In situ soft X-ray absorption spectroscopy applied to solid-liquid heterogeneous cyanopyrazine hydration reaction on titanium oxide catalyst

Journal of Physical Chemistry C

Volumn 119, Issue 14, 2015, Pages 7738-7745

  Yuzawa, Hayato ^a   Nagasaka, Masanari ^a,b   Kosugi, Nobuhiro ^a,b  

^a INSTITUTE FOR MOLECULAR SCIENCE   (Japan)

^b GRADUATE UNIVERSITY FOR ADVANCED STUDIES   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

ACTIVATION ANALYSIS; ACTIVATION ENERGY; CATALYSIS; CATALYSTS; HYDRATION; OXIDE MINERALS; RATE CONSTANTS; SPECTRUM ANALYSIS; SUBSTRATES; TITANIUM DIOXIDE; TITANIUM METALLOGRAPHY; X RAY ABSORPTION SPECTROSCOPY; X RAYS;

HETEROGENEOUS CATALYTIC REACTIONS; HYDRATION REACTION; IN-SITU SPECTROSCOPY; INNER SHELL EXCITATION; KINETIC PROPERTIES; LIQUID COMPONENTS; SOFT X-RAY ABSORPTION SPECTROSCOPIES; TEMPERATURE DEPENDENT;

LIQUIDS;

EID: 84927634667     PISSN: 19327447     EISSN: 19327455     Source Type: Journal    
DOI: 10.1021/jp512891t     Document Type: Article

References (46)

1. Zaera, F. Surface Chemistry at the Liquid/Solid Interface Surf. Sci. 2011, 605, 1141-1145
2. Zaera, F. Probing Liquid/Solid Interfaces at the Molecular Level Chem. Rev. 2012, 112, 2920-2986
3. Ellis, P. J.; Fairlamb, I. J. S.; Hackett, S. F. J.; Wilson, K.; Lee, A. F. Evidence for the Surface-Catalyzed Suzuki-Miyaura Reaction over Palladium Nanoparticles: An Operando XAS Study Angew. Chem., Int. Ed. 2010, 49, 1820-1824
4. Reimann, S.; Stötzel, J.; Frahm, R.; Kleist, W.; Grunwaldt, J.-D.; Baiker, A. Identification of the Active Species Generated from Supported Pd Catalysts in Heck Reactions: An in situ Quick Scanning EXAFS Investigation J. Am. Chem. Soc. 2011, 133, 3921-3930
5. Friebel, D.; Miller, D. J.; Nordlund, D.; Ogasawara, H.; Nilsson, A. Degradation of Bimetallic Model Electrocatalysts: An In Situ X-ray Absorption Spectroscopy Study Angew. Chem., Int. Ed. 2011, 50, 10190-10192
6. Karim, A. M.; Howard, C.; Roberts, B.; Kovarik, L.; Zhang, L.; King, D. L.; Wang, Y. In Situ X-ray Absorption Fine Structure Studies on the Effect of pH on Pt Electronic Density during Aqueous Phase Reforming of Glycerol ACS Catal. 2012, 2, 2387-2394
7. Bellière, V.; Lorentz, C.; Geantet, C.; Yoshimura, Y.; Laurenti, D.; Vrinat, M. Kinetics and Mechanism of Liquid-Phase Alkylation of 3-Methylthiophene with 2-Methyl-2-butene over a Solid Phosphoric acid Appl. Catal., B 2006, 64, 254-261
8. Huang, J.; Long, W.; Agrawal, P. K.; Jones, C. W. Effects of Acidity on the Conversion of the Model Bio-oil Ketone Cyclopentanone on H-Y Zeolites J. Phys. Chem. C 2009, 113, 16702-16710
9. Vjunov, A.; Hu, M. Y.; Feng, J.; Camaioni, D. M.; Mei, D.; Hu, J. Z.; Zhao, C.; Lercher, J. A. Following Solid-Acid-Catalyzed Reactions by MAS NMR Spectroscopy in Liquid Phase-Zeolite-Catalyzed Conversion of Cyclohexanol in Water Angew. Chem., Int. Ed. 2014, 53, 479-482
10. Andanson, J.-M.; Baiker, A. Exploring Catalytic Solid/Liquid Interfaces by In Situ Attenuated Total Reflection Infrared Spectroscopy Chem. Soc. Rev. 2010, 39, 4571-4584
11. 2 J. Phys. Chem. B 2002, 106, 10649-10658
12. Ferri, D.; Diezi, S.; Maciejewski, M.; Baiker, A. Alumina-Catalysed Degradation of Ethyl Pyruvate during Enantioselective Hydrogenation over Pt/Alumina and Its Inhibition by Acetic Acid Appl. Catal., A 2006, 297, 165-173
13. Ferri, D.; Baiker, A. Advances in Infrared Spectroscopy of Catalytic Solid-Liquid Interfaces: The Case of Selective Alcohol Oxidation Top. Catal. 2009, 52, 1323-1333
14. Aguirre, A.; Bonivardi, A. L.; Matkovic, S. R.; Briand, L. E.; Collins, S. E. ATR-FTIR Study of the Decomposition of Acetic Anhydride on Fosfotungstic Wells-Dawson Heteropoly Acid Using Concentration-Modulation Excitation Spectroscopy Top. Catal. 2011, 54, 229-235
15. Leinweber, P.; Kruse, J.; Walley, F. L.; Gillespie, A.; Eckhardt, K.-U.; Blyth, R. I. R.; Regier, T. Nitrogen K-edge XANES-An Overview of Reference Compounds Used to Identify 'Unknown' Organic Nitrogen in Environmental Samples J. Synchrotron Radiat. 2007, 14, 500-511
16. Marsh, A. L.; Burnett, D. J.; Fischer, D. A.; Gland, J. L. Benzene Intermediates and Mechanisms during Catalytic Oxidation on the Pt(111) Surface Using In-Situ Soft X-ray Methods J. Phys. Chem. B 2003, 107, 12472-12479
17. x/Au(1 1 1) Catalysts J. Catal. 2010, 271, 392-400
18. 2 Catalysts for Fischer-Tropsch Synthesis J. Phys. Chem. B 2004, 108, 16201-16207
19. Chantler, C. T. Detailed Tabulation of Atomic Form Factors, Photoelectric Absorption and Scattering Cross Section, and Mass Attenuation Coefficients in the Vicinity of Absorption Edges in the Soft X-ray (Z = 30-36, Z = 60-89, E = 0.1 keV-10 keV), Addressing Convergence Issues of Earlier Work J. Phys. Chem. Ref. Data 2000, 29, 597-1048
20. Schreck, S.; Gavrila, G.; Weniger, C.; Wernet, P. A Sample Holder for Soft X-ray Absorption Spectroscopy of Liquids in Transmission Mode Rev. Sci. Instrum. 2011, 82, 103101
21. Wernet, P.; Nordlund, D.; Bergmann, U.; Cavalleri, M.; Odelius, M.; Ogasawara, H.; Näslund, L.-Å.; Hirsch, T. K.; Ojamäe, L.; Glatzel, P. The Structure of the First Coordination Shell in Liquid Water Science 2004, 304, 995-999
22. Huang, C.; Wikfeldt, K. T.; Tokushima, T.; Nordlund, D.; Harada, Y.; Bergmann, U.; Niebuhr, M.; Weiss, T. M.; Horikawa, Y.; Leetmaa, M. The Inhomogeneous Structure of Water at Ambient Conditions Proc. Natl. Acad. Sci. U. S. A. 2009, 106, 15214-15218
23. Smith, J. D.; Cappa, C. D.; Wilson, K. R.; Messer, B. M.; Cohen, R. C.; Saykally, R. J. Energetics of Hydrogen Bond Network Rearrangements in Liquid Water Science 2004, 306, 851-853
24. Achkar, A. J.; Regier, T. Z.; Wadati, H.; Kim, Y.-J.; Zhang, H.; Hawthorn, D. G. Bulk Sensitive X-ray Absorption Spectroscopy Free of Self-Absorption Effects Phys. Rev. B 2011, 83, 081106(R)
25. 2+ Solution Using Inverse Partial and Partial Fluorescence Yield at the L-Edge J. Phys. Chem. Lett. 2012, 3, 1619-1623
26. Regier, T. Z.; Achkar, A. J.; Peak, D.; Tse, J. S.; Hawthorn, D. G. Dark Channel Fluorescence Observations Result from Concentration Effects Rather than Solvent-Solute Charge Transfer Nat. Chem. 2012, 4, 765-766
27. Soldatov, M. A.; Lange, K. M.; Gotz, M. D.; Engel, N.; Golnak, R.; Kothe, A.; Aziz, E. F. On the Origin of Dips in Total Fluorescence Yield X-ray Absorption Spectra: Partial and Inverse Partial Fluorescence Yield at the L-Edge of Cobalt Aqueous Solution Chem. Phys. Lett. 2012, 546, 164-167
28. Huse, N.; Wen, H.; Nordlund, D.; Szilagyi, E.; Daranciang, D.; Miller, T. A.; Nilsson, A.; Schoenlein, R. W.; Lindenberg, A. M. Probing the Hydrogen-Bond Network of Water via Time-Resolved Soft X-ray Spectroscopy Phys. Chem. Chem. Phys. 2009, 11, 3951-3957
29. Meibohm, J.; Schreck, S.; Wernet, P. Temperature Dependent Soft X-ray Absorption Spectroscopy of Liquids Rev. Sci. Instrum. 2014, 85, 103102
30. Nagasaka, M.; Hatsui, T.; Horigome, T.; Hamamura, Y.; Kosugi, N. Development of a Liquid Flow Cell to Measure Soft X-ray Absorption in Transmission Mode: a Test for Liquid Water J. Electron Spectrosc. Relat. Phenom. 2010, 177, 130-134
31. Nagasaka, M.; Mochizuki, K.; Leloup, V.; Kosugi, N. Local Structures of Methanol-Water Binary Solutions Studied by Soft X-ray Absorption Spectroscopy J. Phys. Chem. B 2014, 118, 4388-4396
32. Nagasaka, M.; Yuzawa, H.; Horigome, T.; Hitchcock, A. P.; Kosugi, N. Electrochemical Reaction of Aqueous Iron Sulfate Solutions Studied by Fe L-edge Soft X-ray Absorption Spectroscopy J. Phys. Chem. C 2013, 117, 16343-16348
33. Nagasaka, M.; Yuzawa, H.; Horigome, T.; Kosugi, N. In Operando Observation System for Electrochemical Reaction by Soft X-ray Absorption Spectroscopy with Potential Modulation Method Rev. Sci. Instrum. 2014, 85, 104105
34. Sugiyama, K.; Miura, H.; Nakano, Y.; Sekiwa, H.; Matsuda, T. Heterogeneous Hydration of Acrylonitrile over the Metal Oxide Catalysts in Liquid Phase Bull. Chem. Soc. Jpn. 1986, 59, 2983-2989
35. Yamaguchi, K.; Matsushita, M.; Mizuno, N. Efficient Hydration of Nitriles to Amides in Water, Catalyzed by Ruthenium Hydroxide Supported on Alumina Angew. Chem., Int. Ed. 2004, 43, 1576-1580
36. 2 Catalyst Appl. Catal., A 2005, 290, 175-180
37. 2 Catalyst Chem.-Eur. J. 2011, 17, 11428-11431
38. 2-Catalyzed Nitrile Hydration to Amide: Reaction Mechanism and Active Sites Catal. Sci. Technol. 2013, 3, 1386-1393
39. Hatsui, T.; Shigemasa, E.; Kosugi, N. Design of a Transmission Grating Spectrometer and an Undulator Beamline for Soft X-ray Emission Studies AIP Conf. Proc. 2004, 705, 921-924
40. 4 Probed by Electron Spectroscopy Chem. Phys. Lett. 1995, 236, 311-317
41. g Excited Nitrogen Clusters Phys. Rev. Lett. 2001, 86, 3767-3770
42. Aminpirooz, S.; Becker, L.; Hillert, B.; Haase, J. High Resolution NEXAFS Studies of Aromatic Molecules Adsorbed and Condensed on Ni(111) Surf. Sci. Lett. 1991, 244, L152-L156
43. Vall-llosera, G.; Gao, B.; Kivimäki, A.; Coreno, M.; álvarez Ruiz, J.; de Simone, M.; Ågren, H.; Rachlew, E. The C 1s and N 1s Near Edge X-ray Absorption Fine Structure Spectra of Five Azabenzenes in the Gas Phase J. Chem. Phys. 2008, 128, 044316
44. 3NCS J. Phys. Chem. 1989, 93, 3068-3077
45. Ikeura-Sekiguchi, H.; Sekiguchi, T.; Kitajima, Y.; Baba, Y. Inner Shell Excitation and Dissociation of Condensed Formamide Appl. Surf. Sci. 2001, 169-170, 282-286
46. Lessard, R.; Cuny, J.; Cooper, G.; Hitchcock, A. P. Inner-Shell Excitation of Gas Phase Carbonates and α,γ-Dicarbonyl Compounds Chem. Phys. 2007, 331, 289-303