Observation of a continuous spectral shift in the solvation kinetics of electrons in neat liquid deuterated water

Journal of Physical Chemistry A

Volumn 101, Issue 24, 1997, Pages 4351-4360

  Pepin C ^a   Goulet, T ^a   Houde, D ^a   Jay Gerin, J P ^a  

^a UNIVERSITY OF SHERBROOKE   (Canada)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 0000241591     PISSN: 10895639     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp970354l     Document Type: Article

References (103)

1. Rentzepis, P. M.; Jones, R. P.; Jortner, J. J. Chem. Phys. 1973, 59, 766.
2. Baxendale, J. H.; Wardman, P. J. Chem. Soc., Faraday Trans, 1 1973, 69, 584.
3. Chase, W. J.; Hunt, J. W. J. Phys. Chem. 1975, 79, 2835.
4. Klassen, N. V.; Gillis, H. A.; Teather, G. G.; Kevan, L. J. Chem. Phys. 1975, 62, 2474.
5. Kenney-Wallace, G. A.; Jonah, C. D. Chem. Phys. Lett. 1976, 39, 596.
6. Baxendale, J. H.; Sharpe, P. H. G. Int. J. Radiat. Phys. Chem. 1976, 8, 621.
7. Gilles, L.; Bono, M. R.; Schmidt, M. Can. J. Chem. 1977, 55, 2003.
8. Okazaki, K.; Freeman, G. R. Can. J. Chem. 1978, 56, 2305.
9. Ogasawara, M.; Shimizu, K.; Yoshida, K.; Kroh, J.; Yoshida, H. Chem. Phys. Lett. 1979, 64, 43. Ogasawara, M.; Shimizu, K.; Yoshida, H. Radiat. Phys. Chem. 1981, 17, 331.
10. Ogasawara, M.; Shimizu, K.; Yoshida, K.; Kroh, J.; Yoshida, H. Chem. Phys. Lett. 1979, 64, 43. Ogasawara, M.; Shimizu, K.; Yoshida, H. Radiat. Phys. Chem. 1981, 17, 331.
11. Wang, Y.; Crawford, M. K.; McAuliffe, M. J.; Eisenthal, K. B. Chem. Phys. Lett. 1980, 74, 160.
12. Wiesenfeld, J. M.; Ippen, E. P. Chem. Phys. Lett. 1980, 73, 47.
13. Kenney-Wallace, G. A.; Jonah, C. D. J. Phys. Chem. 1982, 86, 2572.
14. Lewis, M. A.; Jonah, C. D. J. Phys. Chem. 1986, 90, 5367.
15. Migus, A.; Gauduel, Y.; Martin, J. L.; Antonetti, A. Phys. Rev. Lett. 1987, 58, 1559.
16. Lu, H.; Long, F. H.; Bowman, R. M.; Eisenthal, K. B. J. Phys. Chem. 1989, 93, 27.
17. Gauduel, Y.; Pommeret, S.; Migus, A.; Antonetti, A. J. Phys. Chem. 1989, 93, 3880.
18. Long, F. H.; Lu, H.; Eisenthal, K. B. Chem. Phys. Lett. 1989, 160, 464. Lu, H.; Long, F. H.; Eisenthal, K. B. J. Opt. Soc. Am. B 1990, 7, 1511.
19. Long, F. H.; Lu, H.; Eisenthal, K. B. Chem. Phys. Lett. 1989, 160, 464. Lu, H.; Long, F. H.; Eisenthal, K. B. J. Opt. Soc. Am. B 1990, 7, 1511.
20. Hirata, Y.; Murata, N.; Tanioka, Y.; Malaga, N. J. Phys. Chem. 1989, 93, 4527. Hirata,Y.; Malaga, N. J. Phys. Chem. 1990, 94, 8503; 1991, 95, 9067.
21. Hirata, Y.; Murata, N.; Tanioka, Y.; Malaga, N. J. Phys. Chem. 1989, 93, 4527. Hirata,Y.; Malaga, N. J. Phys. Chem. 1990, 94, 8503; 1991, 95, 9067.
22. Hirata, Y.; Murata, N.; Tanioka, Y.; Malaga, N. J. Phys. Chem. 1989, 93, 4527. Hirata,Y.; Malaga, N. J. Phys. Chem. 1990, 94, 8503; 1991, 95, 9067.
23. Long, F. H.; Lu, H.; Eisenthal, K. B. Phys. Rev. Lett. 1990, 64, 1469.
24. Gauduel, Y.; Pommeret, S.; Migus, A.; Yamada, N.; Antonetti, A. J. Am. Chem. Soc. 1990, 112, 2925.
25. Gauduel, Y.; Pommeret, S.; Migus, A.; Antonetti, A. Chem. Phys. 1990. 149, 1.
26. Long, F. H.; Lu, H.; Shi, X.; Eisenthal, K. B. Chem. Phys. Lett. 1991. 185, 47.
27. Gauduel, Y.; Pommeret, S.; Migus, A.; Antonetti, A. J. Phys. Chem. 1991, 95, 533.
28. Pommeret, S.; Antonetti, A.; Gauduel, Y. J. Am. Chem. Soc. 1991, 113, 9105.
29. Pépin, C.; Houde, D.; Remita, H.; Goulet, T.; Jay-Gerin, J.-P. Phys. Rev. Lett. 1992, 69, 3389.
30. Sander, M.; Brummund, U.; Luther, K.; Troe, J. Ber. Bunsen-Ges. Phys. Chem. 1992, 96, 1486.
31. Gauduel, Y.; Pommeret, S.; Antonetti, A. J. Phys. Chem. 1993, 97, 134.
32. Alfano, J. C.; Walhout, P. K.; Kimura, Y.; Barbara, P. F. J. Chem. Phys. 1993, 98, 5996. Kimura, Y.; Alfano, J. C.; Walhout, P. K.; Barbara, P. F. J. Phys. Chem. 1994, 98, 3450.
33. Alfano, J. C.; Walhout, P. K.; Kimura, Y.; Barbara, P. F. J. Chem. Phys. 1993, 98, 5996. Kimura, Y.; Alfano, J. C.; Walhout, P. K.; Barbara, P. F. J. Phys. Chem. 1994, 98, 3450.
34. Hirata, Y.; Malaga, N. Prog. React. Kinet. 1993, 18, 273.
35. Pépin, C.; Houde, D.; Remita, H.; Goulet, T.; Jay-Gerin, J.-P. J. Chim. Phys. 1993, 90, 745. Houde, D.; Pépin, C.; Goulet, T.; Jay-Gerin, J.-P. In Mode-Locked and Solid State Lasers, Amplifiers, and Applications; Piché, M., Pace, P. W., Eds.; Proceedings of SPIE 2041; International Society for Optical Engineering: Bellingham, WA, 1993; pp 139-152.
36. Pépin, C.; Houde, D.; Remita, H.; Goulet, T.; Jay-Gerin, J.-P. J. Chim. Phys. 1993, 90, 745. Houde, D.; Pépin, C.; Goulet, T.; Jay-Gerin, J.-P. In Mode-Locked and Solid State Lasers, Amplifiers, and Applications; Piché, M., Pace, P. W., Eds.; Proceedings of SPIE 2041; International Society for Optical Engineering: Bellingham, WA, 1993; pp 139-152.
37. Pépin, C.; Goulet, T.; Houde, D.; Jay-Gerin, J.-P. J. Phys. Chem. 1994, 98, 7009.
38. McGowen, J. L.; Ajo, H. M.; Zhang, J. Z.; Schwanz, B. J. Chem. Phys. Lett. 1994, 231, 504.
39. Gauduel, Y. In Ultrafast Dynamics of Chemical Systems; Simon, J. D., Ed.; Kluwer Academic: Dordrecht, 1994; pp 81-136 and references therein.
40. Walhout, P. K.; Alfano, J. C.; Kimura, Y.; Silva, C.; Reid, P. J.; Barbara, P. F. Chem. Phys. Lett. 1995, 232, 135.
41. Shi, X.; Long, F. H.; Lu, H.; Eisenthal, K. B. J. Phys. Chem. 1995, 99, 6917.
42. Pépin, C.; Goulet, T.; Houde, D.; Jay-Gerin, J.-P. J. Chim. Phys. 1996, 93, 182.
43. Shi, X.; Long, F. H.; Lu, K; Eisenthal, K. B. J. Phys. Chem. 1996, 100, 11903.
44. Reuther, A.; Laubereau, A.; Nikogosyan, D. N. J. Phys. Chem. 1996, 100, 16794.
45. Zhang, X.; Jonah, C. D. Chem. Phys. Lett. 1996, 262, 649.
46. Jortner, J. Radiat. Res. Suppl. 1964, 4, 24.
47. Copeland, D. A.; Kestner, N. R.; Jortner, J. J. Chem. Phys. 1970, 53, 1189.
48. Webster, B. J. Phys. Chem. 1975, 79, 2809.
49. Schnitker, J.; Rossky, P. J.; Kenney-Wallace, G. A. J. Chem. Phys. 1986, 85, 2986.
50. Rips, I.; Klafter, J.; Jortner, J. J. Chem. Phys. 1988, 88, 3246, 89, 4288.
51. Rips, I.; Klafter, J.; Jortner, J. J. Chem. Phys. 1988, 88, 3246, 89, 4288.
52. Motakabbir, K. A.; Rossky, P. J. Chem. Phys. 1989, 129, 253. Motakabbir, K. A.; Schnitker, J.; Rossky, P. J. J. Chem. Phys. 1992, 97, 2055.
53. Motakabbir, K. A.; Rossky, P. J. Chem. Phys. 1989, 129, 253. Motakabbir, K. A.; Schnitker, J.; Rossky, P. J. J. Chem. Phys. 1992, 97, 2055.
54. Rossky, P. J.; Schnitker, J. J Phys. Chem. 1988, 92, 4277.
55. Barnett, R. N.; Landman, U.; Nitzan, A. J. Chem. Phys. 1989, 90, 4413.
56. Messmer, M. C.; Simon, J. D. J. Phys. Chem. 1990, 94, 1220.
57. Ferradini, C.; Jay-Gerin, J.-P. Chem. Phys. Lett. 1990, 167, 371.
58. Webster, F. J.; Schnitker, J.; Friedrichs, M. S.; Friesner, R. A.; Rossky, P. J. Phys. Rev. Lett. 1991, 66, 3172.
59. Neria, E.; Nitzan, A.; Barnett, R. N.; Landman, U. Phys. Rev. Lett. 1991, 67, 1011. Neria, E.; Nitzan, A. J. Chem. Phys. 1993, 99, 1109.
60. Neria, E.; Nitzan, A.; Barnett, R. N.; Landman, U. Phys. Rev. Lett. 1991, 67, 1011. Neria, E.; Nitzan, A. J. Chem. Phys. 1993, 99, 1109.
61. Jay-Gerin, J.-P.; Ferradini, C. Can. J. Chem. 1992, 70, 1869. Keszei, E.; Jay-Gerin, J.-P. Can. J. Chem. 1992, 70, 21.
62. Jay-Gerin, J.-P.; Ferradini, C. Can. J. Chem. 1992, 70, 1869. Keszei, E.; Jay-Gerin, J.-P. Can. J. Chem. 1992, 70, 21.
63. Murphrey, T. H.; Rossky, P. J. J. Chem. Phys. 1993, 99, 515.
64. Keszei, E.; Nagy, S.; Murphrey, T. H.; Rossky, P. J. J. Chem. Phys. 1993, 99, 2004.
65. Schwartz, B. J.; Rossky, P. J. J. Phys. Chem. 1994, 98, 4489. J. Chem. Phys. 1994, 101, 6902, 6917.
66. Schwartz, B. J.; Rossky, P. J. J. Phys. Chem. 1994, 98, 4489. J. Chem. Phys. 1994, 101, 6902, 6917.
67. Keszei, E.; Murphrey, T. H.; Rossky, P. J. J. Phys. Chem. 1995, 99, 22.
68. Staib, A.; Borgis, D. J. Chem. Phys. 1995, 103, 2642.
69. Schwartz, B. J.; Rossky, P. J. J. Phys Chem. 1995, 99, 2953.
70. Schwartz, B. J.; Rossky, P. J. J. Chem. Phys. 1996, 105, 6997.
71. Bratos, S.; Leicknam, J.-C1. Chem. Phys. Lett. 1996, 261, 117.
72. Prezhdo, O. V.; Rossky, P. J. J. Phys. Chem. 1996, 100, 17094.
73. Houée-Levin, C.; Jay-Gerin, J.-P. J. Phys. Chem. 1988, 92, 6454. Houée-Levin, C.; Tannous, C.; Jay-Gerin, J.-P. J. Phys. Chem. 1989, 93, 7074.
74. Houée-Levin, C.; Jay-Gerin, J.-P. J. Phys. Chem. 1988, 92, 6454. Houée-Levin, C.; Tannous, C.; Jay-Gerin, J.-P. J. Phys. Chem. 1989, 93, 7074.
75. Mozumder, A. Radiat. Phys. Chem. 1988, 32, 287.
76. Hilczer, M.; Tachiya, M. J. Phys. Chem. 1996, 100, 7691.
77. Goulet, T.; Jay-Gerin, J.-P. J. Chem. Phys. 1992, 96, 5076.
78. Goulet, T.; Mattéi, L.; Jay-Gerin, J.-P. Can. J. Phys. 1990, 68, 912.
79. Sander, M. U.; Luther, K.; Troe, J. Ber. Bunsen-Ges. Phys. Chem. 1993, 97, 953; J. Phys. Chem. 1993, 97, 11489.
80. Sander, M. U.; Luther, K.; Troe, J. Ber. Bunsen-Ges. Phys. Chem. 1993, 97, 953; J. Phys. Chem. 1993, 97, 11489.
81. Crowell, R. A.; Bartels, D. M. J. Phys. Chem. 1996, 100, 17713, 17940.
82. Pimblott, S. M. J. Phys. Chem. 1991, 95, 6946.
83. Jou, F.-Y.; Freeman, G. R. J. Phys. Chem. 1979, 83, 2383.
84. -1
85. Throughout this paper, the uncertainties that we give represent the 95% confidence intervals.
86. -1, where K is the thermal conductivity, ρ the density, and Cν the specific heat, one finds that the values of D in methanol and deuterated water differ by only 20%.
87. Maroncelli, M.; Fleming, G. R. J. Chem. Phys. 1987, 86, 6221.
88. Jarzeba, W.; Walker, G. C.; Johnson, A. E.; Kahlow, M. A.; Barbara, P. F. J. Phys. Chem. 1988, 92, 7039.
89. Bagchi, B.; Chandra, A. Chem. Phys. Lett. 1989, 155, 533.
90. Weaver, M. J.; McManis, G. E.; Jarzȩba, W.; Barbara, P. F. J. Phys. Chem. 1990, 94, 1715.
91. Walker, G. C.; Jarzeba, W.; Kang, T. J.; Johnson, A. E.; Barbara, P. F. J. Opt. Soc. Am. B 1990, 7, 1521.
92. Lin, Y.; Jonah, C. D. J. Phys. Chem. 1993, 97, 295.
93. Kivelson, D.; Friedman, H. J. Phys. Chem. 1989, 93, 7026.
94. See, for example: Baxendale, J. H.; Rasburn, E. J. J. Chem. Soc., Faraday Trans. 1 1974, 70, 705.
95. Barnett, R. N.; Landman, U.; Cleveland, C. L.; Jortner, J. J. Chem. Phys. 1988, 88, 4429.
96. Coe, J. V.; Lee, G. H.; Eaton, J. G.; Arnold, S. T.; Sarkas, H. W.; Bowen, K. H.; Ludewigt, C.; Habertand, H.; Worsnop, D. R. J. Chem. Phys. 1990, 92, 3980.
97. Ayotte, P.; Johnson, M. A. J. Chem. Phys. 1997, 106, 811.
98. + ion are only at a distance of a water molecule diameter at those times.
99. -:OH] triplet introduced in ref 24 can be found in: Pommeret, S. Ph.D. thesis, Université de Paris-Sud, Orsay, 1991.
100. - is left out.
101. Goulet, T.; Bernas, A.; Ferradini, C.; Jay-Gerin, J.-P. Chem. Phys. Lett. 1990, 170, 492.
102. Han, P.; Bartels, D. M. J Phys. Chem. 1990, 94, 5824.
103. See, for example: Madelung, O. Introduction to Solid-State Theory; Springer-Verlag: Berlin, 1978; pp 252-313.