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Volumn 129, Issue 10, 2008, Pages

Heterodyne-detected electronic sum frequency generation: "Up" versus "down" alignment of interfacial molecules

Author keywords

[No Author keywords available]

Indexed keywords

HETERODYNING; NITROGEN COMPOUNDS; OPTICAL MATERIALS; SILICA;

EID: 51749085776     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.2981179     Document Type: Article
Times cited : (163)

References (26)
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    • Yamaguchi, S.1    Tahara, T.2
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    • 0036980809 scopus 로고    scopus 로고
    • SPIE Conference on Nonlinear Spectroscopy, Seattle, WA, (unpublished), Vol., and references therein.
    • R. Lü, Y. Rao, W. Zhang, and H. Wang, SPIE Conference on Nonlinear Spectroscopy, Seattle, WA, 2002 (unpublished), Vol. 4812, p. 115, and references therein.
    • (2002) , vol.4812 , pp. 115
    • Lü, R.1    Rao, Y.2    Zhang, W.3    Wang, H.4
  • 16
    • 51749124193 scopus 로고    scopus 로고
    • If the surface (2) of GaAs in the present in-plane orientation is not negligible compared with the bulk (2), it is necessary to regard aGaAs as complex. However, this point will not affect the (2) spectra in Fig. because aGaAs is canceled out in the normalization.
    • If the surface (2) of GaAs in the present in-plane orientation is not negligible compared with the bulk (2), it is necessary to regard aGaAs as complex. However, this point will not affect the (2) spectra in Fig. because aGaAs is canceled out in the normalization.
  • 20
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    • S. J. Lalama and A. F. Garito, Phys. Rev. A 1050-2947 10.1103/PhysRevA.20.1179 20, 1179 (1979).
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    • Lalama, S.J.1    Garito, A.F.2
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  • 22
    • 51749119179 scopus 로고    scopus 로고
    • We performed time-dependent density functional theory calculations and found that the imaginary part of Β zzz (2) (in resonance with the lowest allowed state) is positive for PNA and DEPNA. Our calculation results are consistent with Refs. as regards PNA.
    • We performed time-dependent density functional theory calculations and found that the imaginary part of Β zzz (2) (in resonance with the lowest allowed state) is positive for PNA and DEPNA. Our calculation results are consistent with Refs. as regards PNA.
  • 23
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    • The polarization SHG measurements showed that 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.58 and b=0.66 for PNA and 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.56 and b=0.61 for DEPNA. If the δ function is assumed for the orientational distribution (i.e., 〈 cos3 θ 〉 / 〈 cos θ 〉 = cos2 θ), θ=140° for PNA and θ=42°for DEPNA.
    • The polarization SHG measurements showed that 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.58 and b=0.66 for PNA and 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.56 and b=0.61 for DEPNA. If the δ function is assumed for the orientational distribution (i.e., 〈 cos3 θ 〉 / 〈 cos θ 〉 = cos2 θ), θ=140°for PNA and θ=42°for DEPNA.


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