Secondary organic aerosol formation from in-use motor vehicle emissions using a potential aerosol mass reactor

Environmental Science and Technology

Volumn 48, Issue 19, 2014, Pages 11235-11242

  Tkacik, Daniel S ^a,b   Lambe, Andrew T ^c   Jathar, Shantanu ^d   Li, Xiang ^a,b   Presto, Albert A ^a,b   Zhao, Yunliang ^a,b   Blake, Donald ^e   Meinardi, Simone ^e   Jayne, John T ^c   Croteau, Philip L ^c   Robinson, Allen L ^a,b  

^a CARNEGIE MELLON UNIVERSITY   (United States)

^b CARNEGIE MELLON UNIVERSITY   (United States)

^c AERODYNE RESEARCH INC   (United States)

^d University of California Davis   (United States)

^e UNIVERSITY OF CALIFORNIA   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ATMOSPHERIC CHEMISTRY; EXPERIMENTS; FLEET OPERATIONS; HYDROCARBON REFINING; MASS SPECTROMETRY; MOBILE POWER PLANTS; OXIDATION; VEHICLES;

AMBIENT PARTICULATE MATTER; ATMOSPHERIC OXIDATION; LIGHT-DUTY GASOLINE VEHICLES; MOTOR VEHICLE EMISSIONS; NATIONAL EMISSIONS INVENTORIES; PARTICULATE MATTER EMISSIONS; SECONDARY ORGANIC AEROSOLS; UNRESOLVED COMPLEX MIXTURES;

AEROSOLS;

AMMONIUM NITRATE; FUEL; GASOLINE; HYDROCARBON; HYDROXYL RADICAL; AEROSOL; AIR POLLUTANT; EXHAUST GAS; NITRIC ACID DERIVATIVE; ORGANIC COMPOUND; PARTICULATE MATTER; VOLATILE ORGANIC COMPOUND;

AEROSOL; ATMOSPHERIC POLLUTION; BIOREACTOR; CONCENTRATION (COMPOSITION); EMISSION INVENTORY; EXHAUST EMISSION; FRAGMENTATION; FUEL CONSUMPTION; NITRATE; NUMERICAL MODEL; OXIDATION; PARTICULATE MATTER; VOLATILE SUBSTANCE;

AIR POLLUTION; ARTICLE; ATMOSPHERE; FRAGMENTATION REACTION; MASS SPECTROMETRY; MOTOR VEHICLE; OXIDATION; PARTICULATE MATTER; PHOTOOXIDATION; POTENTIAL AEROSOL MASS FLOW REACTOR; REACTION ANALYSIS; REACTOR; SECONDARY ORGANIC AEROSOL; URBAN AREA; AEROSOL; AIR POLLUTANT; ANALYSIS; CHEMISTRY; CITY; EXHAUST GAS; OXIDATION REDUCTION REACTION; UNITED STATES;

PENNSYLVANIA; PITTSBURGH; UNITED STATES;

AEROSOLS; AIR POLLUTANTS; ATMOSPHERE; CITIES; GASOLINE; HYDROXYL RADICAL; NITRATES; ORGANIC CHEMICALS; OXIDATION-REDUCTION; PARTICULATE MATTER; PENNSYLVANIA; UNITED STATES; VEHICLE EMISSIONS; VOLATILE ORGANIC COMPOUNDS;

EID: 84907935298     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es502239v     Document Type: Article

References (53)

1. Fine, P. M.; Shen, S.; Sioutas, C. Inferring the sources of fine and ultrafine particulate matter at downwind receptor sites in the Los Angeles basin using multiple continuous measurements. Special issue of Aerosol Science and Technology on findings from the fine particulate matter supersites program Aerosol Sci. Technol. 2004, 38, 182-195
2. Zhang, Q.; Stanier, C. O.; Canagaratna, M. R.; Jayne, J. T.; Worsnop, D. R.; Pandis, S. N.; Jimenez, J. L. Insights into the chemistry of new particle formation and growth events in Pittsburgh based on aerosol mass spectrometry Environ. Sci. Technol. 2004, 38, 4797-4809
3. Twomey, S. Pollution and the planetary albedo Atmos. Environ. 1974, 8, 1251-1256
4. Dockery, D. W.; Pope, C. A., III Health effects of fine particulate air pollution: Lines that connect J. Air Waste Manage. Assoc. 2006, 56, 709+
5. Gordon, T. D.; Presto, A. A.; May, A. A.; Nguyen, N. T.; Lipsky, E. M.; Donahue, N. M.; Gutierrez, A.; Zhang, M.; Maddox, C.; Rieger, P. Secondary organic aerosol formation exceeds primary particulate matter emissions for light-duty gasoline vehicles Atmos. Chem. Phys. Discuss. 2013, 13, 23173-23216
6. Nordin, E. Z.; Eriksson, A. C.; Roldin, P.; Nilsson, P. T.; Carlsson, J. E.; Kajos, M. K.; Hellén, H.; Wittbom, C.; Rissler, J.; Löndahl, J. Secondary organic aerosol formation from idling gasoline passenger vehicle emissions investigated in a smog chamber Atmos. Chem. Phys. 2013, 13, 6101-6116
7. Platt, S. M.; El Haddad, I.; Zardini, A. A.; Clairotte, M.; Astorga, C.; Wolf, R.; Slowik, J. G.; Temime-Roussel, B.; Marchand, N.; Ježek, I. Secondary organic aerosol formation from gasoline vehicle emissions in a new mobile environmental reaction chamber Atmos. Chem. Phys. 2013, 13, 9141-9158
8. Chirico, R.; DeCarlo, P. F.; Heringa, M. F.; Tritscher, T.; Richter, R.; Prévôt, A. S. H.; Dommen, J.; Weingartner, E.; Wehrle, G.; Gysel, M. Impact of aftertreatment devices on primary emissions and secondary organic aerosol formation potential from in-use diesel vehicles: Results from smog chamber experiments Atmos. Chem. Phys. 2010, 10, 11545-11563
9. Volkamer, R.; Jimenez, J. L.; San Martini, F.; Dzepina, K.; Zhang, Q.; Salcedo, D.; Molina, L. T.; Worsnop, D. R.; Molina, M. J. Secondary organic aerosol formation from anthropogenic air pollution: Rapid and higher than expected Geophys. Res. Lett. 2006, 33, L17811
10. De Gouw, J. A.; Brock, C. A.; Atlas, E. L.; Bates, T. S.; Fehsenfeld, F. C.; Goldan, P. D.; Holloway, J. S.; Kuster, W. C.; Lerner, B. M.; Matthew, B. M. Sources of particulate matter in the northeastern United States in summer: 1. Direct emissions and secondary formation of organic matter in urban plumes J. Geophys. Res. Atmos. 2008, 113, D08301
11. De Gouw, J.; Jimenez, J. L. Organic aerosols in the earth's atmosphere Environ. Sci. Technol. 2009, 43, 7614-7618
12. Jimenez, J. L.; Canagaratna, M. R.; Donahue, N. M.; Prevot, A. S. H.; Zhang, Q.; Kroll, J. H.; DeCarlo, P. F.; Allan, J. D.; Coe, H.; Ng, N. L. Evolution of organic aerosols in the atmosphere Science 2009, 326, 1525-1529
13. Heringa, M. F.; DeCarlo, P. F.; Chirico, R.; Tritscher, T.; Dommen, J.; Weingartner, E.; Richter, R.; Wehrle, G.; Prévôt, A. S. H.; Baltensperger, U. Investigations of primary and secondary particulate matter of different wood combustion appliances with a high-resolution time-of-flight aerosol mass spectrometer Atmos. Chem. Phys. 2011, 11, 5945-5957
14. Heringa, M. F.; DeCarlo, P. F.; Chirico, R.; Tritscher, T.; Clairotte, M.; Mohr, C.; Crippa, M.; Slowik, J. G.; Pfaffenberger, L.; Dommen, J. A new method to discriminate secondary organic aerosols from different sources using high-resolution aerosol mass spectra Atmos. Chem. Phys. 2012, 12, 2189-2203
15. Gordon, T. D..; Tkacik, D. S..; Presto, A. A..; Zhang, M..; Jathar, S. H..; Nguyen, N. T..; Massetti, J..; Truong, T..; Cicero-Fernandez, P..; Maddox, C.. Primary gas- and particle-phase emissions and secondary organic aerosol production from gasoline and diesel off-road engines Environ. Sci. Technol. 2013, 47, 14137-14146
16. Lambe, A. T.; Onasch, T. B.; Croasdale, D. R.; Wright, J. P.; Martin, A. T.; Franklin, J. P.; Massoli, P.; Kroll, J. H.; Canagaratna, M. R.; Brune, W. H. Transitions from functionalization to fragmentation reactions of laboratory secondary organic aerosol (SOA) generated from the OH oxidation of alkane precursors Environ. Sci. Technol. 2012, 46, 5430-5437
17. Fraser, M. P.; Cass, G. R. Detection of excess ammonia emissions from in-use vehicles and the implications for fine particle control Environ. Sci. Technol. 1998, 32, 1053-1057
18. Grieshop, A. P.; Lipsky, E. M.; Pekney, N. J.; Takahama, S.; Robinson, A. L. Fine particle emission factors from vehicles in a highway tunnel: Effects of fleet composition and season Atmos. Environ. 2006, 40 (Supple) 287-298
19. Chirico, R.; Prevot, A. S. H.; DeCarlo, P. F.; Heringa, M. F.; Richter, R.; Weingartner, E.; Baltensperger, U. Aerosol and trace gas vehicle emission factors measured in a tunnel using an aerosol mass spectrometer and other on-line instrumentation Atmos. Environ. 2011, 45, 2182-2192
20. Kang, E.; Root, M. J.; Toohey, D. W.; Brune, W. H. Introducing the concept of potential aerosol mass (PAM) Atmos. Chem. Phys. 2007, 7, 5727-5744
21. EIA. Residential Transportation Energy Consumption Survey; U.S. Energy Information Administration, 1994.
22. Schauer, J. J.; Kleeman, M. J.; Cass, G. R.; Simoneit, B. R. T. Measurement of emissions from air pollution sources. 5. C1-C32 organic compounds from gasoline-powered motor vehicles Environ. Sci. Technol. 2002, 36, 1169-1180
23. Loza, C. L.; Craven, J. S.; Yee, L. D.; Coggon, M. M.; Schwantes, R. H.; Shiraiwa, M.; Zhang, X.; Schilling, K. A.; Ng, N. L.; Canagaratna, M. R. Secondary organic aerosol yields of 12-carbon alkanes Atmos. Chem. Phys. 2014, 14, 1423-1439
24. 2 radical concentrations during the winter and summer of 2004 J. Geophys. Res., Atmos. 2007, 112, D21312
25. Ng, N. L.; Herndon, S. C.; Trimborn, A.; Canagaratna, M. R.; Croteau, P. L.; Onasch, T. B.; Sueper, D.; Worsnop, D. R.; Zhang, Q.; Sun, Y. L. An aerosol chemical speciation monitor (ACSM) for routine monitoring of the composition and mass concentrations of ambient aerosol Aerosol Sci. Technol. 2011, 45, 780-794
26. Docherty, K. S.; Jaoui, M.; Corse, E.; Jimenez, J. L.; Offenberg, J. H.; Lewandowski, M.; Kleindienst, T. E. Collection efficiency of the aerosol mass spectrometer for chamber-generated secondary organic aerosols Aerosol Sci. Technol. 2012, 47, 294-309
27. Saukko, E.; Lambe, A. T.; Massoli, P.; Koop, T.; Wright, J. P.; Croasdale, D. R.; Pedernera, D. A.; Onasch, T. B.; Laaksonen, A.; Davidovits, P. Humidity-dependent phase state of SOA particles from biogenic and anthropogenic precursors Atmos. Chem. Phys. 2012, 12, 7517-7529
28. Middlebrook, A. M.; Bahreini, R.; Jimenez, J. L.; Canagaratna, M. R. Evaluation of composition-dependent collection efficiencies for the aerodyne aerosol mass spectrometer using field data Aerosol Sci. Technol. 2011, 46, 258-271
29. x photo-oxidation of low volatility precursors: n -Alkanes Environ. Sci. Technol. 2010, 44, 2029-2034
30. Simpson, I. J.; Colman, J. J.; Swanson, A. L.; Bandy, A. R.; Thornton, D. C.; Blake, D. R.; Rowland, F. S. Aircraft measurements of dimethyl sulfide (DMS) using a whole air sampling technique J. Atmos. Chem. 2001, 39, 191-213
31. 2.5 during the Pittsburgh air quality study Aerosol Sci. Technol. 2004, 38, 80-90
32. 2.5 in Pittsburgh, Pennsylvania Atmos. Environ. 2004, 38, 3305-3318
33. May, A. A.; Presto, A. A.; Hennigan, C. J.; Nguyen, N. T.; Gordon, T. D.; Robinson, A. L. Gas-particle partitioning of primary organic aerosol emissions: (1) Gasoline vehicle exhaust Atmos. Environ. 2013, 77, 128-139
34. Gordon, T. D.; Presto, A. A.; Nguyen, N. T.; Robertson, W. H.; Na, K.; Sahay, K. N.; Zhang, M.; Maddox, C.; Rieger, P.; Chattopadhyay, S. Secondary organic aerosol production from diesel vehicle exhaust: impact of aftertreatment, fuel chemistry and driving cycle Atmos. Chem. Phys. Discuss. 2013, 13, 24223-24262
35. May, A. A.; Nguyen, N. T.; Presto, A. A.; Gordon, T. D.; Lipsky, E. M.; Karve, M.; Gutierrez, A.; Robertson, W. H.; Zhang, M.; Brandow, C. Gas- and particle-phase primary emissions from in-use, on-road gasoline and diesel vehicles Atmos. Environ. 2014, 88, 247-260
36. Durbin, T. D.; Wilson, R. D.; Norbeck, J. M.; Miller, J. W.; Huai, T.; Rhee, S. H. Estimates of the emission rates of ammonia from light-duty vehicles using standard chassis dynamometer test cycles Atmos. Environ. 2002, 36, 1475-1482
37. Burgard, D. A.; Bishop, G. A.; Stedman, D. H. Remote sensing of ammonia and sulfur dioxide from on-road light duty vehicles Environ. Sci. Technol. 2006, 40, 7018-7022
38. Kean, A. J.; Littlejohn, D.; Ban-Weiss, G. A.; Harley, R. A.; Kirchstetter, T. W.; Lunden, M. M. Trends in on-road vehicle emissions of ammonia Atmos. Environ. 2009, 43, 1565-1570
39. Mysliwiec, M. J.; Kleeman, M. J. Source apportionment of secondary airborne particulate matter in a polluted atmosphere Environ. Sci. Technol. 2002, 36, 5376-5384
40. U. S. EPA. National Air Quality and Emissions Trends Report-2003 Special Studies Edition; Research Triangle Park, NC, 2003.
41. Ng, N. L.; Canagaratna, M. R.; Jimenez, J. L.; Chhabra, P. S.; Seinfeld, J. H.; Worsnop, D. R. Changes in organic aerosol composition with aging inferred from aerosol mass spectra Atmos. Chem. Phys. 2011, 11, 6465-6474
42. Ulbrich, I. M.; Canagaratna, M. R.; Zhang, Q.; Worsnop, D. R.; Jimenez, J. L. Interpretation of organic components from positive matrix factorization of aerosol mass spectrometric data Atmos. Chem. Phys. 2009, 9, 2891-2918
43. Canagaratna, M. R.; Jayne, J. T.; Ghertner, D. A.; Herndon, S.; Shi, Q.; Jimenez, J. L.; Silva, P. J.; Williams, P.; Lanni, T.; Drewnick, F. Chase studies of particulate emissions from in-use New York City Vehicles Aerosol Sci. Technol. 2004, 38, 555-573
44. Aiken, A. C.; DeCarlo, P. F.; Kroll, J. H.; Worsnop, D. R.; Huffman, J. A.; Docherty, K. S.; Ulbrich, I. M.; Mohr, C.; Kimmel, J. R.; Sueper, D. O/C and OM/OC ratios of primary, secondary, and ambient organic aerosols with high-resolution time-of-flight aerosol mass spectrometry Environ. Sci. Technol. 2008, 42, 4478-4485
45. Grieshop, A. P.; Donahue, N. M.; Robinson, A. L. Laboratory investigation of photochemical oxidation of organic aerosol from wood fires 2: analysis of aerosol mass spectrometer data Atmos. Chem. Phys. 2009, 9, 2227-2240
46. Lambe, A. T.; Onasch, T. B.; Massoli, P.; Croasdale, D. R.; Wright, J. P.; Ahern, A. T.; Williams, L. R.; Worsnop, D. R.; Brune, W. H.; Davidovits, P. Laboratory studies of the chemical composition and cloud condensation nuclei (CCN) activity of secondary organic aerosol (SOA) and oxidized primary organic aerosol (OPOA) Atmos. Chem. Phys. 2011, 11, 8913-8928
47. Jathar, S. H.; Gordon, T. D.; Hennigan, C. J.; Pye, H. O. T.; Donahue, N. M.; Adams, P. J.; Robinson, A. L. Unspeciated organic emissions from combustion sources and their influence on the secondary organic aerosol budget in the United States Proc. Natl. Acad. Sci. U. S. A. 2014, 111, 10473-10478
48. Murphy, B. N.; Donahue, N. M.; Fountoukis, C.; Pandis, S. N. Simulating the oxygen content of ambient organic aerosol with the 2D volatility basis set Atmos. Chem. Phys. 2011, 11, 7859-7873
49. Zhang, X.; Cappa, C. D.; Jathar, S. H.; McVay, R. C.; Ensberg, J. J.; Kleeman, M. J.; Seinfeld, J. H. Influence of vapor wall loss in laboratory chambers on yields of secondary organic aerosol Proc. Natl. Acad. Sci. U. S. A. 2014, 111, 5802-5807
50. Donahue, N. M.; Epstein, S. A.; Pandis, S. N.; Robinson, A. L. A two-dimensional volatility basis set: 1. Organic-aerosol mixing thermodynamics Atmos. Chem. Phys. 2011, 11, 3303-3318
51. Smith, J. D.; Kroll, J. H.; Cappa, C. D.; Che, D. L.; Liu, C. L.; Ahmed, M.; Leone, S. R.; Worsnop, D. R.; Wilson, K. R. The heterogeneous reaction of hydroxyl radicals with sub-micron squalane particles: A model system for understanding the oxidative aging of ambient aerosols Atmos. Chem. Phys. 2009, 9, 3209-3222
52. U. S. EPA 2008 National Emissions Inventory version 3, 2013.
53. De Gouw, J. A.; Middlebrook, A. M.; Warneke, C.; Goldan, P. D.; Kuster, W. C.; Roberts, J. M.; Fehsenfeld, F. C.; Worsnop, D. R.; Canagaratna, M. R.; Pszenny, A. A. P. Budget of organic carbon in a polluted atmosphere: Results from the New England Air Quality Study in 2002 J. Geophys. Res. 2005, 110, D16305