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If the surface (2) of GaAs in the present in-plane orientation is not negligible compared with the bulk (2), it is necessary to regard aGaAs as complex. However, this point will not affect the (2) spectra in Fig. because aGaAs is canceled out in the normalization.
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If the surface (2) of GaAs in the present in-plane orientation is not negligible compared with the bulk (2), it is necessary to regard aGaAs as complex. However, this point will not affect the (2) spectra in Fig. because aGaAs is canceled out in the normalization.
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We performed time-dependent density functional theory calculations and found that the imaginary part of Β zzz (2) (in resonance with the lowest allowed state) is positive for PNA and DEPNA. Our calculation results are consistent with Refs. as regards PNA.
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We performed time-dependent density functional theory calculations and found that the imaginary part of Β zzz (2) (in resonance with the lowest allowed state) is positive for PNA and DEPNA. Our calculation results are consistent with Refs. as regards PNA.
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The polarization SHG measurements showed that 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.58 and b=0.66 for PNA and 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.56 and b=0.61 for DEPNA. If the δ function is assumed for the orientational distribution (i.e., 〈 cos3 θ 〉 / 〈 cos θ 〉 = cos2 θ), θ=140° for PNA and θ=42°for DEPNA.
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The polarization SHG measurements showed that 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.58 and b=0.66 for PNA and 〈 cos3 θ 〉 / 〈 cos θ 〉 =0.56 and b=0.61 for DEPNA. If the δ function is assumed for the orientational distribution (i.e., 〈 cos3 θ 〉 / 〈 cos θ 〉 = cos2 θ), θ=140°for PNA and θ=42°for DEPNA.
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