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We have recently found that complexes 1a, 1c, and 1d exist in two different bond isomeric forms. These results will be described elsewhere, but the identity of the employed isomer is not influential to the present discussion, since both yielded the same products.
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We have recently found that complexes 1a, 1c, and 1d exist in two different bond isomeric forms. These results will be described elsewhere, but the identity of the employed isomer is not influential to the present discussion, since both yielded the same products.
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Steric effects have also been generically proposed to affect the reactivity of the monomeric complex in a few cases, but the exact role of the steric hindrance has not been clarified. It is also possible that the presence of the ortho methyl groups inhibits the formation of electronically saturated and catalytically inactive monomeric complexes having two chelating ligands in the coordination sphere. However, to the best of our knowledge, this explanation has never been advanced in the literature for the ligands employed in the present study
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