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This statement is consistently corroborated by a number of observations and reasonings: (i) We observe identical spectral shape and similar emission energy for the Ag+-bound 1 and parent complex 3, ii) 3-MLCT emissions are known for their broad and featureless spectrum, iii) While 1 shows a temperature-independent emission wavelength, the silver-loaded complex displays a strong temperature dependence see Supporting Information Figures S12 and S13, Apparently, larger loadings of metal ions change the character of the emission of 1 from 3LC to 3MLCT because ligand 7 becomes increasingly a better acceptor
-
3MLCT because ligand 7 becomes increasingly a better acceptor.
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59
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35848931321
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Association constants were obtained using the computer program SPECFIT, Global Analysis system, Version 3.0.32
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(a) Association constants were obtained using the computer program SPECFIT, Global Analysis system, Version 3.0.32.
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2+) on one molecule of 1.
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2+) on one molecule of 1.
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