Effects of aging on organic aerosol from open biomass burning smoke in aircraft and laboratory studies

Atmospheric Chemistry and Physics

Volumn 11, Issue 23, 2011, Pages 12049-12064

  Cubison, M J ^a   Ortega, A M ^a   Hayes, P L ^a   Farmer, D K ^a   Day, D ^a   Lechner, M J ^a   Brune, W H ^b   Apel, E ^c   Diskin, G S ^d   Fisher, J A ^e   Fuelberg, H E ^f   Hecobian, A ^g   Knapp, D J ^c   Mikoviny, T ^h   Riemer, D ⁱ   Sachse, G W ^j   Sessions, W ^f   Weber, R J ^g   Weinheimer, A J ^c   Wisthaler, A ^h   Jimenez, J L ^a   more..

^a UNIVERSITY OF COLORADO   (United States)

^b PENNSYLVANIA STATE UNIVERSITY   (United States)

^c NATIONAL CENTER FOR ATMOSPHERIC RESEARCH   (United States)

^d NASA LANGLEY RESEARCH CENTER   (United States)

^e HARVARD UNIVERSITY   (United States)

^f FLORIDA STATE UNIVERSITY   (United States)

^g GEORGIA INSTITUTE OF TECHNOLOGY   (United States)

^h UNIVERSITY OF INNSBRUCK   (Austria)

ⁱ UNIVERSITY OF MIAMI   (United States)

^j NATIONAL INSTITUTE OF AEROSPACE   (United States)

more..

Author keywords

[No Author keywords available]

Indexed keywords

AEROSOL; AIRCRAFT; ATMOSPHERIC PLUME; BIOMASS BURNING; ENVIRONMENTAL FATE; LABORATORY METHOD; OXIDATION; SMOKE;

POA;

EID: 82955173008     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-11-12049-2011     Document Type: Article

References (86)

1. Aiken, A. C., DeCarlo, P. F., and Jimenez, J. L.: Elemental Analysis of Organic Species with Electron Ionization High-Resolution Mass Spectrometry, Anal. Chem., 79, 8350-8358, doi:10.1021/ac071150w, 2007. (Pubitemid 350060037)
2. Aiken, A. C., Salcedo, D., Cubison, M. J., Huffman, J. A., DeCarlo, P. F., Ulbrich, I. M., Docherty, K. S., Sueper, D., Kimmel, J. R., Worsnop, D. R., Trimborn, A., Northway, M., Stone, E. A., Schauer, J. J., Volkamer, R. M., Fortner, E., de Foy, B., Wang, J., Laskin, A., Shutthanandan, V., Zheng, J., Zhang, R., Gaffney, J., Marley, N. A., Paredes-Miranda, G., Arnott, W. P., Molina, L. T., Sosa, G., and Jimenez, J. L.: Mexico City aerosol analysis during MILAGRO using high resolution aerosol mass spectrometry at the urban supersite (T0)-Part 1: Fine particle composition and organic source apportionment, Atmos. Chem. Phys., 9, 6633-6653, doi:10.5194/acp-9-6633-2009, 2009.
3. Aiken, A. C., de Foy, B., Wiedinmyer, C., DeCarlo, P. F., Ul-brich, I. M., Wehrli, M. N., Szidat, S., Prevot, A. S. H., Noda, J., Wacker, L., Volkamer, R., Fortner, E., Wang, J., Laskin, A., Shutthanandan, V., Zheng, J., Zhang, R., Paredes-Miranda, G., Arnott, W. P., Molina, L. T., Sosa, G., Querol, X., and Jimenez, J. L.: Mexico city aerosol analysis during MILAGRO using high resolution aerosol mass spectrometry at the urban supersite (T0)-Part 2: Analysis of the biomass burning contribution and the non-fossil carbon fraction, Atmos. Chem. Phys., 10, 5315-5341, doi:10.5194/acp-10-5315-2010, 2010.
4. Akagi, S. K., Craven, J. S., Taylor, J. W., McMeeking, G. R., Yokel-son, R. J., Burling, I. R., Urbanski, S. P., Wold, C. E., Seinfeld, J. H., Coe, H., Alvarado, M. J., and Weise, D. R.: Evolution of trace gases and particles emitted by a chaparral fire in California, Atmos. Chem. Phys. Discuss., 11, 22483-22544, doi:10.5194/acpd-11-22483-2011, 2011.
5. Alfarra, M. R., Coe, H., Allan, J. D., Bower, K. N., Boudries, H., Canagaratna, M. R., Jimenez, J. L., Jayne, J. T., Garforth, A., Li, S. M., and Worsnop, D. R.: Characterization of Urban and Regional Organic Aerosols In the Lower Fraser Valley Using Two Aerodyne Aerosol Mass Spectrometers, Atmos. Environ., 38, 5745-5758, 2004. (Pubitemid 39277943)
6. Alfarra, M. R., Prevot, A. S. H., Szidat, S., Sandradewi, J., Weimer, S., Lanz, V. A., Schreiber, D., Mohr, M., and Baltensperger, U.: Identification of the mass spectral signature of organic aerosols from wood burning emissions, Environ. Sci. Technol., 41, 5770-5777, 2007. (Pubitemid 47292007)
7. Allan, J. D., Coe, H., Bower, K. N., Alfarra, M. R., Delia, A. E., Jimenez, J. L., Middlebrook, A. M., Drewnick, F., Onasch, T. B., Canagaratna, M. R., Jayne, J. T. and Worsnop, D. R: Technical Note: Extraction of Chemically Resolved Mass Spectra from Aerodyne Aerosol Mass Spectrometer Data, J. Aerosol Sci., 35, 909-922, 2004. (Pubitemid 38953786)
8. Apel, E. C., Hills, A. J., Lueb, R., Zindel, S., Eisele, S., and Riemer, D. D.: A fast-GC/MS system to measure C-2 to C-4 carbonyls and methanol aboard aircraft, J. Geophys. Res., 108, D8794, doi:10.1029/2002JD003199, 2003.
9. Bahreini, R., Keywood, M. D., Ng, N. L., Varutbangkul, V., Gao, S., Flagan, R. C., Seinfeld, J. H., Worsnop, D. R., and Jimenez, J. L.: Measurements of Secondary Organic Aerosol (SOA) from oxidation of cycloalkenes, terpenes, and m-xylene using an Aerodyne Aerosol Mass Spectrometer, Environ. Sci. Technol., 9, 5674-5688, doi:10.1021/es048061a, 2005.
10. Bond, T. C., Streets, D. G., Yarber, K. F., Nelson, S. M., Woo, J. H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geo-phys. Res., 109, D14203, doi:10.1029/ 2003JD003697, 2004. (Pubitemid 39366556)
11. Brock, C. A., Cozic, J., Bahreini, R., Froyd, K. D., Middlebrook, A. M., McComiskey, A., Brioude, J., Cooper, O. R., Stohl, A., Aikin, K. C., de Gouw, J. A., Fahey, D. W., Ferrare, R. A., Gao, R.-S., Gore, W., Holloway, J. S., HÜ bler, G., Jefferson, A., Lack, D. A., Lance, S., Moore, R. H., Murphy, D. M., Nenes, A., Novelli, P. C., Nowak, J. B., Ogren, J. A., Peischl, J., Pierce, R. B., Pilewskie, P., Quinn, P. K., Ryerson, T. B., Schmidt, K. S., Schwarz, J. P., Sodemann, H., Spackman, J. R., Stark, H., Thomson, D. S., Thornberry, T., Veres, P., Watts, L. A., Warneke, C., and Wollny, A. G.: Characteristics, sources, and transport of aerosols measured in spring 2008 during the aerosol, radiation, and cloud processes affecting Arctic Climate (ARCPAC) Project, Atmos. Chem. Phys., 11, 2423-2453, doi:10.5194/acp-11-2423- 2011, 2011.
12. Canagaratna, M. R., Jayne, J. T., Jimenez, J. L., Allan, J. D., Al-farra, M. R., Zhang, Q., Onasch, T. B., Drewnick, F., Coe, H., Middlebrook, A., Delia, A., Williams, L. R., Trimborn, A. M., Northway, M. J., DeCarlo, P. F., Kolb, C. E., Davidovits, P., and Worsnop, D. R.: Chemical and Microphysical Characterization of Ambient Aerosols with the Aerodyne Aerosol Mass Spectrometer, Mass Spectrom. Rev., 26, 185-222, 2007. (Pubitemid 46491711)
13. Capes, G., Johnson, B., McFiggans, G., Williams, P. I., Haywood, J., and Coe, H.: Aging of Biomass Burning Aerosols Over West Africa: Aircraft Measurements of Chemical Composition, Mi-crophysical Properties, and Emission Ratios. J. Geophys. Res., 113, D00C15, doi:10.1029/2008JD009845, 2008.
14. Cappa, C. D. and Jimenez, J. L.: Quantitative estimates of the volatility of ambient organic aerosol, Atmos. Chem. Phys., 10, 5409-5424, doi:10.5194/acp-10-5409-2010, 2010.
15. Chen, Q., Farmer, D. K., Schneider, J., Zorn, S. R., Heald, C. L., Karl, T. G., Guenther, A., Allan, J. D., Robinson, N., Coe, H., Kimmel, J. R., Pauliquevis, T., Borrmann, S., Pöschl, U., An-dreae, M. O., Artaxo, P., Jimenez, J. L., and Martin, S. T.: Mass Spectral Characterization of Submicron Biogenic Organic Particles in the Amazon Basin, Geophys. Res. Lett., 36, L20806, doi:10.1029/2009GL039880, 2009.
16. DeCarlo, P. F., Kimmel, J. R., Trimborn, A., Northway, M. J., Jayne, J. T., Aiken, A. C., Gonin, M., Fuhrer, K., Horvath, T., Docherty, K., Worsnop, D. R., and Jimenez, J. L.: Field-deployable, high-resolution, time-of-flight aerosol mass spectrometer, Anal. Chem. 78, 8281-8289, 2006. (Pubitemid 44927604)
17. DeCarlo, P. F., Dunlea, E. J., Kimmel, J. R., Aiken, A. C., Sueper, D., Crounse, J., Wennberg, P. O., Emmons, L., Shinozuka, Y., Clarke, A., Zhou, J., Tomlinson, J., Collins, D. R., Knapp, D., Weinheimer, A. J., Montzka, D. D., Campos, T., and Jimenez, J. L.: Fast airborne aerosol size and chemistry measurements above Mexico City and Central Mexico during the MILAGRO campaign, Atmos. Chem. Phys., 8, 4027-4048, doi:10.5194/acp-8-4027-2008, 2008.
18. DeCarlo, P. F., Ulbrich, I. M., Crounse, J., de Foy, B., Dunlea, E. J., Aiken, A. C., Knapp, D., Weinheimer, A. J., Campos, T., Wennberg, P. O., and Jimenez, J. L.: Investigation of the sources and processing of organic aerosol over the Central Mexican Plateau from aircraft measurements during MILAGRO, At-mos. Chem. Phys., 10, 5257-5280, doi:10.5194/acp-10-5257-2010, 2010.
19. De Gouw, J. and Jimenez, J. L.: Organic Aerosols in the Earth's Atmosphere, Environ. Sci. Technol., 43, 7614-7618, doi:10.1021/es9006004, 2009.
20. Docherty, K. S., Stone, E. A., Ulbrich, I. M., DeCarlo, P. F., Snyder, D. C., Schauer, J. J., Peltier, R. E., Weber, R. J., Murphy, D. M., Seinfeld, J. H., Grover, B. D., Eatough, D. J., and Jimenez, J. L.: Apportionment of Primary and Secondary Organic Aerosols in Southern California during the 2005 Study of Organic Aerosols in Riverside (SOAR), Environ. Sci. Technol., 42, 7655-7662, doi:10.1021/es8008166, 2008.
21. Docherty, K. S., Aiken, A. C., Huffman, J. A., Ulbrich, I. M., De-Carlo, P. F., Sueper, D., Worsnop, D. R., Snyder, D. C., Grover, B. D., Eatough, D. J., Goldstein, A. H., Ziemann, P. J., and Jimenez, J. L.: The 2005 Study of Organic Aerosols at Riverside (SOAR-1): instrumental intercomparisons and fine particle composition, Atmos. Chem. Phys. Discuss., 11, 6301-6362, doi:10.5194/acpd-11- 6301-2011, 2011.
22. Duplissy, J., DeCarlo, P. F., Dommen, J., Alfarra, M. R., Met-zger, A., Barmpadimos, I., Prevot, A. S. H., Weingartner, E., Tritscher, T., Gysel, M., Aiken, A. C., Jimenez, J. L., Cana-garatna, M. R., Worsnop, D. R., Collins, D. R., Tomlinson, J., and Baltensperger, U.: Relating hygroscopicity and composition of organic aerosol particulate matter, Atmos. Chem. Phys., 11, 1155-1165, doi:10.5194/acp-11-1155-2011, 2011.
23. Farmer, D. K., Kimmel, J. R., Phillips, G., Docherty, K. S., Worsnop, D. R., Sueper, D., Nemitz, E., and Jimenez, J. L.: Eddy-Covariance Measurements with High-Resolution Time-of-Flight Aerosol Mass Spectrometry: A New Approach to Chemically-Resolved Aerosol Fluxes, Atmos. Meas. Tech. 4, 1275-1289, doi:10.5194/amt-4-1275-2011, 2011.
24. Fisher, J. A., Jacob, D. J., Purdy, M. T., Kopacz, M., Le Sager, P., Carouge, C. C., Holmes, C. D., Yantosca, R. M., Batche-lor, R. L., Strong, K., Diskin, G. S., Fuelberg, H. E., Holloway, J. S., Hyer, E. J., McMillan, W. W., Warner, J. Streets, D. G., Zhang, Q., Wang, Y., and Wu, S.: Source attribution and in-terannual variability of Arctic pollution in spring constrained by aircraft (ARCTAS, ARCPAC) and satellite (AIRS) observations of carbon monoxide, Atmos. Chem. Phys., 10, 977-996, doi:10.5194/acp-10-977-2010, 2010.
25. Fisher, J. A., Jacob, D. J., Wang, Q., Bahreini, R., Carouge, C. C., Cubison, M. J., Dibb, J. E., Diehl, T., Jimenez, J. L., Leibensperger, E. J., Meinders, M. B. J., Pye, H. O. T., Quinn, P. K., Sharma, S., van Donkelaar, A., and Yan-tosca, R. M.: Sources, distribution, and acidity of sulfate-ammonium aerosol in the Arctic in winter-spring, Atmos. Environ., doi:10.1016/j.atmosenv. 2011.08.030, 2011.
26. Fuelberg, H. E., Harrigan, D. L., and Sessions, W.: A meteorological overview of the ARCTAS 2008 mission, Atmos. Chem. Phys., 10, 817-842, doi:10.5194/acp-10-817-2010, 2010.
27. George, I. J., and Abbatt, J. P. D.: Heterogeneous oxidation of atmospheric aerosol particles by gas-phase radicals, Nature Chem., 2, 713-722, doi:10.1038/nchem.806, 2010.
28. Grieshop, A. P., Logue, J. M., Donahue, N. M., and Robinson, A. L.: Laboratory investigation of photochemical oxidation of organic aerosol from wood fires 1: measurement and simulation of organic aerosol evolution, Atmos. Chem. Phys., 9, 1263-1277, doi:10.5194/acp-9-1263-2009, 2009a.
29. Grieshop, A. P., Donahue, N. M., and Robinson, A. L.: Laboratory investigation of photochemical oxidation of organic aerosol from wood fires 2: analysis of aerosol mass spectrometer data, At-mos. Chem. Phys., 9, 2227-2240, doi:10.5194/acp-9-2227-2009, 2009b.
30. Hallquist, M., Wenger, J. C., Baltensperger, U., Rudich, Y., Simpson, D., Claeys, M., Dommen, J., Donahue, N. M., George, C., Goldstein, A. H., Hamilton, J. F., Herrmann, H., Hoffmann, T., Iinuma, Y., Jang, M., Jenkin, M. E., Jimenez, J. L., Kiendler-Scharr, A., Maenhaut, W., McFiggans, G., Mentel, Th. F., Monod, A., Prévôt, A. S. H., Seinfeld, J. H., Surratt, J. D., Szmigielski, R., and Wildt, J.: The formation, properties and impact of secondary organic aerosol: current and emerging issues, Atmos. Chem. Phys., 9, 5155-5236, doi:10.5194/acp-9-5155-2009, 2009.
31. Hansel, A., Jordan, A., Holzinger, R., Prazeller, P., Vogel, W., and Lindinger, W.: Proton-Transfer Reaction Mass-Spectrometry-Online Trace Gas-Analysis at the ppb Level, Int. J. Mass Spec-trom., 149, 609-619, 1995.
32. Hawkins, L. N. and Russell, L. M.: Oxidation of ketone groups in transported biomass burning aerosol from the 2008 Northern California Lightning Series fires, Atmos. Environ., 44, 4142-4154, doi:10.1016/j.atmosenv.2010.07. 036, 2010.
33. Hecobian, A., Liu, Z., Hennigan, C. J., Huey, L. G., Jimenez, J. L., Cubison, M. J., Vay, S., Diskin, G. S., Sachse, G. W., Wisthaler, A., Mikoviny, T., Weinheimer, A. J., Liao, J., Knapp, D. J., Wennberg, P. O., Kürten, A., Crounse, J. D., Clair, J. St., Wang, Y., and Weber, R. J.: Comparison of the chemical evolution and characteristics of 495 biomass burning plumes intercepted by the NASA DC-8 aircraft during the ARCTAS/CARB-2008 field campaign, Atmos. Chem. Phys. Discuss., 11, 18589-18631, doi:10.5194/acpd-11-18589-2011, 2011
34. Hennigan, C. J., Sullivan, A. P., Collett, J. L., and Robinson, A. L.: Levoglucosan stability in biomass burning particles exposed to hydroxyl radicals, Geophys. Res. Lett., 37, L09806, doi:10.1029/2010GL043088, 2010a.
35. Hennigan, C. J., Miracolo, M. A., Engelhart, G. J., May, A. A., Presto, A. A., Lee, T., Sullivan, A. P., McMeeking, G. R., Coe, H., Wold, C. E., Hao, W.-M., Gilman, J. B., Kuster, W. C., de Gouw, J., Schichtel, B. A., J. L. Collett Jr., Kreidenweis, S. M., and Robinson, A. L.: Chemical and physical transformations of organic aerosol from the photo-oxidation of open biomass burning emissions in an environmental chamber, Atmos. Chem. Phys., 11, 7669-7686, doi:10.5194/acp-11-7669-2011, 2011.
36. Hoffmann, D., Tilgner, A., Iinuma, Y., and Herrmann, H.: Atmospheric Stability of Levoglucosan: A Detailed Laboratory and Modeling Study, Environ. Sci. Technol., 44, 694-699, 2010.
37. Hudman, R. C., Jacob, D. J., Turquety, S., Leibensperger, E. M., Murray, L. T., Wu, S., Gilliland, A. B., Avery, M., Bertram, T. H., and Brune, W.: Surface and lightning sources of nitrogen oxides over the United States: Magnitudes, chemical evolution, and outflow, J. Geophys. Res., 112, D12S05, doi:10.1029/2006JD007912, 2007. (Pubitemid 47241661)
38. Huffman, J. A., Docherty, K. S., Aiken, A. C., Cubison, M. J., Ul-brich, I. M., DeCarlo, P. F., Sueper, D., Jayne, J. T., Worsnop, D. R., Ziemann, P. J., and Jimenez, J. L.: Chemically-resolved aerosol volatility measurements from two megacity field studies, Atmos. Chem. Phys., 9, 7161-7182, doi:10.5194/acp-9-7161-2009, 2009a.
39. Huffman, J. A., Docherty, K. S., Mohr, C., Cubison, M. J., Ul-brich, I. M., Ziemann, P. J., Onasch, T. B., and Jimenez, J. L.: Chemically-Resolved Volatility Measurements of Organic Aerosol from Different Sources. Environ. Sci. Technol., 43, 5351-5357, doi:10.1021/es803539d, 2009b.
40. Hung, H. M. and Tang, C. W.: Effects of Temperature and Physical State on Heterogeneous Oxidation of Oleic Acid Droplets with Ozone, J. Phys. Chem., A114, 13104-13112, 2010.
41. Jacob, D. J., Crawford, J. H., Maring, H., Clarke, A. D., Dibb, J. E., Emmons, L. K., Ferrare, R. A., Hostetler, C. A., Russell, P. B., Singh, H. B., Thompson, A. M., Shaw, G. E., McCauley, E., Ped-erson, J. R., and Fisher, J. A.: The Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARC-TAS) mission: design, execution, and first results, Atmos. Chem. Phys., 10, 5191-5212, doi:10.5194/acp-10-5191-2010, 2010.
42. Jimenez, J. L., Jayne, J. T., Shi, Q., Kolb, C. E., Worsnop, D. R., Yourshaw, I., Seinfeld, J. H., Flagan, R. C., Zhang, X., Smith, K. A., Morris, J., and Davidovits, P.: Ambient Aerosol Sampling with an Aerosol Mass Spectrometer, J. Geophys. Res.-Atmos., 108, 8425, doi:10.1029/2001JD001213, 2003.
43. Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., Aiken, A. C., Docherty, K. D., Ulbrich, I.M., Grieshop, A. P., Robinson, A. L., Duplissy, J., Smith, J. D., Wilson, K. R., Lanz, V. A., Hueglin, C., Sun, Y. L., Tian, J., Laak-sonen, A., Raatikainen, T., Rautiainen, J., Vaattovaara, P., Ehn, M., Kulmala, M., Tomlinson, J. M., Collins, D. R., Cubison, M. J., Dunlea, E. J., Huffman, J. A., Onasch, T. B., Alfarra, M. R., Williams, P. I., Bower, K., Kondo, Y., Schneider, J., Drewnick, F., Borrmann, S., Weimer, S., Demerjian, K., Salcedo, D., Cot-trell, L., Griffin, R., Takami, A., Miyoshi, T., Hatakeyama, S., Shimono, A., Sun, J. Y., Zhang, Y. M., Dzepina, K., Kimmel, J. R., Sueper, D., Jayne, J. T., Herndon, S. C., Trimborn, A. M., Williams, L. R., Wood, E. C., Kolb, C. E., Middlebrook, A. M., Baltensperger, U., and Worsnop, D. R.: Evolution of Organic Aerosols in the Atmosphere, Science, 326, 1525-1529, doi:10.1126/science.1180353, 2009.
44. Kang, E., Root, M. J., Toohey, D. W., and Brune, W. H.: Introducing the concept of Potential Aerosol Mass (PAM), Atmos. Chem. Phys., 7, 5727-5744, doi:10.5194/acp-7-5727-2007, 2007.
45. Kang, E., Toohey, D. W., and Brune, W. H.: Dependence of SOA oxidation on organic aerosol mass concentration and OH exposure: experimental PAM chamber studies, Atmos. Chem. Phys., 11, 1837-1852, doi:10.5194/acp-11-1837-2011, 2011.
46. Katrib, Y., Biskos, G., Buseck, P. R., Davidovits, P., Jayne, J. T., Mochida, M., Wise, M. E., Worsnop, D. R., and Martin, S. T.: Ozonolysis of mixed oleic-acid/stearic-acid particles: Reaction kinetics and chemical morphology, J. Phys, Chem. A., 109, 10910-10919, doi:10.1021/jp054714d, 2005. (Pubitemid 43010675)
47. Kessler, S. H., Smith, J. D., Che, D. L., Worsnop, D. R., Wilson, K. R., and Kroll, J. H.: Chemical Sinks of Organic Aerosol: Kinetics and Products of the Heterogeneous Oxidation of Erythri-tol and Levoglucosan, Environ. Sci. Technol., 44, 7005-7010, doi:10.1021/es101465m, 2010.
48. Kimmel, J. R., Farmer, D. K., Cubison, M. J., Sueper, D., Tanner, C., Nemitz, E., Worsnop, D. R., Gonin, M., and Jimenez, J. L.: Real-time Aerosol Mass Spectrometry with Millisecond Resolution, Int. J. Mass. Spectrom., 303, 15-26, doi:10.1016/j.ijms.2010.12.004, 2011.
49. Kroll, J. H., Donahue, N. M. Jimenez, J. L., Kessler, S. H., Cana-garatna, M. R., Wilson, K. R., Altieri, K. E., Mazzoleni, L. R., Wozniak, A. S., Bluhm, H., Mysak, E. R., Smith, J. D., Kolb, C. E., and Worsnop, D. R.: Carbon Oxidation State as a Metric for Describing the Chemistry of Atmospheric Organic Aerosol, Nature Chem., 3, 133-139, doi:10.1038/NCHEM.948, 2011.
50. Lee, T., Sullivan, A. P., Mack, L., Jimenez, J. L., Kreidenweis, S. M., Onasch, T. B., Worsnop, D. R., Malm, W., Wold, C. E., Hao, W. M., and Collett, J. L.: Variation of chemical smoke marker emissions during flaming vs. smoldering phases of laboratory open burning of wildland fuels, Aerosol Sci. Technol., 44, 1-5, doi:10.1080/02786826.2010.499884, 2010
51. Liggio J., Li S. M., and McLaren, R.: Reactive update of gly-oxal by particulate matter, J. Geophys. Res., 110, D10304, doi:10.1029/2004JD005113, 2005. (Pubitemid 40919776)
52. Massoli, P., Lambe, A. T., Ahern, A. T., Williams, L. R., Ehn, M., Mikkilä, J., Canagaratna, M. R., Brune, W. H., Onasch, T. B., Jayne, J.T., Petäjä, T., Kulmala, M., Laaksonen, A., Kolb, C. E. Davidovits, P., and Worsnop, D. R.: Relationship between Aerosol Oxidation Level and Hygroscopic Properties of Laboratory Generated Secondary Organic Aerosol (SOA) Particles, Geophys. Res. Lett., 37, L24801, doi:10.1029/2010GL045258, 2010.
53. McMeeking, G. R., Kreidenweis, S. M., Baker, S., Carrico, C. M., Chow, J. C., Collett, J. L., Hao, W. M., Holden, A. S., Kirch-stetter, T. W., Malm, W. C., Moosmuller, H., Sullivan, A. P., and Wold, C. E.: Emissions of trace gases and aerosols during the open combustion of biomass in the laboratory, J. Geophys. Res., 114, D19210, doi:10.1029/2009JD011836, 2009.
54. Mohr, C., Huffman, J. A., Cubison, M. J., Aiken, A. C., Docherty, K. S., Kimmel, J. R., Ulbrich, I. M., Hannigan, M., Garcia, J., and Jimenez, J. L.: Characterization of Primary Organic Aerosol Emissions from Meat Cooking, Trash Burning, and Motor Vehicles with High-Resolution Aerosol Mass Spectrometry and Comparison with Ambient and Chamber Observations, Environ. Sci. Technol., 43, 2443-2449, doi:10.1021/es8011518, 2009.
55. Murphy, D. M. Czizco, D. J., Froyd, K. D., Hudson, P. K., Matthew, B. M., Middlebrook, A. M., Peltier, R. E., Sullivan, A., Thomson, D.S., and Weber, R. J.: Single-particle mass-spectrometry of tropospheric aerosol particles, J. Geophys. Res., 111, D23S32, doi:10.1029/2006JD007340, 2006. (Pubitemid 47260840)
56. Ng, N. L., Canagaratna, M. R., Zhang, Q., Jimenez, J. L., Tian, J., Ulbrich, I. M., Kroll, J. H., Docherty, K. S., Chhabra, P. S., Bahreini, R., Murphy, S. M., Seinfeld, J. H., Hildebrandt, L., Donahue, N. M., DeCarlo, P. F., Lanz, V. A., Prévôt, A. S. H., Dinar, E., Rudich, Y., and Worsnop, D. R.: Organic aerosol components observed in Northern Hemispheric datasets from Aerosol Mass Spectrometry, Atmos. Chem. Phys., 10, 4625-4641, doi:10.5194/acp-10-4625-2010, 2010.
57. Ng, N. L., Herndon, S. C., Trimborn, A., Canagaratna, M. R., Croteau, P., Onasch, T. M., Sueper, D., and Worsnop, D. R.: An Aerosol Chemical Speciation Monitor (ACSM) for routine monitoring of atmospheric aerosol composition, Aerosol Sci. Tech-nol., 45, 770-784, 2011a.
58. Ng, N. L., Canagaratna, M. R., Jimenez, J. L., Zhang, Q., Ul-brich, I. M., and Worsnop, D. R.: Real-Time Methods for Estimating Organic Component Mass Concentrations from Aerosol Mass Spectrometer Data, Environ. Sci. Technol., 45, 910-916, doi:10.1021/es102951k, 2011b.
59. Ortega, A., Brune, W., Cubison, M. J., Welsh-Bon, D., de Gouw, J. A., Lee, T., Kreidenweis, S., Robinson, A. L., Hennigan, C. J., and Jimenez, J. L.: Variability of Secondary Organic Aerosol Production and Aerosol Oxidation from Rapid and Intense Photochemical Processing of Biomass Burning Smokes, International Aerosol Conference, Helsinki, Finland, 29 August-3 September 2010, P3W32, available online at: http://www.atm. helsinki.fi/IAC2010/abstracts/pdf/ 224.pdf, 2010.
60. Robinson, A. L., Subramanian, R., Donahue, N. M., Bernardo-Bricke, A., and Rogge, W. F.: Source Apportionment of Molecular Markers and Organic Aerosol1. Polycyclic Aromatic Hydrocarbons and Methodology for Data Visualization, Environ. Sci. Technol., 40, 7803-7810, doi:10.1021/es0510414, 2006. (Pubitemid 46012579)
61. Robinson, A. L., Donahue, N. M., Shrivastava, M. K., Weitkamp, E. A., Sage, A. M., Grieshop, A. P., Lane, T. E., Pierce, J. R., and Pandis, S. N.: Rethinking organic aerosols: Semivolatile emissions and photochemical aging, Science, 315, 1259-1262, doi:10.1126/science.1133061, 2007. (Pubitemid 46364260)
62. Sachse, G. W., Hill, G. F., and Perry, M. G.: Fast-response, high-precision Carbon Monoxide sensor using a tunable diode-laser absorption technique, J. Geophys. Res., 92, 2071-2081, 1987. (Pubitemid 17070932)
63. Sage, A. M., Weitkamp, E. A., Robinson, A. L., and Donahue, N. M.: Evolving mass spectra of the oxidized component of organic aerosol: results from aerosol mass spectrometer analyses of aged diesel emissions, Atmos. Chem. Phys., 8, 1139-1152, doi:10.5194/acp-8-1139-2008, 2008.
64. Schauer, J. J., Rogge, W. F. Hildemann, L. M., Mazurek, M. A., and Cass, G. R.: Source apportionment of airborne particulate matter using organic compounds as tracers, Atmos. Environ., 30, 3837-3855, 1996.
65. Schneider, J., Weimer, S., Drewnick, F., Borrmann, S., Helas, G., Gwaze, P., Schmid, O., Andreae, M. O. and Kirchner, U.: Mass spectrometric analysis and aerodynamic properties of various types of combustion-related aerosol particles, Int. J. Mass. Spec., 258, 37-49, 2006.
66. Simoneit, B. R. T., Schauer, J. J., Nolte, C. G., Oros, D. R., Elias, V. O., Fraser, M. P., Rogge, W. F., Cass, G. R.: Levoglucosan, a tracer for cellulose in biomass burning and atmospheric particles, Atmos. Environ., 33, 173-182, 1999. (Pubitemid 28561853)
67. Singh, H. B., Anderson, B. E., Brune, W. H., Cai, C., Cohen, R. C., Crawford, J. H., Cubison, M. J., Czech, E. P., Emmons, L., Fu-elberg, H. E., Huey, G., Jacob, D. J., Jimenez, J. L., Kaduwela, A., Kondo, Y., Mao, J., Olson, J. R., Sachse, G. W., Vay, S. A., Weinheimer, A., Wennberg, P. O., Wisthaler, A., and the ARC-TAS Science Team: Pollution influences on atmospheric composition and chemistry at high northern latitudes: Boreal and California forest fire emissions, Atmos. Environ., 44, 4553-4564, doi:10.1016/j.atmosenv. 2010.08.026, 2010.
68. Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O. Baker, D. M., Duda, M. G., Huang, X., Wang, W., and Powers, J. G.: A description of the Advanced Research WRF version 3.874, NCAR Tech. Note NCAR/TN-475+STR, 113, 2008.
69. Spracklen, D. V., Jimenez, J. L., Carslaw, K. S., Worsnop, D. R., Evans, M. J., Mann, G. W., Zhang, Q., Canagaratna, M. R., Allan, J., Coe, H., McFiggans, G., Rap, A., and Forster, P.: Aerosol mass spectrometer constraint on the global secondary organic aerosol budget, Atmos. Chem. Phys. Discuss., 11, 5699-5755, doi:10.5194/acpd-11-5699-2011, 2011.
70. Takegawa, N., Miyakawa, T., Kawamura, K., and Kondo, Y.: Contribution of Selected Dicarboxylic and w-Oxocarboxylic Acids in Ambient Aerosol to the m/z 44 Signal of an Aerodyne Aerosol Mass Spectrometer, Aerosol Sci. Technol., 41, 418-437, 2007. (Pubitemid 46393087)
71. Ulbrich, I. M., Canagaratna, M. R., Zhang, Q., Worsnop, D. R., and Jimenez, J. L.: Interpretation of organic components from Positive Matrix Factorization of aerosol mass spectrometric data, At-mos. Chem. Phys., 9, 2891-2918, doi:10.5194/acp-9-2891-2009, 2009a.
72. Ulbrich, I. M., Lechner, M., and Jimenez, J. L.: AMS Spectral Database, http://cires.colorado.edu/jimenez-group/AMSsd/, last access: 2 December 2011, 2009b.
73. Vaden, T. D., Imre, D., Beranek, J., Shrivastava, M., and Ze-lenyuk, A.: Evaporation kinetics and phase of laboratory and ambient secondary organic aerosol, PNAS, 108, 2190-2195, doi:10.1073/pnas.1013391108, 2011.
74. Virtanen, A., Joutsensaara, J., Koop, T., Kannosto, J., Yli-Pirila, P., Leskinen, J., Makela, J. M., Holopainen, J. K., Pöschl, U., Kul-mala, M., Worsnop, D. R., and Laaksonen, A.: An amorphous solid state of biogenic secondary organic aerosol particles, Nature, 467, 824-827, doi:10.1038/ nature09455, 2010.
75. Volkamer, R., Jimenez, J. L., San Martini, F., Dzepina, K., Zhang, Q., Salcedo, D., Molina, M. T., Worsnop, D. R., and Molina, M. J.: Secondary organic aerosol formation from anthropogenic air pollution: Rapid and higher than expected, Geophys. Res. Lett., 33, L17811, doi:10.1029/2006GL026899, 2006. (Pubitemid 44945682)
76. Wang, Q., Jacob, D. J., Fisher, J. A., Mao, J., Leibensperger, E. M., Carouge, C. C., Le Sager, P., Kondo, Y., Jimenez, J. L., Cubi-son, M. J., and Doherty, S. J.: Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter-spring: implications for radiative forcing, Atmos. Chem. Phys. Discuss., 11, 19395-19442, doi:10.5194/acpd-11-19395-2011, 2011.
77. Warneke, C., Bahreini, R., Brioude, J., Brock, C. A., de Gouw, J. A., Fahey, D. W., Froyd, K. D., Holloway, J. S., Middlebrook, A. M., Miller, L., Montzka, S., Murphy, D. M., Peischl, J., Ryerson, T. B., Schwarz, J. P., Spackmann, J. R., and Veres, P.: Biomass burning in Siberia and Kazakhstan as an important source for haze over the Alaskan Arctic in April 2008, Geophys. Res. Lett., 36, L02813, doi:10.1029/2008GL036194, 2009.
78. Warneke, C., Froyd, K. D., Brioude, J., Bahreini, R., Brock, C. A., Cozic, J., de Gouw, J. A., Fahey, D. W., Ferrare, R., Hol-loway, J. S., Middlebrook, A. M., Miller, L., Montzka, S., Schwarz, J. P., Sodemann, H., Spackmann, J. R., and Stohl, A.: An important contribution to springtime Arctic aerosol from biomass burning in Russia, Geophys. Res. Lett., 37, L01801, doi:10.1029/2009GL041816, 2010.
79. Weimer, S., Alfarra, M. R., Schreiber, D., Mohr, C., Prevot, A. S. H., and Baltensperger, U.: Organic aerosol mass spectral signatures from wood-burning emissions: Influence of burning conditions and wood type, J. Geophys. Res., 113, D10304, doi:10.1029/2007JD009309, 2008.
80. Weinheimer, A. J., Walega, J. G., Ridley, B. A., Gary, B. L., Blake, D. R., Blake, N. J., Rowland, F. S., Sachse, G. W., Anderson, B. E., and Collins, J. E.: Meridional distributions of NOx, Noy, and other species in the lower stratosphere and upper troposphere during AASE II, Geophys. Res. Lett., 21, 2583-2586, 1994.
81. Wisthaler, A., Hansel., A., Dickerson, R. R., and Crutzen, P. J.: Organic trace gas measurements by PTR-MS during INDOEX 1999, J. Geophys. Res. 107, D8024, doi:10.1029/2001JD000576, 2002. (Pubitemid 44793913)
82. Wisthaler, A., Mikoviny, T., Diskin, G. S., Sachse, G. W., and Burkhart, J. F.: Chemical characterization of air masses transported to the Arctic during the ARCTAS-A spring deployment: biomass burning versus fossil fuel combustion signatures, AGU Fall Meeting, San Francisco, USA, A33F-05, 2009.
83. Yokelson, R. J., Crounse, J. D., DeCarlo, P. F., Karl, T., Urbanski, S., Atlas, E., Campos, T., Shinozuka, Y., Kapustin, V., Clarke, A. D., Weinheimer, A., Knapp, D. J., Montzka, D. D., Holloway, J., Weibring, P., Flocke, F., Zheng, W., Toohey, D., Wennberg, P. O., Wiedinmyer, C., Mauldin, L., Fried, A., Richter, D., Walega, J., Jimenez, J. L., Adachi, K., Buseck, P. R., Hall, S. R., and Shetter, R.: Emissions from biomass burning in the Yucatan, At-mos. Chem. Phys., 9, 5785-5812, doi:10.5194/acp-9-5785-2009, 2009.
84. Zhang, Q., Jimenez, J. L., Canagaratna, M. R., Allan, J. D., Coe, H., Ulbrich, I., Alfarra, M. R., Takami, A., Middlebrook, A. M., Sun, Y. L., Dzepina, K., Dunlea, E., Docherty, K. S., De-Carlo, P. F., Salcedo, D., Onasch, T., Jayne, J. T., Miyoshi, T., Shimono, A., Hatakeyama, S., Takegawa, N., Kondo, Y., Schneider, J., Drewnick, F., Weimer, S., Demerjian, K., Williams, P. I., Bower, K., Bahreini, R., Cottrell, L., Griffin, R. J., Rautiainen, J., and Worsnop, D. R.: Ubiquity and Dominance of Oxygenated Species in Organic Aerosols in Anthropogenically-Influenced Northern Hemisphere Mid-latitudes. Geophys. Res. Lett., 34, L13801, doi:10.1029/2007GL029979, 2007. (Pubitemid 47399659)
85. Zhang, X., Hecobian, A., Zheng, M., Frank, N. H., and Weber, R. J.: Biomass burning impact on PM2.5 over the southeastern US during 2007: integrating chemically speciated FRM filter measurements, MODIS fire counts and PMF analysis, Atmos. Chem. Phys., 10, 6839-6853, doi:10.5194/acp-10-6839-2010, 2010.
86. Ziemann, P. J.: Aerosol products, mechanisms, and kinetics of heterogeneous reactions of ozone with oleic acid in pure and mixed particles, Faraday Discuss., 130, 469-490, doi:10.1039/b417502f, 2005. (Pubitemid 41223701)