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Finlayson, C.E.1
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At higher concentrations of cytochrome c, we see a slight blue shift and a quenching of the emission intensity. Moreover, there is a second peak/shoulder observable at around 560 nm, which is only apparent at higher concentrations than 1.43 ± 10-6 M of cytochrome c
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-6 M of cytochrome c.
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-5 M for the QDs.
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-5 M for the QDs.
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-5 M for cyt c, respectively. All experiments were carried out were carried out in a standard 2 mm quartz cuvette utilizing an excitation wavelength of 387 nm with a laser energy per pulse around 200 nJ.
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-5 M for cyt c, respectively. All experiments were carried out were carried out in a standard 2 mm quartz cuvette utilizing an excitation wavelength of 387 nm with a laser energy per pulse around 200 nJ.
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Transient absorption measurements with cytochrome c in either oxidation state reveal mainly features that are best described as the mirror image to the ground state absorptions in the visible-see Figures S8 and SlO, Supporting Information, These transients are, however, very shortlived and decay with lifetimes of 8.1 and 6.3 ps for Fe(II) and Fe(III, respectively, quantitatively back to the ground state. Please find the corresponding time-absorption profiles in Figures S9 and S11 Supporting Information
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Transient absorption measurements with cytochrome c in either oxidation state reveal mainly features that are best described as the mirror image to the ground state absorptions in the visible-see Figures S8 and SlO, Supporting Information). These transients are, however, very shortlived and decay with lifetimes of 8.1 and 6.3 ps for Fe(II) and Fe(III), respectively, quantitatively back to the ground state. Please find the corresponding time-absorption profiles in Figures S9 and S11 (Supporting Information).
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