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33645939441
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The optimized C-S-S-C dihedral angles for the cyclic disulfides and the maximum distance spanned by the sulfur atoms of the chelating dithiol were determined by molecular modeling using PC Model V 5.0: Serena Software, Bloomington, IN
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The optimized C-S-S-C dihedral angles for the cyclic disulfides and the maximum distance spanned by the sulfur atoms of the chelating dithiol were determined by molecular modeling using PC Model V 5.0: Serena Software, Bloomington, IN.
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35
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84990149346
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85087999532
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cH2; values were checked on several different slides for immersion times ≥1 h. All measurements consistently showed higher crystallinities for the SAMs absorbed from ethanol, thereby excluding influence from instrumental error.
-
cH2; values were checked on several different slides for immersion times ≥1 h. All measurements consistently showed higher crystallinities for the SAMs absorbed from ethanol, thereby excluding influence from instrumental error.
-
-
-
-
47
-
-
33645917262
-
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For example, it is possible that, relative to isooctane, ethanol destabilizes the physisorbed state (vide infra). In this scenario, alkanethiols might chemisorb directly (and thus rapidly) from ethanol without requiring the intermediacy of a physisorption preequilibrium.
-
For example, it is possible that, relative to isooctane, ethanol destabilizes the physisorbed state (vide infra). In this scenario, alkanethiols might chemisorb directly (and thus rapidly) from ethanol without requiring the intermediacy of a physisorption preequilibrium.
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48
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53
-
-
33645915968
-
-
note
-
Although data from the coadsorption of d-C17 and n-C17 might offer further insight to these discussions, the indistinguishable thicknesses, wettabilities, and IR spectra of the SAMs derived from these two adsorbates presently precludes this type of study.
-
-
-
-
55
-
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33645947539
-
-
In coadsorption studies involving m-C17 and d-C17, it is possible that H1-C17 adsorbs preferentially as a kinetically trapped species. The exchange experiments involving preformed SAMs and free thiols in solution (see ref 52), however, argue against this hypothesis.
-
In coadsorption studies involving m-C17 and d-C17, it is possible that H1-C17 adsorbs preferentially as a kinetically trapped species. The exchange experiments involving preformed SAMs and free thiols in solution (see ref 52), however, argue against this hypothesis.
-
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56
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0032166150
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Fenter, P.; Schreiber, F.; Herman, L.; Scoles, G.; Eisenberger, P.; Bedzyk, M. J. Surf. Sci. 1998, 412/413, 213.
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Fenter, P.1
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Bedzyk, M.J.6
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57
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33645928481
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note
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57
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59
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33645905951
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Syracuse University, Syracuse, NY. Personal communication
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Lees, W. J. Syracuse University, Syracuse, NY. Personal communication.
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Lees, W.J.1
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