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The Ru-Ga system is an interesting target for soft chemical synthesis of unusual intermetallics. See Supporting Information for details
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All energies herein are given as relative free energies ΔGo for the standard state.
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All energies herein are given as relative free energies ΔGo for the standard state.
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70349969129
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Substituent-free Ga atoms in a linearly bridging position have been observed previously by S. Aldridge et al. and K. Ueno et al. However, these examples contain the gallium in the oxidation state Ga(III) and bonded to the transition-metal carbonyl fragments, rather than Ga(I) bonded to the carbonyl-free transition-metal fragments. See, for example: a) N. R. Bunn, S. Aldridge, D. L. Coombs, A. Rossin, D. J. Willock, C. Jones, L. L. Ooi, Chem. Commun. 2004, 1732-1733
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Substituent-free Ga atoms in a linearly bridging position have been observed previously by S. Aldridge et al. and K. Ueno et al. However, these examples contain the gallium in the oxidation state Ga(III) and bonded to the transition-metal carbonyl fragments, rather than Ga(I) bonded to the carbonyl-free transition-metal fragments. See, for example: a) N. R. Bunn, S. Aldridge, D. L. Coombs, A. Rossin, D. J. Willock, C. Jones, L. L. Ooi, Chem. Commun. 2004, 1732-1733
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