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A typical experimental procedure: a 25 mL round bottom flask with a magnetic bar was charged with 0.5 mmol of 1c, following the method described in Ref, 6b, and 10 mL of CH3CN. To this suspension was added 0.6 mmol (1.2 equiv, of NO+BF4, The reaction mixture became clear. The solution was stirred at room temperature for 2.5 h until TLC showed the completion of reaction. The solution was then concentrated under vacuum and purified by column chromatography on silica gel (petroleum ether/ethyl acetate, 1:2, v/v) to afford pure 2c. The single crystal was grown in chloroform-hexane at room temperature. All products were identified by 1H and 13C NMR, MS, IR, and HR-ESI-MS. Selected data for compound 2c: white solid, mp 187-188 °C; IR (KBr, max 3408, 2984, 2907, 1717, 1658, 1598, 1437, 1279, 1097, 840 and 800 cm-1. 1H NMR (400 MHz, CDCl3, δ (ppm, 10.35 (br, s, 1H, 7.56 d, 2H
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