Two-photon dissociation and ionization of liquid water studied by femtosecond transient absorption spectroscopy

Journal of Chemical Physics

Volumn 110, Issue 7, 1999, Pages 3453-3462

  Thomsen, C L ^a   Madsen, D ^a   Keiding, S R ^a   Thogersen J ^a   Christiansen, O ^b  

^a AARHUS UNIVERSITY   (Denmark)

^b JOHANNES GUTENBERG UNIVERSITY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

ABSORPTION SPECTROSCOPY; ATOMS; ELECTRON ENERGY LEVELS; ELECTRON TRANSITIONS; ELECTRONS; MOLECULES; NUMERICAL METHODS; PHOTODISSOCIATION; PHOTOIONIZATION; PHOTONS; PROTONS; ULTRAVIOLET RADIATION;

FEMTOSECOND TRANSIENT ABSORPTION SPECTROSCOPY; GEMINATE RECOMBINATION; HYDRATED ELECTRONS; PROTON TRANSFER;

WATER;

EID: 0033556934     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.478212     Document Type: Article

References (90)

1. N. Pugliano, D. K. Palit, A. Z. Szarka, and R. M. Hochstrasser, J. Chem. Phys. 99, 7273 (1993).
2. N. Pugliano, A. Z. Szarka, and R. M. Hochstrasser, J. Chem. Phys. 104, 5062 (1996).
3. T. Kühne and P. Vöhringer, J. Chem. Phys. 105, 10788 (1996).
4. E. Gershgoren, U. Banin, and S. Ruhman, J. Phys. Chem. 102, 9 (1998).
5. P. K. Walhout, C. Silva, and P. F. Barbara, J. Phys. Chem. 100, 5188 (1996).
6. J. Aa. Poulsen, C. L. Thomsen, S. R. Keiding, and J. Thøgersen, J. Chem. Phys. 108, 8461 (1998).
7. J. Thøgersen, C. L. Thomsen, J. Aa. Poulsen, and S. R. Keiding, J. Phys. Chem. 102, 4186 (1998).
8. D. N. Nikogosyan, A. A. Oraevsky, and V. I. Rupasov, Chem. Phys. 77, 131 (1983).
9. J. W. Boyle, J. A. Ghormley, C. J. Hochanadel, and J. F. Riley, J. Phys. Chem. 73, 2886 (1969).
10. U. Sokolov and G. Stein, J. Chem. Phys. 44, 3329 (1966).
11. S. O. Nielsen, B. D. Michael, and E. J. Hart, J. Phys. Chem. 80, 2482 (1976).
12. P. Pagsberg, H. Christensen, J. Rabani, G. Nilsson, J. Fenger, and S. O. Nielsen, J. Phys. Chem. 73, 1029 (1969).
13. H. Okabe, Photochemistry of Small Molecules (Wiley, New York, 1978).
14. J. M. Heller Jr., R. N. Hamm, R. D. Birkoff, and L. R. Painter, J. Chem. Phys. 60, 3483 (1974).
15. G. D. Kerr, R. N. Hamm, M. W. Williams, R. D. Birkhoff, and L. R. Painter, Phys. Rev. A 5, 2523 (1972).
16. F. Williams, S. P. Varma, and S. Hillenius, J. Chem. Phys. 64, 1549 (1976).
17. D. G. Imre and J. Zhang, Chem. Phys. 139, 89 (1989).
18. V. Engle, V. Staemmler, and R. Schinke, J. Chem. Phys. 88, 129 (1988).
19. K. Weide and R. Schinke, J. Chem. Phys. 87, 4627 (1987).
20. K. Weide and R. Schinke, J. Chem. Phys. 90, 7150 (1989).
21. I. P. Vinogradov and F. I. Vilesov, Opt. Spectrosc. 40, 32 (1976).
22. L. J. Stief, W. A. Payne, and R. B. Klemm, J. Chem. Phys. 62, 4000 (1975).
23. D. Grand, A. Bernas, and E. Amouyal, Chem. Phys. 44, 73 (1979).
24. A. Iwata, N. Nakashima, Y. Izawa, and C. Yamanaka, Chem. Lett. 21, 1939 (1993).
25. J. L. McGowen, H. M. Ajo, J. Z. Zhang, and B. J. Schwartz, Chem. Phys. Lett. 231, 503 (1994).
26. W. A. Goddard III and W. J. Hunt, Chem. Phys. Lett. 24, 464 (1974).
27. O. Dutuit, A. Tabche-Fouhaile, I. Nenner, H. Frochlich, and P. M. Guyon, J. Chem. Phys. 83, 584 (1985).
28. P. Han and D. M. Bartels, J. Phys. Chem. 94, 5824 (1990).
29. M. U. Sander, K. Luther, and J. Troe, Ber. Bunsenges. Phys. Chem. 97, 953 (1993).
30. T. Goulet, A. Bernas, C. Ferradini, and J.-P. Jay-Gerin, Chem. Phys. Lett. 170, 492 (1990).
31. A. Bernas, C. Ferradini, and J.-P. Jay-Gerin, Chem. Phys. 222, 151 (1997).
32. H. Shiraishi, G. R. Sunaryo, and K. Ishigure, J. Phys. Chem. 98, 5164 (1994).
33. R. A. Crowell and D. M. Bartels, J. Phys. Chem. 100, 17940 (1996).
34. P. Han and D. M. Bartels, J. Phys. Chem. 96, 4899 (1992).
35. D. N. Nikogosyan and H. J. Goerner, J. Photochem. Photobiol., B 13, 219 (1992).
36. M. Anbar, G. A. St. John, H. R. Gloria, and R. F. Reinisch, in Water Structure at the Water-Polymer Interface, edited by H. H. G. Jellinek (Plenum, New York, 1972), p. 85.
37. A. Bernas and D. Grand, J. Phys. Chem. 98, 3440 (1994).
38. E. J. Hart and M. Anbar, The Hydrated Electron (Wiley-Interscince, New York, 1971).
39. A. J. Swallow, Radiation Chemistry. An introduction (Longman, London, 1973).
40. K. J. Hartig and N. Getoff, J. Photochem. 18, 29 (1982).
41. T. Goulet and J.-P. Jay-Gerin, J. Chem. Phys. 96, 5076 (1992).
42. F.-Y. Jou and G. R. Freeman, J. Phys. Chem. 81, 909 (1977).
43. E. Rabinowitch, Rev. Mod. Phys. 14, 112 (1942).
44. P. Pagsberg (private communication).
45. E. J. Hart and J. W. Boag, J. Am. Chem. Soc. 84, 4090 (1962); J. W. Boag and E. J. Hart, Nature (London) 197, 45 (1963).
46. E. J. Hart and J. W. Boag, J. Am. Chem. Soc. 84, 4090 (1962); J. W. Boag and E. J. Hart, Nature (London) 197, 45 (1963).
47. A. Reuther, A. Laubereau, and D. N. Nikogosyan, J. Phys. Chem. 100, 16794 (1996).
48. P. K. Walhout and P. F. Barbara, in Ultrafast Processes in Chemistry and Photobiology, edited by M. A. El-Sayed, I. Tanaka, and Y. Molin (UPAC-A, Chemistry for the 21st Century Monograph, Blackwell Science, London, 1995).
49. Y. Kimura, J. C. Alfano, P. K. Walhout, and P. F. Barbara, J. Phys. Chem. 98, 3450 (1994).
50. C. Silva, P. K. Walhout, K. Yokoyama, and P. F. Barbara, Phys. Rev. Lett. 80, 1086 (1998).
51. F. H. Long and K. B. Eisenthal, in Ultrafast Processes in Chemistry and Photobiology, edited by M. A. El-Sayed, I. Tanaka, and Y. Molin (UPAC-A, Chemistry for the 21st Century Monograph, Blackwell Science, London, 1995).
52. H. Lu, F. H. Long, R. M. Bowman, and K. B. Eisenthal, J. Phys. Chem. 93, 27 (1989).
53. F. H. Long, H. Lu, and K. B. Eisenthal, Phys. Rev. Lett. 64, 1469 (1990).
54. X. Shi, F. H. Long, H. Lu, and K. B. Eisenthal, J. Phys. Chem. 100, 11903 (1996).
55. Y. Gauduel, S. Pommeret, A. Migus, and A. Antonetti, J. Phys. Chem. 93, 3880 (1989).
56. Y. Gauduel, S. Pommeret, A. Migus, and A. Antonetti, Chem. Phys. 149, 1 (1990).
57. A. Migus, Y. Gauduel, J. L. Martin, and A. Antonetti, Phys. Rev. Lett. 58, 1559 (1987).
58. C. Pépin, T. Goulet, D. Houde, and J.-P. Jay-Gerin, J. Phys. Chem. 101, 4351 (1997).
59. M. F. Emde, A. Baltuška, A. Kummrov, M. S. Pshenichnikov, and D. A. Wiersma, Phys. Rev. Lett. 80, 4645 (1998).
60. M. Assel, R. Laenen, and A. Laubereau, J. Phys. Chem. 102, 2256 (1998).
61. B. J. Schwartz and P. J. Rossky, J. Chem. Phys. 105, 6997 (1996).
62. B. J. Schwartz and P. J. Rossky, J. Chem. Phys. 101, 6902 (1994).
63. S. Bratos, J.-Cl. Leicknam, D. Borgis, and A. Staib, Phys. Rev. E 55, 7217 (1997).
64. R. B. Barnett, A. Nitzan, and U. Landman, J. Chem. Phys. 90, 4413 (1989).
65. I. Rips, Chem. Phys. Lett. 245, 79 (1995).
66. P. R. Monson and W. M. McClain, J. Chem. Phys. 53, 29 (1970).
67. C. Hättig, O. Christiansen, and P. Jørgensen, J. Chem. Phys. 108, 8355 (1998).
68. O. Christiansen, H. Kock, A. Halkier, P. Jørgensen, T. Helgaker, and A. Sanchez de Meras, J. Chem. Phys. 105, 6921 (1996).
69. O. Christiansen, A. Halkier, H. Kock, P. Jørgensen, and T. Helgaker, J. Chem. Phys. 108, 2801 (1998).
70. D. E. Woon and T. H. Dunning, J. Chem. Phys. 100, 2975 (1994).
71. M. B. Robin, Higher Excited States of Polyatomic Molecules, Vol. III (Academic, Orlando, 1985).
72. F.-Y. Jou and G. R. Freeman, J. Phys. Chem. 83, 2383 (1979).
73. P. Clifford, N. J. B. Green, and M. J. Pilling, J. Phys. Chem. 88, 4171 (1984).
74. S. M. Pimblott, J. Phys. Chem. 95, 6946 (1991).
75. M. Terrissol and A. Beaudré, Radiat. Prot. Dosim. 31, 175 (1990).
76. L. Onsager, Phys. Rev. 54, 554 (1938).
77. G. C. Abell and A. Mozumder, J. Chem. Phys. 56, 4079 (1972).
78. G. V. Buxton, C. L. Greenstrock, W. P. Helman, and A. B. Ross, J. Phys. Chem. Ref. Data 17, 513 (1988).
79. F. Busi, M. D'Angelantonio, G. Bettoli, V. Concialini, O. Tubertini, and G. C. Barker, Inorg. Chim. Acta 84, 105 (1984).
80. K. H. Schmidt and W. L. Buck, Science 151, 70 (1966); G. C. Barker, P. Fowles, D. C. Sammon, and B. Stringer, Trans. Faraday Soc. 66, 1498 (1970).
81. K. H. Schmidt and W. L. Buck, Science 151, 70 (1966); G. C. Barker, P. Fowles, D. C. Sammon, and B. Stringer, Trans. Faraday Soc. 66, 1498 (1970).
82. N. J. B. Green, M. J. Pilling, S. M. Pimblott, and P. Clifford, J. Phys. Chem. 94, 251 (1990).
83. N. J. B. Green, Chem. Phys. Lett. 107, 485 (1984).
84. C. Biondi and L. Bellugi, Chem. Phys. 62, 145 (1981); A. J. Elliot, D. R. McCracken, G. V. Buxton, and N. D. Wood, J. Chem. Soc., Faraday Trans. 86, 1539 (1990).
85. C. Biondi and L. Bellugi, Chem. Phys. 62, 145 (1981); A. J. Elliot, D. R. McCracken, G. V. Buxton, and N. D. Wood, J. Chem. Soc., Faraday Trans. 86, 1539 (1990).
86. F. C. Collins and G. E. Kimball, J. Colloid Sci. 4, 425 (1949); F. C. Collins, ibid. 5, 499 (1950).
87. F. C. Collins and G. E. Kimball, J. Colloid Sci. 4, 425 (1949); F. C. Collins, ibid. 5, 499 (1950).
88. S. Woutersen, U. Emmerichs, H.-K. Nienhuys, and H. J. Bakker, Phys. Rev. Lett. 81, 1106 (1998).
89. R. Rey and J. T. Hynes, J. Chem. Phys. 104, 2356 (1996).
90. Y. Cohen, I. Bar, and S. Rosenwaks, J. Chem. Phys. 102, 3612 (1995).