Development cycle 2 of the Modular Earth Submodel System (MESSy2)

Geoscientific Model Development

Volumn 3, Issue 2, 2010, Pages 717-752

  Jockel P ^a,d   Kerkweg, A ^b   Pozzer, A ^c   Sander, R ^a   Tost, H ^a   Riede, H ^a   Baumgaertner, A ^a   Gromov, S ^a   Kern, B ^a  

^a MAX PLANCK INSTITUTE FOR CHEMISTRY   (Germany)

^b JOHANNES GUTENBERG UNIVERSITY   (Germany)

^c CYPRUS INSTITUTE   (Cyprus)

^d GERMAN AEROSPACE CENTER DLR   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

ATMOSPHERIC CHEMISTRY; ATMOSPHERIC GENERAL CIRCULATION MODEL; CLIMATE MODELING; EARTH STRUCTURE; NUMERICAL MODEL;

EID: 78751532389     PISSN: 1991959X     EISSN: 19919603     Source Type: Journal    
DOI: 10.5194/gmd-3-717-2010     Document Type: Article

References (83)

1. Allen, D. J. and Pickering, K. E.: Evaluation of lightning flash rate parameterizations for use in a global chemical transport model, J. Geophys. Res., 107, 4711, doi:10.1029/2002JD002066, 2002.
2. Allen, D. J., Rood, R. B., Thompson, A. M., and Hudson, R. D.: Three-dimensional radon 222 calculations using assimilated meteorological data and a convective mixing algorithm, J. Geophys. Res., 101, 6871-6881, 1996.
3. Austin, J., Struthers, H., Scinocca, J., Plummer, D. A., Akiyoshi, H., Baumgaertner, A. J. G., Bekki, S., Bodeker, G. E., Braesicke, P., Brühl, C., Butchart, N., Chipperfield, M. P., Cugnet, D., Dameris, M., Dhomse, S., Frith, S., Garny, H., Gettelman, A., Hardiman, S. C., Jöckel, P., Kinnison, D., Kubin, A., Lamarque, J. F., Langematz, U., Mancini, E., Marchand, M., Michou, M., Morgenstern, O., Nakamura, T., Nielsen, J. E., Pitari, G., Pyle, J., Rozanov, E., Shepherd, T. G., Shibata, K., Smale, D., Teyssèdre, H., and Yamashita, Y.: Chemistry-climate model simulations of spring Antarctic ozone, J. Geophys. Res., 115, D00M11, doi:10.1029/2009JD013577, http://dx.doi.org/10. 1029/2009JD013577, 2010.
4. x produced by low energy electrons, Atmos. Chem. Phys., 9, 2729-2740, doi:10.5194/acp-9-2729-2009, 2009.
5. Baumgaertner, A. J. G., Jöckel, P., Riede, H., Stiller, G., and Funke, B.: Energetic particle precipitation in ECHAM5/MESSy - Part 2: Solar proton events, Atmos. Chem. Phys., 10, 7285-7302, doi:10.5194/acp-10-7285-2010, 2010a.
6. Baumgaertner, A. J. G., Jöckel, P., Steil, B., Tost, H., and Sander, R.: A fast stratospheric chemistry solver: the E4CHEM submodel for the atmospheric chemistry global circulation model EMAC, Geosci. Model Dev., 3, 321-328, doi:10.5194/gmd-3-321-2010, 2010b.
7. Blitz, M., Heard, D., Pilling, M., Arnold, S. R., and Chipperfield, M. P.: Pressure and temperature-dependent quantum yields for the photodissocuation od acetone between 279 and 327.5 nm, Geophys. Res. Lett., 31, L06111, doi:10.1029/2003GL018793, 2004.
8. Brenninkmeijer, C. A. M., Crutzen, P., Boumard, F., Dauer, T., Dix, B., Ebinghaus, R., Filippi, D., Fischer, H., Franke, H., Frieß, U., Heintzenberg, J., Helleis, F., Hermann, M., Kock, H. H., Koeppel, C., Lelieveld, J., Leuenberger, M., Martinsson, B. G., Miemczyk, S., Moret, H. P., Nguyen, H. N., Nyfeler, P., Oram, D., O'Sullivan, D., Penkett, S., Platt, U., Pupek, M., Ramonet, M., Randa, B., Reichelt, M., Rhee, T. S., Rohwer, J., Rosenfeld, K., Scharffe, D., Schlager, H., Schumann, U., Slemr, F., Sprung, D., Stock, P., Thaler, R., Valentino, F., van Velthoven, P., Waibel, A., Wandel, A., Waschitschek, K., Wiedensohler, A., Xueref-Remy, I., Zahn, A., Zech, U., and Ziereis, H.: Civil Aircraft for the regular investigation of the atmosphere based on an instrumented container: The new CARIBIC system, Atmos. Chem. Phys., 7, 4953-4976, doi:10.5194/acp-7-4953-2007, 2007. (Pubitemid 47505049)
9. Bronstein, I. N., Semendjajew, K. A., Musiol, G., and Mühlig, H.: Taschenbuch der Mathematik, Verlag Harri Deutsch, 2005.
10. Buchholz, J.: Simulations of physics and chemistry of polar stratospheric clouds with a general circulation model, Ph. D. thesis, University of Mainz, Germany, http://nbn-resolving.de/urn/resolver.pl?urn=urn:nbn:de:hebis:77-8187, 2005.
11. Damian, V., Sandu, A., Damian, M., Potra, F., and Carmichael, G. R.: The kinetic preprocessor KPP - a software environment for solving chemical kinetics, Comput. Chem. Eng., 26, 1567-1579, 2002.
12. 222 using on-line and off-line global models at different horizontal resolutions: A detailed comparison with measurements, Tellus, 51 B, 573-602, 1999.
13. Emmons, L. K., Hauglustaine, D. A., Müller, J.-F., Carroll, M. A., Brasseur, G. P., Brunner, D., Staehelin, J., Thouret, V., and Marenco, A.: Data composites of airborne observation of tropospheric ozone and its precursor, J. Geophys. Res., 105, 20497-20538, 2000.
14. 5 hydrolysis on global model budgets of tropospheric nitrogen oxides, ozone and OH, Geophys. Res. Lett., 32, L09813, doi:10.1029/2005GL022469, 2005. (Pubitemid 40875844)
15. Giorgetta, M. A. and Bengtsson, L.: The potential role of the quasibiennial oscillation in the stratosphere-troposphere exchange as found in water vapour in general circulation model experiments, J. Geophys. Res., 104, 6003-6019, 1999.
16. Grewe, V., Brunner, D., Dameris, M., Grenfell, J. L., Hein, R., Shindell, D., and Staehelin, J.: Origin and variability of upper tropospheric nitrogen oxides and ozone at northern mid-latitudes, Atmos. Environ., 35, 3421-3433, 2001.
17. Gromov, S., Jöckel, P., Sander, R., and Brenninkmeijer, C. A. M.: A kinetic chemistry tagging technique and its application to modelling the stable isotopic composition of atmospheric trace gases, Geosci. Model Dev., 3, 337-364, doi:10.5194/gmd-3-337-2010, 2010.
18. Holmes, C. D., Jacob, D. J., and Yang, X.: Global lifetime of elemental mercury against oxidation by atomic bromine in the free troposphere, Geophys. Res. Lett., 33, L20808, doi:10.1029/2006GL027176, 2006. (Pubitemid 44941737)
19. Holmes, C. D., Jacob, D. J., Corbitt, E. S., Mao, J., Yang, X., Talbot, R., and Slemr, F.: Global atmospheric model for mercury including oxidation by bromine atoms, Atmos. Chem. Phys., 10, 12037-12057, doi:10.5194/acp-10-12037- 2010, 2010.
20. Jacob, D. J., Field, B. D., Li, Q., Blake, D. R., de Gouw, J., Warneke, C., Hansel, A., Wisthaler, A., Singh, H. B., and Guenther, A.: Global budget of methanol: Constraints from atmospheric observations, J. Geophys. Res., 110, D08303, doi:10.1029/2004JD005172, 2005. (Pubitemid 40906177)
21. Jacobson, M. Z.: Fundamentals of atmospheric modeling, Cambridge University Press, 2nd edn., 2005.
22. 14CO as tracer for atmosperic chemistry and transport, Ph. D. thesis, Combined Faculties for the Natural Sciences and for Mathematics of the Rupertus Carola University of Heidelberg, Germany, http://www.ub.uni-heidelberg.de/archiv/1426, 2000.
23. Jöckel, P.: Technical note: Recursive rediscretisation of geoscientific data in the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys., 6, 3557-3562, doi:10.5194/acp-6-3557-2006, 2006. (Pubitemid 44306766)
24. 14CO at the surface level: A solar cycle adjusted, zonal average climatology based on observations, J. Geophys. Res., 107, 4656, doi:10.1029/2001JD001104, 2002. (Pubitemid 44793810)
25. 14CO to changes in solar activity, J. Geophys. Res., 105, 6737-6744, 2000.
26. 14CO, J. Geophys. Res., 107, 4446, doi:10.1029/2001JD001324, 2002.
27. Jöckel, P., Brenninkmeijer, C. A. M., and Crutzen, P. J.: A discussion on the determination of atmospheric OH and its trends, Atmos. Chem. Phys., 3, 107-118, doi:10.5194/acp-3-107-2003, 2003.
28. Jöckel, P., Sander, R., Kerkweg, A., Tost, H., and Lelieveld, J.: Technical Note: The Modular Earth Submodel System (MESSy) - a new approach towards Earth System Modeling, Atmos. Chem. Phys., 5, 433-444, doi:10.5194/acp-5-433-2005, 2005.
29. Jöckel, P., Tost, H., Pozzer, A., Brühl, C., Buchholz, J., Ganzeveld, L., Hoor, P., Kerkweg, A., Lawrence, M. G., Sander, R., Steil, B., Stiller, G., Tanarhte, M., Taraborrelli, D., van Aardenne, J., and Lelieveld, J.: The atmospheric chemistry general circulation model ECHAM5/MESSy1: consistent simulation of ozone from the surface to the mesosphere, Atmos. Chem. Phys., 6, 5067-5104, doi:10.5194/acp-6-5067-2006, 2006.
30. Jöckel, P., Kerkweg, A., Buchholz-Dietsch, J., Tost, H., Sander, R., and Pozzer, A.: Technical Note: Coupling of chemical processes with the Modular Earth Submodel System (MESSy) submodel TRACER, Atmos. Chem. Phys., 8, 1677-1687, doi:10.5194/acp-8-1677-2008, 2008.
31. Keene, W. C., Sander, R., Pszenny, A. A. P., Vogt, R., Crutzen, P. J., and Galloway, J. N.: Aerosol pH in the marine boundary layer: A review and model evaluation, J. Aerosol Sci., 29, 339-356, doi:10.1016/S0021-8502 (97) 10011-8, 1998.
32. Kerkweg, A., Buchholz, J., Ganzeveld, L., Pozzer, A., Tost, H., and Jöckel, P.: Technical Note: An implementation of the dry removal processes DRY DEPosition and SEDImentation in the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys., 6, 4617-4632, doi:10.5194/acp-6-4617-2006, 2006a.
33. Kerkweg, A., Sander, R., Tost, H., and Jöckel, P.: Technical note: Implementation of prescribed (OFFLEM), calculated (ON-LEM), and pseudo-emissions (TNUDGE) of chemical species in the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys., 6, 3603-3609, doi:10.5194/acp-6-3603-2006, 2006b. (Pubitemid 44329040)
34. Kerkweg, A., Sander, R., Tost, H., Jöckel, P., and Lelieveld, J.: Technical Note: Simulation of detailed aerosol chemistry on the global scale using MECCA-AERO, Atmos. Chem. Phys., 7, 2973-2985, doi:10.5194/acp-7-2973-2007, 2007. (Pubitemid 46906748)
35. Kerkweg, A., Jöckel, P., Pozzer, A., Tost, H., Sander, R., Schulz, M., Stier, P., Vignati, E., Wilson, J., and Lelieveld, J.: Consistent simulation of bromine chemistry from the marine boundary layer to the stratosphere - Part 1: Model description, sea salt aerosols and pH, Atmos. Chem. Phys., 8, 5899-5917, doi:10.5194/acp-8-5899-2008, 2008a.
36. Kerkweg, A., Jöckel, P., Warwick, N., Gebhardt, S., Brenninkmeijer, C. A. M., and Lelieveld, J.: Consistent simulation of bromine chemistry from the marine boundary layer to the stratosphere - Part 2: Bromocarbons, Atmos. Chem. Phys., 8, 5919-5939, doi:10.5194/acp-8-5919-2008, 2008b.
37. Kirner, O.: Prozessstudien der stratosphaerischen Chemie und Dynamik mit Hilfe des Chemie-Klima-Modells ECHAM5/MESSy1, Ph. D. thesis, Universitaet Karsruhe, http://digbib.ubka.uni-karlsruhe.de/volltexte/1000010199, 2008.
38. Kirner, O., Ruhnke, R., Buchholz-Dietsch, J., Jöckel, P., Brühl, C., and Steil, B.: Simulation of polar stratospheric clouds in the chemistry-climate-model EMAC via the submodel PSC, Geosci. Model Dev. Discuss., 3, 2071-2108, doi:10.5194/gmdd-3-2071-2010, 2010.
39. Koch, D. M., Jacob, D. J., and Graustein, W. C.: Vertical transport of tropospheric aerosols as indicated by and in a chemical tracer model, J. Geophys. Res., 101, 18651-18666, 1996.
40. Landgraf, J. and Crutzen, P. J.: An efficient method for online calculations of photolysis and heating rates, J. Atmos. Sci., 55, 863-878, 1998.
41. Lauer, A., Eyring, V., Hendricks, J., Jöckel, P., and Lohmann, U.: Global model simulations of the impact of ocean-going ships on aerosols, clouds, and the radiation budget, Atmos. Chem. Phys., 7, 5061-5079, doi:10.5194/acp-7-5061-2007, 2007. (Pubitemid 47530942)
42. Leroy, S. S.: The Effects of Orbital Precession on Remote Climate Monitoring, J. Climate, 14, 4330-4337, 2001.
43. Lingenfelter, R. E.: Production of carbon 14 by cosmic-ray neutrons, Rev. Geophys., 1, 35-55, 1963.
44. 7Be on wet deposition and transport in a global threedimensional chemical tracer model driven by assimilated meteorological fields, J. Geophys. Res., 106, 12109-12128, 2001.
45. MacKay, C., Pandow, M., and Wolfgang, R.: On the chemistry of natural radiocarbon, J. Geophys. Res., 68, 3929-3931, 1963.
46. Mahowald, N. M., Rasch, P. J., Eaton, B. E., Whittlestone, S., and Prinn, R. G.: Transport of 222Radon to the remote troposphere using the Model of Atmospheric Transport and Chemistry and assimilated winds from ECMWF and the National Center for Environmental Prediction/NCAR, J. Geophys. Res., 102, 28139-28151, 1997. (Pubitemid 127599874)
47. Marenco, A., Thouret, V., Nédélec, P., Smit, H., Helten, M., Kley, D., Karcher, F., Simon, P., Law, K., Pyle, J., Poschmann, G., Von Wrede, R., Hume, C., and Cook, T.: Measurement of ozone and water vapor by Airbus in-service aircraft: The MOZAIC airborne program, An overview, J. Geophys. Res., 103, 25631-25642, 1998. (Pubitemid 128700109)
48. Masarik, J. and Beer, J.: Simulation of particle fluxes and cosmogenic nuclide production in the Earth's atmosphere, J. Geophys. Res., 104, 12099-12111, 1999.
49. Matsumoto, M. and Nishimura, T.: Mersenne twister: a 623-dimensionally equidistributed uniform pseudo-random number generator, ACM Trans. Model. Comput. Simul., 8, 3-30, 1998.
50. Nissen, K. M., Matthes, K., Langematz, U., and Mayer, B.: Towards a better representation of the solar cycle in general circulation models, Atmos. Chem. Phys., 7, 5391-5400, doi:10.5194/acp-7-5391-2007, 2007. (Pubitemid 47603134)
51. Novelli, P. C., Masarie, K. A., and Lang, P. M.: Distributions and recent changes in carbon monoxide in the lower troposphere, J. Geophys. Res., 103, 19015-19033, 1998.
52. Pandow, M., MacKay, C., and Wolfgang, R.: The reaction of atomic carbon with oxygen: Significance for the natural radio-carbon cycle, J. Inorg. Nucl. Chem., 14, 153-158, 1960.
53. x for use in regional and chemical transport models, J. Geophys. Res., 103, 31203-31216, 1998. (Pubitemid 128665498)
54. Pozzer, A., Jöckel, P., Sander, R., Williams, J., Ganzeveld, L., and Lelieveld, J.: Technical Note: The MESSy-submodel AIRSEA calculating the air-sea exchange of chemical species, Atmos. Chem. Phys., 6, 5435-5444, doi:10.5194/acp-6-5435-2006, 2006.
55. Pozzer, A., Jöckel, P., Tost, H., Sander, R., Ganzeveld, L., Kerkweg, A., and Lelieveld, J.: Simulating organic species with the global atmospheric chemistry general circulation model ECHAM5/MESSy1: a comparison of model results with observations, Atmos. Chem. Phys., 7, 2527-2550, doi:10.5194/acp-7-2527-2007, 2007.
56. Pozzer, A., Jöckel, P., Kern, B., and Haak, H.: The Atmosphere-Ocean General Circulation Model EMAC-MPIOM, to be submitted to Geosci. Model Dev. Discuss., 2011.
57. Preiss, N. and Genthon, C.: Use of a new database of lead 210 for global aerosol model validation, J. Geophys. Res., 102, 25347-25357, 1997.
58. Preiss, N., Mélières, M.-A., and Pourchet, M.: A compilation of data on lead 210 concentration in surface air and fluxes at the air-surface and water-sediment interfaces, J. Geophys. Res., 101, 28847-28862, 1996.
59. Pressyanov, D. S.: Short solution of the radioactive decay chain equations, Am. J. Phys., 70, 444-445, 2002.
60. Price, C. and Rind, D.: A simple Lightning Parametrization for Calculating Global Lightning Distributions, J. Geophys. Res., 97, 9919-9933, 1992.
61. Price, C. and Rind, D.: Modeling Global Lightning Distributions in a General Circulation Model, Mon. Weather Rev., 122, 1930-1939, 1994.
62. Pringle, K. J., Tost, H., Message, S., Steil, B., Giannadaki, D., Nenes, A., Fountoukis, C., Stier, P., Vignati, E., and Lelieveld, J.: Description and evaluation of GMXe: a new aerosol submodel for global simulations (v1), Geosci. Model Dev., 3, 391-412, doi:10.5194/gmd-3-391-2010, 2010.
63. Randerson, J. T., van der Werf, G. R., Giglio, L., Collatz, G. J., and Kasibhatla, P. S.: Global Fire Emissions Database, Version 2 (GFEDv2.1), Tech. rep., Oak Ridge National Laboratory Distributed Active Archive Center, Oak Ridge, Tennessee, USA, doi:10.3334/ORNLDAAC/849, http://daac.ornl.gov/, 2007.
64. 90Sr, J. Geophys. Res., 100, 26141-26161, 1995.
65. 17O isotopic variations to provide insights into the high northern latitude surface CO inventory, Atmos. Chem. Phys., 2, 147-159, doi:10.5194/acp-2-147-2002, 2002.
66. Roeckner, E., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kornblueh, L., Manzini, E., Schlese, U., and Schulzweida, U.: Sensitivity of simulated climate to horizontal and vertical resolution in the ECHAM5 atmosphere model, J. Climate, 19, 3771-3791, 2006.
67. Sander, R., Kerkweg, A., Jockel, P., and Lelieveld, J.: Technical note: The new comprehensive atmospheric chemistry module MECCA, Atmos. Chem. Phys., 5, 445-450, doi:10.5194/acp-5-445-2005, 2005.
68. Sander, S. P., Friedl, R. R., Golden, D. M., Kurylo, M. J., Moortgat, G. K., Keller-Rudek, H., Wine, P. H., Ravishankara, A. R., Kolb, C. E., Molina, M. J., Finlayson-Pitts, B. I., Huie, R. E., and Orkin, V. L.: Chemical Kinetics and Photochemical Data for Use in Atmospheric Studies, Evaluation Number 15, JPL Publication 06-2, Jet Propulsion Laboratory, Pasadena, CA, 2006.
69. Sander, R., Baumgaertner, A., Gromov, S., Harder, H., Jockel, P., Kerkweg, A., Kubistin, D., Regelin, E., Riede, H., Sandu, A., Taraborrelli, D., Tost, H., and Xie, Z.-Q.: The atmospheric chemistry box model CAABA/MECCA-3.0, to be submitted to Geosci. Model Dev. Discuss., 2011.
70. Sandu, A. and Sander, R.: Technical note: Simulating chemical systems in Fortran90 and Matlab with the Kinetic Preprocessor KPP-2.1, Atmos. Chem. Phys., 6, 187-195, doi:10.5194/acp-6-187-2006, 2006.
71. Schery, S. D. and Wasiolek, M. A.: Modeling radon flux from the earth's surface, in: Radon and Thoron in the Human Environment, Proceedings of the 7 th Tohwa University International Symposium, edited by: Katase, A. and Shimo, M., World Scientific, Singapore, 1998.
72. Schumann, U. and Huntrieser, H.: The global lightning-induced nitrogen oxides source, Atmos. Chem. Phys., 7, 3823-3907, doi:10.5194/acp-7-3823-2007, 2007.
73. Seigneur, C. and Lohman, K.: Effect of bromine chemistry on the atmospheric mercury cycle, J. Geophys. Res., 113 D, D23309, doi:10.1029/ 2008JD010262, 2008.
74. Selin, N. E., Jacob, D. J., Yantosca, R. M., Strode, S., Jaegle, L., and Sunderland, E. M.: Global 3-D land-ocean-atmosphere model for mercury: Present-day versus preindustrial cycles and anthropogenic enrichment factors for deposition, Glob. Biogeochem. Cy., 22, GB2011, doi:10.1029/2007GB003040, 2008.
75. Tost, H.: Global Modelling of Cloud, Convection and Precipitation Influences on Trace Gases and Aerosols, Ph. D. thesis, University of Bonn, Germany, http://hss.ulb.uni-bonn. de/diss-online/math-nat-fak/2006/tost-holger), 2006.
76. Tost, H., Jockel, P., Kerkweg, A., Sander, R., and Lelieveld, J.: Technical note: A new comprehensive SCAVenging submodel for global atmospheric chemistry modelling, Atmos. Chem. Phys., 6, 565-574, doi:10.5194/acp-6-565-2006, 2006a.
77. Tost, H., Jockel, P., and Lelieveld, J.: Influence of different convection parameterisations in a GCM, Atmos. Chem. Phys., 6, 5475-5493, doi:10.5194/acp-6-5475-2006, 2006b.
78. Tost, H., Jöckel, P., and Lelieveld, J.: Lightning and convection parameterisations - uncertainties in global modelling, Atmos. Chem. Phys., 7, 4553-4568, doi: 10.5194/acp-7-4553-2007, 2007. (Pubitemid 47373629)
79. Usoskin, I. G., Alanko-Huotari, K., Kovaltsov, G. A., and Mursula, K.: Heliospheric modulation of cosmic rays: Monthly reconstruction for 1951-2004, J. Geophys. Res., 110, A12108, doi: 10.1029/2005JA011250, 2005. (Pubitemid 44971467)
80. van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Kasibhatla, P. S., and Arellano Jr., A. F.: Interannual variability in global biomass burning emissions from 1997 to 2004, Atmos. Chem. Phys., 6, 3423-3441, doi: 10.5194/acp-6-3423-2006, 2006. (Pubitemid 44272961)
81. Vignati, E., Wilson, J., and Stier, P.: M7: An efficient size-resolved aerosol microphysics module for large-scale aerosol transport models, J. Geophys. Res., 109, D22202, doi:10.1029/2003JD004485, 2004. (Pubitemid 40294868)
82. Xie, Z.-Q., Sander, R., Poschl, U., and Slemr, F.: Simulation of atmospheric mercury depletion events (AMDEs) during polar springtime using the MECCA box model, Atmos. Chem. Phys., 8, 7165-7180, doi: 10.5194/acp-8-7165-2008, 2008.
83. Zhang, K., Wan, H., Zhang, M., and Wang, B.: Evaluation of the atmospheric transport in a GCM using radon measurements: sensitivity to cumulus convection parameterization, Atmos. Chem. Phys., 8, 2811-2832, doi: 10.5194/acp-8-2811-2008, 2008.