State-resolved diffraction oscillations imaged for inelastic collisions of NO radicals with He, Ne and Ar

Nature Chemistry

Volumn 6, Issue 3, 2014, Pages 216-221

  Von Zastrow, Alexander ^a   Onvlee, Jolijn ^a   Vogels, Sjoerd N ^a   Groenenboom, Gerrit C ^a   Van Der Avoird, Ad ^a   Van De Meerakker, Sebastiaan Y T ^a  

^a RADBOUD UNIVERSITY NIJMEGEN   (Netherlands)

Author keywords

[No Author keywords available]

Indexed keywords

ARGON; HELIUM; NEON; NITRIC OXIDE;

ARTICLE; CHEMISTRY; QUANTUM THEORY; RADIATION SCATTERING;

ARGON; HELIUM; NEON; NITRIC OXIDE; QUANTUM THEORY; SCATTERING, RADIATION;

EID: 84895184915     PISSN: 17554330     EISSN: 17554349     Source Type: Journal    
DOI: 10.1038/nchem.1860     Document Type: Article

References (34)

1. Levine, R. D. & Bernstein, R. B. Molecular Reaction Dynamics and Chemical Reactivity (Oxford Univ. Press, 1987).
2. Lee, S-H. & Liu, K. in Modern Trends in Chemical Reaction Dynamics: Experiment and Theory Vol. 14, Part II, 1-42 (eds Yang, X. & Liu, K.) (World Scientific, 2004).
3. 2O + D. Science 333, 440-442 (2011).
4. Dong, W. et al. Transition-state spectroscopy of partial wave resonances in the F+HD reaction. Science 327, 1501-1502 (2010).
5. Chandler, D. W. & Houston, P. L. Two-dimensional imaging of state-selected photodissociation products detected by multiphoton ionization. J. Chem. Phys. 87, 1445-1447 (1987).
6. Eppink, A. T. J. B. & Parker, D. H. Velocity map imaging of ions and electrons using electrostatic lenses: application in photoelectron and photofragment ion imaging of molecular oxygen. Rev. Sci. Instrum. 68, 3477-3484 (1997). (Pubitemid 127665685)
7. Ashfold, M. N. R. et al. Imaging the dynamics of gas phase reactions. Phys. Chem. Chem. Phys. 8, 26-53 (2006).
8. Suits, A. G., Bontuyan, L. S., Houston, P. L. & Whitaker, B. J. Differential cross sections for state-selected products by direct imaging: Ar + NO. J. Chem. Phys. 96, 8618-8620 (1992).
9. Kohguchi, H., Suzuki, T. & Alexander, M. H. Fully state-resolved differential cross sections for the inelastic scattering of the open-shell NO molecule by Ar. Science 294, 832-834 (2001). (Pubitemid 33032096)
10. Townsend, D. et al. The roaming atom: straying from the reaction path in formaldehyde decomposition. Science 306, 1158-1161 (2004). (Pubitemid 39488989)
11. 2. Science 335, 1075-1078 (2012).
12. Lorenz, K. T. et al. Direct measurement of the preferred sense of NO rotation after collision with argon. Science 293, 2063-2066 (2001). (Pubitemid 32848050)
13. Eyles, C. J. et al. Interference structures in the differential cross-sections for inelastic scattering of NO by Ar. Nature Chem. 3, 597-602 (2011).
14. 4 reaction. Science 300, 966-969 (2003). (Pubitemid 36548881)
15. 3 preferentially promote reactivity toward the chlorine atom? Science 316, 1723-1726 (2007). (Pubitemid 46988542)
16. 3 reaction inhibits CH bond cleavage. Science 325, 303-306 (2009).
17. 3 with chlorine atom. Science 331, 900-903 (2011).
18. Mikosch, J. et al. Imaging nucleophilic substitution dynamics. Science 319, 183-186 (2008).
19. Lipciuc, M. L., Buijs, J. B. & Janssen, M. H. M. High resolution slice imaging of a molecular speed distribution. Phys. Chem. Chem. Phys. 8, 219-223 (2006).
20. Bethlem, H. L., Berden, G. & Meijer, G. Decelerating neutral dipolar molecules. Phys. Rev. Lett. 83, 1558-1561 (1999). (Pubitemid 129689776)
21. Van de Meerakker, S. Y. T., Bethlem, H. L., Vanhaecke, N. & Meijer, G. Manipulation and control of molecular beams. Chem. Rev. 112, 4828-4878 (2012).
22. Gilijamse, J. J., Hoekstra, S., van de Meerakker, S. Y. T., Groenenboom, G. C. & Meijer, G. Near-threshold inelastic collisions using molecular beams with a tunable velocity. Science 313, 1617-1620 (2006). (Pubitemid 44414031)
23. Kirste, M. et al. Quantum-state resolved bimolecular collisions of velocitycontrolled OH with NO radicals. Science 338, 1060-1063 (2012).
24. Faubel, M. The 'Fraunhofer theory' of rotational inelastic scattering of He on small molecules. J. Chem. Phys. 81, 5559-5569 (1984).
25. 2. J. Chem. Phys. 68, 5654-5655 (1978).
26. 2 anisotropic van der Waals potential. Test of a simple model using state-to-state differential scattering cross-sections. Faraday Discuss. Chem. Soc. 73, 205-220 (1982).
27. Casavecchia, P. in Dynamics of Polyatomic van der Waals Complexes (eds Halberstadt, N. & Janda, K. C.), 123-141 (Plenum, 1990).
28. Yonekura, N., Gebauer, Ch., Kohguchi, H. & Suzuki, T. A crossed molecular beam apparatus using high-resolution ion imaging. Rev. Sci. Instrum. 70, 3265-3270 (1999). (Pubitemid 129577246)
29. Aoiz, F. J., Verdasco, J. E., Herrero, V. J., Sáez Rábanos, V. & Alexander, M. H. Attractive and repulsive interactions in the inelastic scattering of NO by Ar: a comparison between classical trajectory and close-coupling quantum mechanical results. J. Chem. Phys. 119, 5860 (2003).
30. 2P) van der Waals complex: bound states and fully quantum and quasi-classical scattering. J. Chem. Phys. 137, 014312 (2012).
31. Warntjes, J. B. M., Robicheaux, F., Bakker, J. M. & Noordam, L. D. Autoionizing Rydberg states of NO in strong electric fields. J. Chem. Phys. 111, 2556-2564 (1999). (Pubitemid 129643547)
32. Yan, B. et al. A new high intensity and short-pulse molecular beam valve. Rev. Sci. Instrum. 84, 023102 (2013).
33. Gijsbertsen, A., Linnartz, H., Taatjes, C. A. & Stolte, S. Quantum interference as the source of steric asymmetry and parity propensity rules in NO-rare gas inelastic scattering. J. Am. Chem. Soc. 128, 8777-8789 (2006). (Pubitemid 44061536)
34. 2 inelastic collisions. Science 341, 1094-1096 (2013).