Challenge to the charging model of semiconductor-nanocrystal fluorescence intermittency from off-state quantum yields and multiexciton blinking

Physical Review Letters

Volumn 104, Issue 15, 2010, Pages

  Zhao, Jing ^a   Nair, Gautham ^a   Fisher, Brent R ^a   Bawendi, Moungi G ^a  

^a MASSACHUSETTS INSTITUTE OF TECHNOLOGY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

BIEXCITON; CHARGING MODELS; DARK PERIODS; DARK STATE; FLUORESCENCE INTERMITTENCY; MULTIEXCITONS; ON/OFF RATIO; PL INTENSITY; PL QUANTUM YIELD; SEMICONDUCTOR NANOCRYSTALS; TIME TRACE;

CADMIUM COMPOUNDS; NANOCRYSTALS; SEMICONDUCTOR QUANTUM DOTS;

QUANTUM THEORY;

EID: 77951067937     PISSN: 00319007     EISSN: 10797114     Source Type: Journal    
DOI: 10.1103/PhysRevLett.104.157403     Document Type: Article

References (39)

1. M. Nirmal, Nature (London) NATUAS 0028-0836 383, 802 (1996). 10.1038/383802a0
2. S.A. Empedocles, Adv. Mater. ADVMEW 0935-9648 11, 1243 (1999). 10.1002/(SICI)1521-4095(199910)11:15<1243::AID-ADMA1243>3.0.CO;2-2
3. S. Coe-Sullivan, Nature (London) NATUAS 0028-0836 420, 800 (2002). 10.1038/nature01217
4. J. Zhao, Nano Lett. 6, 463 (2006). NALEFD 1530-6984 10.1021/nl052417e
5. P.O. Anikeeva, Phys. Rev. B PRBMDO 1098-0121 78, 085434 (2008). 10.1103/PhysRevB.78.085434
6. J.-M. Caruge, Nat. Photon. 1749-4885 2, 247 (2008). 10.1038/nphoton.2008. 34
7. P.O. Anikeeva, Nano Lett. 9, 2532 (2009). NALEFD 1530-6984 10.1021/nl9002969
8. V.I. Klimov, Science 290, 314 (2000). SCIEAS 0036-8075 10.1126/science.290.5490.314
9. M. Dahan, Science 302, 442 (2003). SCIEAS 0036-8075 10.1126/science. 1088525
10. S. Courty, Nano Lett. 6, 1491 (2006). NALEFD 1530-6984 10.1021/nl060921t
11. M. Howarth, Nat. Methods 5, 397 (2008). 1548-7091 10.1038/nmeth.1206
12. B. Lounis, Chem. Phys. Lett. 329, 399 (2000). CHPLBC 0009-2614 10.1016/S0009-2614(00)01042-3
13. P. Michler, Nature (London) NATUAS 0028-0836 406, 968 (2000). 10.1038/35023100
14. X. Brokmann, Appl. Phys. Lett. 85, 712 (2004). APPLAB 0003-6951 10.1063/1.1775280
15. B.R. Fisher, Phys. Rev. Lett. 94, 087403 (2005). PRLTAO 0031-9007 10.1103/PhysRevLett.94.087403
16. A.L. Efros and M. Rosen, Phys. Rev. Lett. 78, 1110 (1997). PRLTAO 0031-9007 10.1103/PhysRevLett.78.1110
17. B. Mahler, Nature Mater. NMAACR 1476-1122 7, 659 (2008). 10.1038/nmat2222
18. Y. Chen, J. Am. Chem. Soc. 130, 5026 (2008). JACSAT 0002-7863 10.1021/ja711379k
19. D.I. Chepic, J. Lumin. 47, 113 (1990). JLUMA8 0022-2313 10.1016/0022-2313(90)90007-X
20. V.I. Klimov, Science 287, 1011 (2000). SCIEAS 0036-8075 10.1126/science.287.5455.1011
21. V.I. Klimov, Annu. Rev. Phys. Chem. 58, 635 (2007). ARPLAP 0066-426X 10.1146/annurev.physchem.58.032806.104537
22. K.T. Shimizu, Phys. Rev. B PRBMDO 0163-1829 63, 205316 (2001). 10.1103/PhysRevB.63.205316
23. R. Verberk, A.M. van Oijen, and M. Orrit, Phys. Rev. B PRBMDO 0163-1829 66, 233202 (2002). 10.1103/PhysRevB.66.233202
24. M. Kuno, Phys. Rev. B PRBMDO 0163-1829 67, 125304 (2003). 10.1103/PhysRevB.67.125304
25. J. Tang and R.A. Marcus, J. Chem. Phys. 123, 054704 (2005). JCPSA6 0021-9606 10.1063/1.1993567
26. P.A. Frantsuzov and R.A. Marcus, Phys. Rev. B PRBMDO 1098-0121 72, 155321 (2005). 10.1103/PhysRevB.72.155321
27. See supplementary material at http://link.aps.org/supplemental/10.1103/ PhysRevLett.104.157403 for supplementary data and derivations.
28. G. Nair, J. Zhao, and M.G. Bawendi (unpublished).
29. J.-M. Caruge, Phys. Rev. B PRBMDO 1098-0121 70, 085316 (2004). 10.1103/PhysRevB.70.085316
30. C. Bonati, Phys. Rev. B PRBMDO 1098-0121 71, 205317 (2005). 10.1103/PhysRevB.71.205317
31. A. Franceschetti and M.C. Troparevsky, J. Phys. Chem. C 111, 6154 (2007). 1932-7447 10.1021/jp070223c
32. M.G. Bawendi, M.L. Steigerwald, and L.E. Brus, Annu. Rev. Phys. Chem. 41, 477 (1990). ARPLAP 0066-426X 10.1146/annurev.pc.41.100190.002401
33. L.-W. Wang, Phys. Rev. Lett. 91, 056404 (2003). PRLTAO 0031-9007 10.1103/PhysRevLett.91.056404
34. P. Jha and P. Guyot-Sionnest, ACS Nano 3, 1011 (2009). 1936-086X 10.1021/nn9001177
35. G. Nair and M.G. Bawendi, Phys. Rev. B PRBMDO 1098-0121 76, 081304(R) (2007). 10.1103/PhysRevB.76.081304
36. P. Spinicelli, Phys. Rev. Lett. 102, 136801 (2009). PRLTAO 0031-9007 10.1103/PhysRevLett.102.136801
37. D.E. Gómez, ACS Nano 3, 2281 (2009). 1936-086X 10.1021/nn900296q
38. J. Tang and R.A. Marcus, Phys. Rev. Lett. 95, 107401 (2005). PRLTAO 0031-9007 10.1103/PhysRevLett.95.107401
39. P.A. Frantsuzov, S. Volkan-Kacso, and B. Janko, Phys. Rev. Lett. 103, 207402 (2009). PRLTAO 0031-9007 10.1103/PhysRevLett.103.207402