness of the NaF, NaCl and NaBr Salt Aqueous Solutions Probed with Non-Resonant Surface Second Harmonic Generation (SHG) Phys. Chem. Chem. Phys. 2008, 10, 4920-4931
132. Ghosal, S.; Brown, M. A.; Bluhm, H.; Krisch, M. J.; Salmeron, M.; Jungwirth, P.; Hemminger, J. C. Ion Partitioning at the Liquid/Vapor Interface of a Multicomponent Alkali Halide Solution: A Model for Aqueous Sea Salt Aerosols J. Phys. Chem. A 2008, 112, 12378-12384
133. Brown, M. A.; D'Auria, R.; Kuo, I.-F. W.; Krisch, M. J.; Starr, D. E.; Bluhm, H.; Tobias, D. J.; Hemminger, J. C. Ion Spatial Distributions at the Liquid-Vapor Interface of Aqueous Potassium Fluoride solutions Phys. Chem. Chem. Phys. 2008, 10, 4778-4784
134. Cheng, M. H.; Callahan, K. M.; Margarella, A. M.; Tobias, D. J.; Hemminger, J. C.; Bluhm, H.; Krisch, M. J. Ambient Pressure X-ray Photoelectron Spectroscopy and Molecular Dynamics Simulation Studies of Liquid/Vapor Interfaces of Aqueous NaCl, RbCl, and RbBr Solutions J. Phys. Chem. C 2012, 116, 4545-4555
135. Brown, E. C.; Mucha, M.; Jungwirth, P.; Tobias, D. J. Structure and Vibrational Spectroscopy of Salt Water/Air Interfaces: Predictions from Classical Molecular Dynamics Simulations J. Phys. Chem. B 2005, 109, 7934-7940 (Pubitemid 40644018)
136. Salvador, P.; Curtis, J. E.; Tobias, D. J.; Jungwirth, P. Polarizability of the Nitrate Anion and Its Solvation at the Air/Water Interface Phys. Chem. Chem. Phys. 2003, 5, 3752-3757
137. Gopalakrishnan, S.; Jungwirth, P.; Tobias, D. J.; Allen, H. C. Air-Liquid Interfaces of Aqueous Solutions Containing Ammonium and Sulfate: Spectroscopic and Molecular Dynamics Studies J. Phys. Chem. B 2005, 109, 8861-8872 (Pubitemid 40750922)
138. 2O Interactions in Aqueous Solutions and at Interfaces J. Chem. Phys. 2006, 124, 066101/1-066101/3
139. Thomas, J. L.; Roeselova, M.; Dang, L. X.; Tobias, D. J. Molecular Dynamics Simulations of the Solution-Air Interface of Aqueous Sodium Nitrate J. Phys. Chem. A 2007, 111, 3091-3098 (Pubitemid 46732992)
140. Molina, J. J.; Lectez, S.; Tazi, S.; Salanne, M.; Dufreache, J.-F.; Roques, J.; Simoni, E.; Madden, P. A.; Turq, P. Ions in Solutions: Determining Their Polarizabilities from First-Principles J. Chem. Phys. 2011, 134, 014511/1-014511/6
141. Brown, M. A.; Winter, B.; Faubel, M.; Hemminger, J. C. Spatial Distribution of Nitrate and Nitrite Anions at the Liquid/Vapor Interface of Aqueous Solutions J. Am. Chem. Soc. 2009, 131, 8354-8355
142. Otten, D. E.; Petersen, P. B.; Saykally, R. J. Observation of Nitrate Ions at the Air/Water Interface by UV-Second Harmonic Generation Chem. Phys. Lett. 2007, 449, 261-265 (Pubitemid 350160603)
143. Jungwirth, P.; Curtis, J. E.; Tobias, D. J. Polarizability and Aqueous Solvation of the Sulfate Dianion Chem. Phys. Lett. 2003, 367, 704-710
144. 2 at a Water Surface J. Am. Chem. Soc. 2006, 128, 3256-3267
145. Du, H.; Liu, J.; Ozdemir, O.; Nguyen, A. V.; Miller, J. D. Molecular Features of the Air/Carbonate Solution Interface J. Colloid Interface Sci. 2008, 318, 271-277
146. Hua, W.; Chen, X.; Allen, H. C. Phase-Sensitive Sum Frequency Revealing Accommodation of Bicarbonate Ions, and Charge Separation of Sodium and Carbonate Ions within the Air/Water Interface J. Phys. Chem. A 2011, 115, 6233-6238
147. Charlson, R. J.; Lovelock, J. E.; Andrea, M. O.; Warren, S. G. Oceanic Phytoplankton, Atmospheric Sulfur, Cloud Albedo and Climate Nature 1987, 326, 655-661
148. Schwartz, S. E. Are Global Cloud Albedo and Climate Controlled by Marine-Phytoplankton? Nature 1988, 336, 441-445 (Pubitemid 19303879)
149. Berresheim, H.; Eisele, F. L.; Tanner, D. J.; McInnes, L. M.; Ramseybell, D. C.; Covert, D. S. 1993, Atmospheric Sulfur Chemistry and Cloud Condensation Nuclei (CCN) Concentrations over the Northeastern Pacific Coast J. Geophys. Res., Atmos. 1993, 98, 12701-12711
150. Charlson, R. J.; Schwartz, S. E.; Hales, J. M.; Cess, R. D.; Coakley, J. A., Jr; Hansen, J. E.; Hofmann, D. J. Climate Forcing by Anthropogenic Aerosols Science 1992, 255, 423-430
151. Kiehl, J. T.; Briegleb, B. P. The Relative Roles of Sulfate Aerosols and Greenhouse Gases in Climate Forcing Science 1993, 260, 311-314
152. Tarbuck, T. L.; Richmond, G. L. Adsorption of Organosulfur Species at Aqueous Surfaces: Molecular Bonding and Orientation J. Phys. Chem. B 2005, 109, 20868-20877 (Pubitemid 41698347)
153. Allen, H. C.; Raymond, E. A.; Richmond, G. L. Surface Structural Studies of Methanesulfonic Acid at Air/Aqueous Solution Interfaces Using Vibrational Sum Frequency Spectroscopy J. Phys. Chem. A 2001, 105, 1649-1655
154. Benjamin, I. Structure, Thermodynamics, and Dynamics of the Liquid/Vapor Interface of Water/Dimethylsulfoxide Mixtures J. Chem. Phys. 1999, 110, 8070-8079
155. Chen, X.; Minofar, B.; Jungwirth, P.; Allen, H. C. Interfacial Molecular Organization at Aqueous Solution Surfaces of Atmospherically Relevant Dimethyl Sulfoxide and Methanesulfonic Acid Using Sum Frequency Spectroscopy and Molecular Dynamics Simulation J. Phys. Chem. B 2010, 114, 15546-15553
156. Darvas, M.; Pojják, K.; Horvai, G.; Jedlovszky, P. Molecular Dynamics Simulation and Identification of the Truly Interfacial Molecules (ITIM) Analysis of the Liquid-Vapor Interface of Dimethyl Sulfoxide J. Chem. Phys. 2010, 132, 134701/1-134701/11
157. Chen, X.; Allen, H. C. Water Structure at Aqueous Solution Surfaces of Atmospherically Relevant Dimethyl Sulfoxide and Methanesulfonic Acid Revealed by Phase-Sensitive Sum Frequency Spectroscopy J. Phys. Chem. B 2010, 114, 14983-14988
158. Lopez, C. F.; Nielsen, S. O.; Klein, M. L.; Moore, P. B. Hydrogen Bonding Structure and Dynamics of Water at the Dimyristoylphosphatidylcholine Lipid Bilayer Surface from a Molecular Dynamics Simulation J. Phys. Chem. B 2004, 108, 6603-6610
159. Watry, M. R.; Tarbuck, T. L.; Richmond, G. L. Vibrational Sum-Frequency Studies of a Series of Phospholipid Monolayers and the Associated Water Structure at the Vapor/Water Interface J. Phys. Chem. B 2003, 107, 512-518
160. Viswanath, P.; Aroti, A.; Motschmann, H.; Leontidis, E. Vibrational Sum Frequency Generation Spectroscopic Investigation of the Interaction of Thiocyanate Ions with Zwitterionic Phospholipid Monolayers at the Air-Water Interface J. Phys. Chem. B 2009, 113, 14816-14823
161. Sung, W.; Seok, S.; Kim, D.; Tian, C. S.; Shen, Y. R. Sum-Frequency Spectroscopic Study of Langmuir Monolayers of Lipids Having Oppositely Charged Headgroups Langmuir 2010, 26, 18266-18272
162. Chen, X.; Hua, W.; Huang, Z.; Allen, H. C. Interfacial Water Structure Associated with Phospholipid Membranes Studied by Phase-Sensitive Vibrational Sum Frequency Generation Spectroscopy J. Am. Chem. Soc. 2010, 132, 11336-11342
163. Nagata, Y.; Mukamel, S. Vibrational Sum-Frequency Generation Spectroscopy at the Water/Lipid Interface: Molecular Dynamics Simulation Study J. Am. Chem. Soc. 2010, 132, 6434-6442
164. Mondal, J. A.; Nihonyanagi, S.; Yamaguchi, S.; Tahara, T. Three Distinct Water Structures at a Zwitterionic Lipid/Water Interface Revealed by Heterodyne-Detected Vibrational Sum Frequency Generation J. Am. Chem. Soc. 2012, 134, 7842-7850
165. Chen, X.; Yang, T. L.; Kataoka, S.; Cremer, P. S. Specific Ion Effects on Interfacial Water Structure near Macromolecules J. Am. Chem. Soc. 2007, 129, 12272-12279 (Pubitemid 47556862)
166. Vlachy, N.; Jagoda-Cwiklik, B.; Vácha, R.; Touraud, D.; Jungwirth, P.; Kunz, W. Hofmeister Series and Specific Interactions of Charged Headgroups with Aqueous Ions Adv. Colloid Polym. Sci. 2009, 146, 42-47
167. Lyklema, J. Simple Hofmeister Series Chem. Phys. Lett. 2009, 467, 217-222
168. Kunz, W. Specific Ion Effects in Colloidal and Biological Systems Curr. Opin. Colloid Interface Sci. 2010, 15, 34-39
169. Zhang, Y.; Cremer, P. S. Chemistry of Hofmeister Anions and Osmolytes Annu. Rev. Phys. Chem. 2010, 61, 63-83
170. Johnson, C. M.; Tyrode, E.; Baldelli, S.; Rutland, M. W.; Leygraf, C. A Vibrational Sum Frequency Spectroscopy Study of the Liquid-Gas Interface of Acetic Acid-Water Mixtures: 1. Surface Speciation J. Phys. Chem. B 2005, 109, 321-328 (Pubitemid 40120976)
171. Minofar, B.; Jungwirth, P.; Das, M. R.; Manash, R.; Kunz, W.; Mahiuddin, S. Propensity of Formate, Acetate, Benzoate, and Phenolate for the Aqueous
172. Mahiuddin, S.; Minofar, B.; Borah, J. M.; Jayanta, M.; Das, M. R.; Manash, R.; Jungwirth, P. Propensities of Oxalic, Citric, Succinic, and Maleic Acids for the Aqueous Solution/Vapour Interface: Surface Tension Measurements and Molecular Dynamics Simulations Chem. Phys. Lett. 2008, 462, 217-221
173. Johnson, C. M.; Tyrode, E.; Kumpulainen, A.; Leygraf, C. Vibrational Sum Frequency Spectroscopy Study of the Liquid/Vapor Interface of Formic Acid/Water Solutions J. Phys. Chem. C 2009, 113, 13209-13218
174. Rao, Y.; Subir, M.; McArthur, E. A.; Turro, N. J.; Eisenthal, K. B. Organic Ions at the Air/Water Interface Chem. Phys. Lett. 2009, 477, 241-244
175. 2+ Effect on the Hydration and Orientation of the Phosphate Group of DPPC at Air-Water and Air-Hydrated Silica Interfaces J. Phys. Chem. B 2010, 114, 9485-9495
176. 2+ Binding to the COOH Headgroup of a Palmitic Acid Monolayer Studied by Sum Frequency Spectroscopy J. Phys. Chem. B 2011, 115, 34-40
177. Uosaki, K.; Noguchi, H.; Yamamoto, R.; Nihonyanagi, S. Interfacial Molecular Structures of Polyelectrolyte Brush in Contact with Dry Nitrogen, Water Vapor, Liquid Water, and Aqueous Electrolyte Solution Studied by Sum Frequency Generation Spectroscopy J. Am. Chem. Soc. 2010, 132, 17271-17276
178. Kondo, T.; Gemmei-Ide, M.; Kitano, H.; Ohno, K.; Noguchi, H.; Uosaki, K. Sum Frequency Generation Study on the Structure of Water in the Vicinity of an Amphoteric Polymer Brush Colloid Surf., B 2012, 91, 215-218
179. Kondo, T.; Nomura, K.; Murou, M.; Gemmei-Ide, M.; Kitano, H.; Noguchi, H.; Uosaki, K.; Ohno, K.; Saruwatari, Y. Structure of Water in the Vicinity of a Zwitterionic Polymer Brush as Examined by Sum Frequency Generation Method Colloid Surf., B 2012, 100, 126-132
180. Chen, X.; Flores, S. C.; Lim, S.-M.; Zhang, Y.; Yang, T.; Kherb, J.; Cremer, P. S. Specific Anion Effects on Water Structure Adjacent to Protein Monolayers Langmuir 2010, 26, 16447-16454
181. Tian, C. S.; Shen, Y. R. Structure and Charging of Hydrophobic Material/Water Interfaces Studied by Phase-Sensitive Sum-Frequency Vibrational Spectroscopy Proc. Natl. Acad. Sci. U.S.A. 2009, 106, 15148-15153
182. Hopkins, A. J.; McFearin, C. L.; Richmond, G. L. SAMs under Water: The Impact of Ions on the Behavior of Water at Soft Hydrophobic Surfaces J. Phys. Chem. C 2011, 115, 11192-11203
183. Brown, G. E., Jr.; Henrich, V. E.; Casey, W. H.; Clark, D. L.; Eggleston, C.; Felmy, A.; Goodman, D. W.; Grätzel, M.; Maciel, G.; McCarthy, M. I.; Nealson, K. H.; Sverjensky, D. A.; Toney, M. F.; Zachara, J. M. Metal Oxide Surfaces and Their Interactions with Aqueous Solutions and Microbial Organisms Chem. Rev. 1999, 99, 77-174 (Pubitemid 129657132)
184. Al-Abadleh, H. A.; Grassian, V. H. Oxide Surfaces as Environmental Interfaces Surf. Sci. Rep. 2003, 52, 63-161
185. Grassian, V. H. Surface Science of Complex Environmental Interfaces: Oxide and Carbonate Surfaces in Dynamic Equilibrium with Water Vapor Surf. Sci. 2008, 602, 2955-2962
186. 2O Interface Langmuir 2001, 17, 7721-7724 (Pubitemid 35330937)
187. 2/Water Interface Langmuir 2010, 26, 10784-10790
188. Jubb, A. M.; Allen, H. C. Sulfate Adsorption at the Buried Fluorite-Solution Interface Revealed by Vibrational Sum Frequency Generation Spectroscopy J. Phys. Chem. C 2012, 116, 9085-9091
189. Flörsheimer, M.; Kruse, K.; Polly, R.; Abdelmonem, A.; Schimmelpfennig, B.; Klenze, R.; Fanghänel, T. Hydration of Mineral Surfaces Probed at the Molecular Level Langmuir 2008, 24, 13434-13439
190. 3 (0001) J. Phys. Chem. C 2008, 112, 1751-1754 (Pubitemid 351322037)
191. 3 (11̄02) Interface Structure Studied by Sum-Frequency Vibrational Spectroscopy J. Phys. Chem. C 2011, 115, 13887-13893
192. Ostroverkhov, V.; Waychunas, G. A.; Shen, Y. R. Vibrational Spectra of Water at Water/α-Quartz (0001) Interface Chem. Phys. Lett. 2004, 386, 144-148
193. Yang, Z.; Li, Q. F.; Chou, K. C. Structures of Water Molecules at the Interfaces of Aqueous Salt Solutions and Silica: Cation Effects J. Phys. Chem. C 2009, 113, 8201-8205
194. Jena, K. C.; Hore, D. K. Variation of Ionic Strength Reveals the Interfacial Water Structure at a Charged Mineral Surface J. Phys. Chem. C 2009, 113, 15364-15372
195. Jena, K. C.; Covert, P. A.; Hore, D. K. The Effect of Salt on the Water Structure at a Charged Solid Surface: Differentiating Second- and Third-Order Nonlinear Contributions J. Phys. Chem. Lett. 2011, 2, 1056-1061
196. Azam, M. S.; Weeraman, C. N.; Gibbs-Davis, J. M. Specific Cation Effects on the Bimodal Acid-Base Behavior of the Silica/Water Interface J. Phys. Chem. Lett. 2012, 3, 1269-1274
197. Flores, S. C.; Kherb, J.; Konelick, N.; Chen, X.; Cremer, P. S. The Effects of Hofmeister Cations at Negatively Charged Hydrophilic Surfaces J. Phys. Chem. C 2012, 116, 5730-5734
198. Flores, S. C.; Kherb, J.; Cremer, P. S. Direct and Reverse Hofmeister Effects on Interfacial Water Structure J. Phys. Chem. C 2012, 116, 14408-14413
199. 2/Aqueous Interface Langmuir 2004, 20, 1662-1666
200. Zhang, L.; Tian, C.; Waychunas, G. A.; Shen, Y. R. Structures and Charging of α-Alumina (0001)/Water Interfaces Studied by Sum-Frequency Vibrational Spectroscopy J. Am. Chem. Soc. 2008, 130, 7686-7694 (Pubitemid 351842133)
201. Arnolds, H.; Bonn, M. Ultrafast Surface Vibrational Dynamics Surf. Sci. Rep. 2010, 65, 45-66
202. Ghosh, A.; Smits, M.; Bredenbeck, J.; Dijkhuizen, N.; Bonn, M. Femtosecond Time-Resolved and Two-Dimensional Vibrational Sum Frequency Spectroscopic Instrumentation to Study Structural Dynamics at Interfaces Rev. Sci. Instrum. 2008, 79, 093907/1-093907/9
203. McGuire, J. A.; Shen, Y. R. Ultrafast Vibrational Dynamics at Water Interfaces Science 2006, 313, 1945-1948 (Pubitemid 44497998)
204. Smits, M.; Ghosh, A.; Sterrer, M.; Müller, M.; Bonn, M. Ultrafast Vibrational Energy Transfer between Surface and Bulk Water at the Air-Water Interface Phys. Rev. Lett. 2007, 98, 098302/1-098302/4
205. Hsieh, C.-S.; Campen, R. K.; Vila Verde, A. C.; Bolhuis, P.; Nienhuys, H.-K.; Bonn, M. Ultrafast Reorientation of Dangling OH Groups at the Air-Water Interface Using Femtosecond Vibrational Spectroscopy Phys. Rev. Lett. 2011, 107, 116102/1-116102/5
206. Ghosh, A.; Smits, M.; Bredenbeck, J.; Bonn, M. Membrane-Bound Water is Energetically Decoupled from Nearby Bulk Water: An Ultrafast Surface-Specific Investigation J. Am. Chem. Soc. 2007, 129, 9608-9609 (Pubitemid 47237470)
207. Bonn, M.; Bakker, H. J.; Ghosh, A.; Yamamoto, S.; Sovago, M.; Campen, R. K. Structural Inhomogeneity of Interfacial Water at Lipid Monolayers Revealed by Surface-Specific Vibrational Pump-Probe Spectroscopy J. Am. Chem. Soc. 2010, 132, 14971-14978
208. Eftekhari-Bafrooei, A.; Borguet, E. Effect of Surface Charge on the Vibrational Dynamics of Interfacial Water J. Am. Chem. Soc. 2009, 131, 12034-12035
209. Eftekhari-Bafrooei, A.; Borguet, E. Effect of Hydrogen-Bond Strength on the Vibrational Relaxation of Interfacial Water J. Am. Chem. Soc. 2010, 132, 3756-3761
210. Eftekhari-Bafrooei, A.; Borguet, E. Effect of Electric Fields on the Ultrafast Vibrational Relaxation of Water at a Charged Solid-Liquid Interface as Probed by Vibrational Sum Frequency Generation J. Phys. Chem. Lett. 2011, 2, 1353-1358
211. Bredenbeck, J.; Ghosh, A.; Nienhuys, H.-K.; Bonn, M. Interface-Specific Ultrafast Two-Dimensional Vibrational Spectroscopy Acc. Chem. Res. 2009, 42, 1332-1342
212. Xiong, W.; Laaser, J. E.; Mehlenbacher, R. D.; Zanni, M. T. Adding a Dimension to the Infrared Spectra of Interfaces Using Heterodyne Detected 2D Sum-Frequency Generation (HD 2D SFG) Spectroscopy Proc. Natl. Acad. Sci. U.S.A. 2011, 108, 20902-20907
213. Zhang, Z.; Piatkowski, L.; Bakker, H. J.; Bonn, M. Interfacial Water Structure Revealed by Ultrafast Two-Dimensional Surface Vibrational Spectroscopy J. Chem. Phys. 2011, 135, 021101/1-021101/3
214. Zhang, Z.; Piatkowski, L.; Bakker, H. J.; Bonn, M. Ultrafast Vibrational Energy Transfer at the Water/Air Interface Revealed by Two-Dimensional Surface Vibrational Spectroscopy Nat. Chem. 2011, 3, 888-893
215. Isaienko, O.; Borguet, E. Ultra-Broadband Sum-Frequency Vibrational Spectrometer of Aqueous Interfaces Based on a Non-Collinear Optical Parametric Amplifier Opt. Express 2012, 20, 547-561