Changes in organic aerosol composition with aging inferred from aerosol mass spectra

Atmospheric Chemistry and Physics

Volumn 11, Issue 13, 2011, Pages 6465-6474

  Ng, N L ^a   Canagaratna, M R ^a   Jimenez, J L ^b   Chhabra, P S ^c   Seinfeld, J H ^c   Worsnop, D R ^a  

^a AERODYNE RESEARCH INC   (United States)

^b UNIVERSITY OF COLORADO   (United States)

^c California Institute of Technology   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

AEROSOL COMPOSITION; AEROSOL FORMATION; CHEMICAL COMPOSITION; HYDROCARBON; MASS SPECTROMETRY; PARAMETERIZATION; PHOTOCHEMISTRY;

EID: 79960133513     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-11-6465-2011     Document Type: Article

References (29)

1. Aiken, A. C., DeCarlo, P. F., and Jimenez, J. L.: Elemental Analysis of Organic Species with Electron Ionization High-Resolution Mass Spectrometry, Anal. Chem., 79, 8350-8358, doi:8310.1021/ac071150w, 2007. (Pubitemid 350060037)
2. Aiken, A. C., DeCarlo, P. F., Kroll, J. H., Worsnop, D. R., Huffman, J. A., Docherty, K. S., Ulbrich, I. M., Mohr, C., Kimmel, J. R., Sueper, D., Sun, Y., Zhang, Q., Trimborn, A., Northway, M., Ziemann, P. J., Canagaratna, M. R., Onasch, T. B., Alfarra, M. R., Prevot, A. S. H., Dommen, J., Duplissy, J., Metzger, A., Baltensperger, U., and Jimenez, J. L.: O/C and OM/OC ratios of primary, secondary, and ambient organic aerosols with high-resolution time-of-flight aerosol mass spectrometry, Environ. Sci. Technol., 42, 4478-4485, 2008. (Pubitemid 351842394)
3. Aiken, A. C., Salcedo, D., Cubison, M. J., Huffman, J. A., DeCarlo, P. F., Ulbrich, I. M., Docherty, K. S., Sueper, D., Kimmel, J. R., Worsnop, D. R., Trimborn, A., Northway, M., Stone, E. A., Schauer, J. J., Volkamer, R. M., Fortner, E., de Foy, B., Wang, J., Laskin, A., Shutthanandan, V., Zheng, J., Zhang, R., Gaffney, J., Marley, N. A., Paredes-Miranda, G., Arnott, W. P., Molina, L. T., Sosa, G., and Jimenez, J. L.: Mexico City aerosol analysis during MILAGRO using high resolution aerosol mass spectrometry at the urban supersite (T0) - Part 1: Fine particle composition and organic source apportionment, Atmos. Chem. Phys., 9, 6633-6653, doi:10.5194/acp-9-6633-2009, 2009.
4. Chhabra, P. S., Flagan, R. C., and Seinfeld, J. H.: Elemental analysis of chamber organic aerosol using an aerodyne high-resolution aerosol mass spectrometer, Atmos. Chem. Phys., 10, 4111-4131, doi:10.5194/acp-10-4111-2010, 2010.
5. Chhabra, P. S., Ng, N. L., Canagaratna, M. R., Corrigan, A. L., Russell, L. M., Worsnop, D. R., Flagan, R. C., and Seinfeld, J. H.: Elemental composition and oxidation of chamber organic aerosol, Atmos. Chem. Phys. Discuss., 11, 10305-10342, doi:10.5194/acpd-11-10305-2011, 2011.
6. Cubison, M. J., Ortega, A. M., Hayes, P. L., Farmer, D. K., Day, D., Lechner, M. J., Brune, W. H., Apel, E., Diskin, G. S., Fisher, J. A., Fuelberg, H. E., Hecobian, A., Knapp, D. J., Mikoviny, T., Riemer, D., Sachse, G. W., Sessions, W., Weber, R. J., Wein-heimer, A. J., Wisthaler, A., and Jimenez, J. L.: Effects of aging on organic aerosol from open biomass burning smoke in aircraft and lab studies, Atmos. Chem. Phys. Discuss., 11, 12103-12140, doi:10.5194/acpd-11-12103-2011, 2011.
7. DeCarlo, P. F., Ulbrich, I. M., Crounse, J., de Foy, B., Dunlea, E. J., Aiken, A. C., Knapp, D., Weinheimer, A. J., Campos, T., Wennberg, P. O., and Jimenez, J. L.: Investigation of the sources and processing of organic aerosol over the Central Mexican Plateau from aircraft measurements during MILAGRO, At-mos. Chem. Phys., 10, 5257-5280, doi:10.5194/acp-10-5257-2010, 2010.
8. Decesari, S., Mircea, M., Cavalli, F., Fuzzi, S., Moretti, F., Tagli-avini, E., and Facchini, M. C.: Source attribution of water-soluble organic aerosol by nuclear magnetic resonance spec-troscopy, Environ. Sci. Technol., 41, 2479-2484, 2007. (Pubitemid 46595215)
9. Docherty, K. S., Stone, E. A., Ulbrich, I. M., DeCarlo, P. F., Snyder, D. C., Schauer, J. J., Peltier, R. E., Weber, R. J., Murphy, S. M., Seinfeld, J. H., Grover, B. D., Eatough, D. J., and Jiimenez, J. L.: Apportionment of Primary and Secondary Organic Aerosols in Southern California during the 2005 Study of Organic Aerosols in Riverside (SOAR-1), Environ. Sci. Technol., 42, 7655-7662, 2008.
10. Duplissy, J., DeCarlo, P. F., Dommen, J., Alfarra, M. R., Met-zger, A., Barmpadimos, I., Prevot, A. S. H., Weingartner, E., Tritscher, T., Gysel, M., Aiken, A. C., Jimenez, J. L., Cana-garatna, M. R., Worsnop, D. R., Collins, D. R., Tomlinson, J., and Baltensperger, U.: Relating hygroscopicity and composition of organic aerosol particulate matter, Atmos. Chem. Phys., 11, 1155-1165, doi:10.5194/acp-11-1155-2011, 2011.
11. Heald, C. L., Kroll, J. H., Jimenez, J. L., Docherty, K. S., DeCarlo, P. F., Aiken, A. C., Chen, Q., Martin, S. T., Farmer, D. K., and Artaxo, P.: A simplified description of the evolution of organic aerosol composition in the atmosphere, Geophys. Res. Lett., 37, L08803, doi:08810.01029/02010GL042737, 2010.
12. Huang, X.-F., He, L.-Y., Hu, M., Canagaratna, M. R., Sun, Y., Zhang, Q., Zhu, T., Xue, L., Zeng, L.-W., Liu, X.-G., Zhang, Y.-H., Jayne, J. T., Ng, N. L., and Worsnop, D. R.: Highly time-resolved chemical characterization of atmospheric submi-cron particles during 2008 Beijing Olympic Games using an Aerodyne High-Resolution Aerosol Mass Spectrometer, Atmos. Chem. Phys., 10, 8933-8945, doi:10.5194/acp-10-8933-2010, 2010.
13. Huang, X.-F., He, L.-Y., Hu, M., Canagaratna, M. R., Kroll, J. H., Ng, N. L., Zhang, Y.-H., Lin, Y., Xue, L., Sun, T.-L., Liu, X.-G., Shao, M., Jayne, J. T., and Worsnop, D. R.: Characterization of submicron aerosols at a rural site in Pearl River Delta of China using an Aerodyne High-Resolution Aerosol Mass Spectrometer, Atmos. Chem. Phys., 11, 1865-1877, doi:10.5194/acp-11-1865-2011, 2011.
14. x/air in the presence of natural sunlight, J. Geophys. Res.-Atmos., 106, 12541-12558, 2001.
15. Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., Aiken, A. C., Docherty, K. S., Ulbrich, I. M., Grieshop, A. P., Robinson, A. L., Duplissy, J., Smith, J. D., Wilson, K. R., Lanz, V. A., Hueglin, C., Sun, Y. L., Tian, J., Laak-sonen, A., Raatikainen, T., Rautiainen, J., Vaattovaara, P., Ehn, M., Kulmala, M., Tomlinson, J. M., Collins, D. R., Cubison, M. J., Dunlea, E. J., Huffman, J. A., Onasch, T. B., Alfarra, M. R., Williams, P. I., Bower, K., Kondo, Y., Schneider, J., Drewnick, F., Borrmann, S., Weimer, S., Demerjian, K., Salcedo, D., Cot-trell, L., Griffin, R., Takami, A., Miyoshi, T., Hatakeyama, S., Shimono, A., Sun, J. Y., Zhang, Y. M., Dzepina, K., Kimmel, J. R., Sueper, D., Jayne, J. T., Herndon, S. C., Trimborn, A. M., Williams, L. R., Wood, E. C., Middlebrook, A. M., Kolb, C. E., Baltensperger, U., and Worsnop, D. R.: Evolution of Organic Aerosols in the Atmosphere, Science, 326, 1525-1529, 2009.
16. Johnson, D., Jenkin, M. E., Wirtz, K., and Martin-Reviejo, M.: Simulating the formation of secondary organic aerosol from the pho-tooxidation of toluene, Environ. Chem., 1, 150-165, 2004.
17. Johnson, D., Jenkin, M. E., Wirtz, K., and Martin-Reviejo, M.: Simulating the formation of secondary organic aerosol from the pho-tooxidation of aromatic hydrocarbons, Environ. Chem., 2, 35-48, 2005.
18. Kroll, J. H., Smith, J. D., Che, D. L., Kessler, S. H., Worsnop, D. R., and Wilson, K. R.: Measurement of fragmentation and function-alization pathways in the heterogeneous oxidation of oxidized organic aerosol, Phys. Chem. Chem. Phys., 11, 8005-8014, 2009.
19. Kroll, J. H., Donahue, N. M., Jimenez, J. L., Kessler, S. H., Cana-garatna, M. R., Wilson, K. R., Altieri, K. E., Mazzoleni, L. R., Wozniak, A. S., Bluhm, H., Mysak, E. R., Smith, J. D., Kolb, C. E., and Worsnop, D. R.: Carbon oxidation state as a metric for describing the chemistry of atmospheric organic aerosol, Nat. Chem., 3, 133-139, doi:110.1038/NCHEM.1948, 2011.
20. Lambe, A. T., Onasch, T. B., Massoli, P., Croasdale, D. R., Wright, J. P., Ahern, A. T., Williams, L. R., Worsnop, D. R., Brune, W. H., and Davidovits, P.: Laboratory studies of the chemical composition and cloud condensation nuclei (CCN) activity of secondary organic aerosol (SOA) and oxidized primary organic aerosol (OPOA), Atmos. Chem. Phys. Discuss., 11, 13617- 13653, doi:10.5194/acpd-11-13617-2011, 2011.
21. Massoli, P., Lambe, A. T., Ahern, A. T., Williams, L. R., Ehn, M., Mikkila, J., Canagaratna, M. R., Brune, W. H., Onasch, T. B., Jayne, J. T., Petaja, T., Kulmala, M., Laaksonen, A., Kolb, C. E., Davidovits, P., and Worsnop, D. R.: Relationship between aerosol oxidation level and hygroscopic properties of laboratory generated secondary organic aerosol (SOA) particles, Geo-phys. Res. Lett., 37, L24801, doi:24810.21029/22010GL045258, 2010.
22. Morgan, W. T., Allan, J. D., Bower, K. N., Highwood, E. J., Liu, D., McMeeking, G. R., Northway, M. J., Williams, P. I., Krejci, R., and Coe, H.: Airborne measurements of the spatial distribution of aerosol chemical composition across Europe and evolution of the organic fraction, Atmos. Chem. Phys., 10, 4065-4083, doi:10.5194/acp-10-4065-2010, 2010.
23. Ng, N. L., Canagaratna, M. R., Zhang, Q., Jimenez, J. L., Tian, J., Ulbrich, I. M., Kroll, J. H., Docherty, K. S., Chhabra, P. S., Bahreini, R., Murphy, S. M., Seinfeld, J. H., Hildebrandt, L., Donahue, N. M., DeCarlo, P. F., Lanz, V. A., Prévôt, A. S. H., Dinar, E., Rudich, Y., and Worsnop, D. R.: Organic aerosol components observed in Northern Hemispheric datasets from Aerosol Mass Spectrometry, Atmos. Chem. Phys., 10, 4625- 4641, doi:10.5194/acp-10-4625-2010, 2010.
24. Ng, N. L., Herndon, S. C., Trimborn, A., Canagaratna, M. R., Croteau, P., Onasch, T. M., Sueper, D., Worsnop, D. R., Zhang, Q., Sun, Y. L., and Jayne, J. T.: An Aerosol Chemical Speciation Monitor (ACSM) for routine monitoring of atmospheric aerosol composition, Aerosol Sci. Technol., 45, 770-784, 2011.
25. Russell, L. M., Bahadur, R., and Ziemann, P. J.: Identifying organic aerosol sources by comparing functional group composition in chamber and atmospheric particles, Proc. Natl. Acad. Sci. USA, 108, 3516-3521, doi:10.1073/pnas.1006461108, 2011.
26. Sun, Y.-L., Zhang, Q., Schwab, J. J., Demerjian, K. L., Chen, W.-N., Bae, M.-S., Hung, H.-M., Hogrefe, O., Frank, B., Rattigan, O. V., and Lin, Y.-C.: Characterization of the sources and processes of organic and inorganic aerosols in New York city with a high-resolution time-of-flight aerosol mass apectrometer, At-mos. Chem. Phys., 11, 1581-1602, doi:10.5194/acp-11-1581-2011, 2011.
27. Surratt, J. D., Murphy, S. M., Kroll, J. H., Ng, N. L., Hildebrandt, L., Sorooshian, A., Szmigielski, R., Vermeylen, R., Maenhaut, W., Claeys, M., Flagan, R. C., and Seinfeld, J. H.: Chemical composition of secondary organic aerosol formed from the photooxidation of isoprene, J. Phys. Chem. A, 110, 9665-9690, 2006. (Pubitemid 44318455)
28. Szmigielski, R., Surratt, J. D., Gomez-Gonzalez, Y., Van der Veken, P., Kourtchev, I., Vermeylen, R., Blockhuys, F., Jaoui, M., Klein-dienst, T. E., Lewandowski, M., Offenberg, J. H., Edney, E. O., Seinfeld, J. H., Maenhaut, W., and Claeys, M.: 3-methyl-1,2,3-butanetricarboxylic acid: An atmospheric tracer for ter-pene secondary organic aerosol, Geophys.Res. Lett., 34, L24811, doi:24810.21029/22007GL031338, 2007.
29. Van Krevelen, D. W.: Graphical-statistical method for the study of structure and reaction processes of coal, Fuel, 24, 269-284, 1950.