Budget of tropospheric ozone during TOPSE from two chemical transport models

Journal of Geophysical Research: Atmospheres

Volumn 108, Issue 8, 2003, Pages

  Emmons, L K ^a   Hess, P ^a   Klonecki, A ^a   Tie, X ^a   Horowitz, L ^b   Lamarque, J F ^a   Kinnison, D ^a   Brasseur, G ^c   Atlas, E ^a   Browell, E ^d   Cantrell, C ^a   Eisele, F ^a   Mauldin, R L ^a   Merrill, J ^e   Ridley, B ^a   Shetter, R ^a  

^a NATIONAL CENTER FOR ATMOSPHERIC RESEARCH   (United States)

^b PRINCETON UNIVERSITY   (United States)

^c MAX PLANCK INSTITUTE FOR METEOROLOGY   (Germany)

^d NASA LANGLEY RESEARCH CENTER   (United States)

^e UNIVERSITY OF RHODE ISLAND   (United States)

Author keywords

Chemical transport model; Ozone budget; Stratosphere troposphere exchange; TOPSE; Tropospheric ozone

Indexed keywords

ATMOSPHERIC CHEMISTRY; ATMOSPHERIC TRANSPORT; NUMERICAL MODEL; OZONE; STRATOSPHERE-TROPOSPHERE INTERACTION; TROPOSPHERE;

EID: 20244387808     PISSN: 01480227     EISSN: None     Source Type: Journal    
DOI: 10.1029/2002jd002665     Document Type: Article

References (52)

1. 3 with water-ice surfaces at temperatures of the free troposphere, Geophys. Res. Lett., 24, 1479-1482, 1997.
2. Appenzeller, C., J. R. Holton, and K. H. Rosenlof, Seasonal variation of mass transport across the tropopause, J. Geophys. Res., 101, 15,071-15,078, 1996.
3. Atlas, E. L., B. A. Ridley, and C. Cantrell, The Tropospheric Ozone Production about the Spring Equinox (TOPSE) Experiment: Introduction, J. Geophys. Res., 108(D4), 8353, doi:10.1029/2002JD003172, 2003.
4. Barth, M. C., P. J. Rasch, J. T. Kiehl, C. M. Benkovitz, and S. E. Schwartz, Sulfur chemistry in the National Center for Atmospheric Research Community Climate Model: Description, evaluation, features, and sensitivity to aqueous chemistry, J. Geophys. Res., 105, 1387-1416, 2000.
5. Brasseur, G. P., D. A. Hauglustaine, S. Walters, P. J. Rasch, J.-F. Müller, C. Granier, and X.-X. Tie, MOZART: A global chemical transport model for ozone and related chemical tracers, part 1: Model description, J. Geophys. Res., 103, 28,265-28,289, 1998.
6. Brasseur, G. P., J. J. Orlando, and G. S. Tyndall, Atmospheric Chemistry and Global Change, Oxford Univ. Press, New York, 1999.
7. Browell, E. V., et al., Ozone, aerosol, potential vorticity, and trace gas trends observed at high-latitudes over North America from February to May 2000, J. Geophys. Res., 108(D4), 8369, doi:10.1029/2001JD001390, 2003
8. Cantrell, C. A., et al., Steady state free radical budgets and ozone photochemistry during TOPSE, J. Geophys. Res., 108(D4), 8361, doi:10.1029/2002JD002198, 2003.
9. European Centre for Medium-Range Weather Forecasting (ECMWF), The description of the ECMWF/WCRP Level III-A Global Atmospheric Data Archive, Reading, UK, 1995.
10. Giorgi, F., and W. L. Chameides, The rainout parameterization in a photochemical model, J., Geophys. Res., 90, 7872-7880, 1985.
11. Grell, G. A., J. Dudhia, and D. R. Stauffer, A description of the fifth generation Penn State/NCAR Mesoscale Model (MM5), NCAR/TN398+IA, Natl. Cent. for Atmos. Res., Boulder, Colo., 116 pp., 1993.
12. 5 on submicron sulfuric acid aerosols, J. Phys. Chem. A, 104, 3984-3990, 2000.
13. Hauglustaine, D. A., G. P. Brasseur, S. Walters, P. J. Rasch, J.-F. Müller, L. K. Emmons, and M. A. Carroll, MOZART: A global chemical transport model for ozone and related chemical tracers, part 2: Model results and evaluation, J. Geophys. Res., 103, 28,291-28,335, 1998.
14. Hess, P. G., Model and measurement analysis of springtime transport and chemistry of the Pacific basin, J. Geophys. Res., 106, 12,689-12,717, 2001.
15. Hess, P. G., S. Flocke, J.-F. Lamarque, M. C. Barth, and S. Madronich, Episodic modeling of the chemical structure of the troposphere as revealed during the spring MLOPEX 2 intensive, J. Geophys. Res., 105, 26,809-26,840, 2000.
16. Holton, J. R., P. H. Haynes, M. E. McIntyre, A. R. Douglas, R. B. Rood, and L. Pfister, Stratosphere-troposphere exchange, Rev. Geophys, 33, 403-439, 1995.
17. Jöckel, P., R. von Kuhlmann, M. Lawrence, B. Steil, C. Brenninkmeijer, P. Crutzen, P. Rasch, and B. Eaton, On a fundamental problem in implementing flux-form advection schemes for tracer transport in 3-dimensional general circulation and chemical tracer models, Q. J. R. Meteorol. Soc., 127, 1035-1052, 2001.
18. Johnston, H., and D. Kinnison, Methane photooxidation in the atmosphere: Contrast between two methods of analysis, J. Geophys. Res., 103, 21,967-21,984, 1998.
19. Kiehl, J. T., T. L. Schneider, P. J. Rasch, and M. C. Barth, J. Geophys. Res., 105, 1441-1457, 2000.
20. Klonecki, A., Model study of the tropospheric chemistry of ozone, Ph.D. thesis, Princeton Univ., Princeton, N. J., 1999.
21. Klonecki, A., P. Hess, L. Emmons, L. Smith, J. Orlando, and D. Blake, Seasonal changes in the transport of pollutants into the Arctic troposphere-model study, J. Geophys. Res., 108(D4), 8367, doi:10.1029/2002JD002199, 2003.
22. Lamarque, J.-F., and P. G. Hess, Cross-tropopause mass exchange and potential vorticity budget in a simulated tropopause folding, J. Atmos. Sci., 51, 2246-2269, 1994.
23. Lamarque, J.-F., and P. G. Hess, Model analysis of the temporal and geographical origin of the CO distribution during the TOPSE campaign, J. Geophys. Res., 108(D4), 8354, doi:10.1029/2002JD002077, 2003.
24. Lamarque, J.-F., P. G. Hess, and X. X. Tie, Three-dimensional model study of the influence of stratosphere-troposphere exchange and its distribution on tropospheric chemistry, J. Geophys. Res., 104, 26,363-26,372, 1999.
25. Logan, J., An analysis of ozonesonde data for the troposphere: Recommendations for testing 3-D models and development of a gridded climatology for tropospheric ozone, J. Geophys. Res., 104, 16,115-16,149, 1999.
26. Mauldin, R. L., III, C. A. Cantrell, M. A. Zondlo, E. Kosciuch, B. A. Ridley, R. Weber, and F. E. Eisele, Measurements of OH, H2SO4, and MSA during Tropospheric Ozone Production About the Spring Equinox (TOPSE), J. Geophys. Res., 108(D4), 8366, doi:10.1029/2002JD002295, 2003.
27. McLinden, C. A., S. C. Olsen, B. Hannegan, O. Wild, M. J. Prather, and J. Sundet, Stratospheric ozone in 3-D models: A simple chemistry and the cross-tropopause flux, J. Geophys. Res., 105, 14,653-14,665, 2000.
28. Müller, J.-F., Geographical distribution and seasonal variation of surface emissions and deposition velocities of atmospheric trace gases, J. Geophys. Res., 97, 3787-3804, 1992.
29. Müller, J.-F., and G. Brasseur, IMAGES: A three-dimensional chemical transport model of the global troposphere, J. Geophys. Res., 100, 16,445-16,490, 1995.
30. Olivier, J. G. J., A. F. Bouwman, C. W. M. van der Mass, J. J. M. Berdowski, C. Veldt, J. P. J. Bloos, A. J. H. Visschedijk, P. Y. J. Zandveld, and J. L. Haverlag, Description of EDGAR version 2.0: A set of global emission inventories of greenhouse gases and ozone-depleting substances for all anthropogenic and most natural sources on a per country basis and on a 1 × 1 degree grid, RIVM Rep. 771060 002, TNO-MEP Rep. R96/119, Natl. Inst. of Public Health and the Environ., Bilthoven, Netherlands, 1996.
31. Oltmans, S., and H. Levy II, Surface ozone measurements from a global network, Atmos. Environ., 23, 9-24, 1994.
32. Penkett, S. A., and K. A. Brice, The spring maximum in photochemical oxidants in the Northern Hemisphere, Nature, 319, 655-657, 1986.
33. Pickering, K. E., Y. Wang, W.-K. Tao, C. Price, and J.-F. Muller, Vertical distributions of lightning NOx for use in regional and global chemical transport models, J. Geophys. Res., 103, 31,203-31,216, 1998.
34. Prather, M., et al., Atmospheric chemistry and greenhouse gases, in Climate Change 2001: The Scientific Basis, Contribution of Working Group I to the Third Assessment Report of the Intergovernmental Panel on Climate Change, edited by J. T. Houghton et al., 881 pp., Cambridge Univ. Press, New York, 2001.
35. Price, C., and D. Rind, A simple lightning parameterization for calculating global lightning distributions, J. Geophys. Res., 97, 9919-9933, 1992.
36. x from lightning, 1, Global distribution based on lightning physics, J. Geophys. Res., 102, 5929-5941, 1997.
37. Randel, W. J., F. Wu, J. M. Russell III, A. Roche, and J. Waters, Seasonal cycles and QBO variations in stratospheric CH4 and H2O observed in UARS HALOE data., J. Atmos. Sci., 55, 163-185, 1998.
38. Rasch, P. J., M. C. Barth, J. T. Kiehl, S. E. Schwartz, and C. M. Benkovitz, A description of the global sulfur cycle and its controlling processes in the National Center for Atmospheric Research Community Climate Model, version 3, J. Geophys. Res., 105, 1367-1386, 2000.
39. Richard, E. C., et al., Severe chemical ozone loss inside the Arctic polar vortex during winter 1999-2000 inferred from in situ airborne measurements, Geophys. Res. Lett., 28, 2197-2200, 2001.
40. Ridley, B. A., et al., Ozone depletion events observed in the high latitude surface layer during the TOPSE aircraft program, J. Geophys. Res., 108(D4), 8356, doi:10.1029/2001JD001507, 2003.
41. 3 levels, Tellus, Ser. B, 49, 38-55, 1997.
42. Shetter, R. E., and M. Müller, Photolysis frequency measurements on the NASA DC-8 during the PEM-Tropics Mission using actinic flux spectroradiometry: Instrument description and results, J. Geophys. Res., 104, 5647-5661, 1999.
43. Shetter, R. E., L. Cinquini, B. L. Lefer, S. R. Hall, and S. Madronich, Comparison of airborne measured and calculated spectral actinic flux and derived photolysis frequencies during the PEM Tropics B mission, J. Geophys. Res., 107, 8234, doi:10.1029/2001JD001320, 2002 [printed 108(D2), 2003].
44. Sinnhuber, B.-M., et al., Large loss of total ozone during the Arctic winter of 1999/2000, Geophys. Res. Lett., 27, 3473-3476, 2000.
45. Simmonds, P. G., S. Seuring, G. Nickless, and R. G. Derwent, Segregation and interpolation of ozone and carbon monoxide measurements by air mass origin at the TOR station Mace Head, Ireland from 1987-1995, J. Atmos. Chem., 28, 45-59, 1997.
46. Thompson, A. M., M. A. Huntley, and R. W. Stewart, Perturbations to tropospheric oxidants, 1985-2035, 1: Calculations of ozone and OH in chemically coherent regions, J. Geophys. Res., 95, 9829-9844, 1990.
47. Tie, X., G. Brasseur, L. Emmons, L. Horowitz, and D. Kinnison, Effects of aerosols on tropospheric oxidants: A global model study, J. Geophys. Res., 106, 22,931-22,964, 2001.
48. Tie, X., et al., Effects of sulfate aerosol on tropospheric NOx and ozone budgets: Model simulations and TOPSE evidence, J. Geophys. Res., 108(D4), 8364, doi:10.1029/2001JD001508, 2003.
49. x -hydrocarbon chemistry, 3, Origin of tropospheric ozone and effects of nonmethane hydrocarbons, J. Geophys. Res., 103, 10,757-10,767, 1998.
50. Wang, Y., et al., Springtime photochemistry at northern mid and high latitudes, J. Geophys. Res., 108(D4), 8358, doi:10.1029/2002JD002227, 2003.
51. Wesely, M. L., Parameterization of surface resistances to gaseous dry deposition in regional-scale numerical models, Atmos. Environ., 23, 1293-1304, 1989.
52. Yienger, J. J., A. A. Klonecki, H. Levy H, W. J. Moxim, and G.R. Carmichael, An evaluation of chemistry's role in the winter-spring ozone maximum found in the northern midlatitude free troposphere, J. Geophys. Res., 104, 3655-3667, 1999.