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Volumn 64, Issue 3, 2001, Pages

Laser-induced electronic desorption from InP surfaces studied by femtosecond nonresonant ionization spectroscopy

Author keywords

[No Author keywords available]

Indexed keywords

INDIUM; PHOSPHORUS;

EID: 4244136909     PISSN: 10980121     EISSN: 1550235X     Source Type: Journal    
DOI: 10.1103/PhysRevB.64.035414     Document Type: Article
Times cited : (18)

References (30)
  • 1
    • 85038341008 scopus 로고    scopus 로고
    • M. Von Allmen, (Springer, Berlin, 1995)
    • M. Von Allmen, Laser-Beam Interaction with Materials; Principles and Applications (Springer, Berlin, 1995).
  • 14
    • 0004067140 scopus 로고
    • N. H. Tolk, M. M. Traum, J. C. Tully, T. E. Madey, Springer, Berlin, edited by, and
    • Desorption Induced by Electronic Transitions I, edited by N. H. Tolk, M. M. Traum, J. C. Tully, and T. E. Madey (Springer, Berlin, 1983).
    • (1983) Desorption Induced by Electronic Transitions I
  • 21
    • 85038266987 scopus 로고    scopus 로고
    • For evaluating ρ, we introduce a mean velocity (formula presented) and a width W (formula presented) for a rectangular form of velocity distribution of desorbed neutrals. At a time delay, neutral species with a velocity (formula presented) arrive at the center of the ionization volume which is separated from the surface by the distance, formula presented) Because of the finite size of the ionization volume, which is characterized by the diameter, of the volume, neutral species with velocities (formula presented) are present in the ionization volume at the delay time. For the time delay (formula presented) when the central part of the velocity distribution arrives at the center of the volume, (formula presented) is given by (formula presented) where (formula presented) Since (formula presented) the fraction can be evaluated as (formula presented) Under the present experimental condition that (formula presented) and (formula presented) we can estimate that (formula presented)
    • For evaluating ρ, we introduce a mean velocity (formula presented) and a width W (formula presented) for a rectangular form of velocity distribution of desorbed neutrals. At a time delay t, neutral species with a velocity (formula presented) arrive at the center of the ionization volume which is separated from the surface by the distance L: (formula presented) Because of the finite size of the ionization volume, which is characterized by the diameter d of the volume, neutral species with velocities (formula presented) are present in the ionization volume at the delay time. For the time delay (formula presented) when the central part of the velocity distribution arrives at the center of the volume, (formula presented) is given by (formula presented) where (formula presented) Since (formula presented) the fraction can be evaluated as (formula presented) Under the present experimental condition that (formula presented) and (formula presented) we can estimate that (formula presented)
  • 24
    • 85038333784 scopus 로고    scopus 로고
    • As shown by the analysis of the results in Fig. 55, the effective excitation cross section (formula presented) is not dependent on the excitation laser intensity φ. If the nonlinear decay process of the excited state is significant, then we have solutions of (formula presented) which is nonlinearly dependent on φ. In such a case, we have fluence-dependent (formula presented), which is not consistent with the results. Therefore, the first-order decay should be assumed to be much larger than the nonlinear decay of the excited species. This is not at all contradictory to the idea of two-hole localization, since two-hole localization is assumed to take place successively, not simultaneously. The successive capture of the second hole by the first-hole localized site can be treated in the frame of monomolecular decay of the excited species (Ref
    • As shown by the analysis of the results in Fig. 55, the effective excitation cross section (formula presented) is not dependent on the excitation laser intensity φ. If the nonlinear decay process of the excited state is significant, then we have solutions of (formula presented) which is nonlinearly dependent on φ. In such a case, we have fluence-dependent (formula presented), which is not consistent with the results. Therefore, the first-order decay should be assumed to be much larger than the nonlinear decay of the excited species. This is not at all contradictory to the idea of two-hole localization, since two-hole localization is assumed to take place successively, not simultaneously. The successive capture of the second hole by the first-hole localized site can be treated in the frame of monomolecular decay of the excited species (Ref. 22).


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