Removal of heavy metal ions from wastewater by a novel HEA/AMPS copolymer hydrogel: Preparation, characterization, and mechanism

Environmental Science and Pollution Research

Volumn 20, Issue 3, 2013, Pages 1511-1525

  Li, Zhengkui ^a   Wang, Yueming ^a   Wu, Ningmei ^a   Chen, Qichun ^a   Wu, Kai ^a  

^a NANJING UNIVERSITY   (China)

Author keywords

2 Acrylamido 2 methylpropane sulfonic (AMPS) acid; 2 Hydroxyethyl acrylate (HEA); Heavy metal adsorption; Multicomponent adsorption; Porous structure

Indexed keywords

ADSORPTION; CATION; EQUILIBRIUM; GEL; HEAVY METAL; ISOTHERM; NUMERICAL MODEL; PERMEABILITY; PH; POLLUTANT REMOVAL; POLYMER; POROUS MEDIUM; SEWAGE TREATMENT;

EID: 84874319679     PISSN: 09441344     EISSN: 16147499     Source Type: Journal    
DOI: 10.1007/s11356-012-0973-2     Document Type: Article

References (48)

1. Abdel-Halim ES, Al-Deyab SS (2011) Hydrogel from crosslinked polyacrylamide/guar gum graft copolymer for sorption of hexavalent chromium ion. Carbohyd Polym 86: 1306-1312.
2. Abdel-Halim ES, El-Rafie MH, Al-Deyab SS (2011) Polyacrylamide/guar gum graft copolymer for preparation of silver nanoparticles. Carbohyd Polym 85: 692-697.
3. Aguado J, Arsuaga JM, Arencibia A, Lindo M, Gascon V (2009) Aqueous heavy metals removal by adsorption on amine-functionalized mesoporous silica. J Hazard Mater 163: 213-221.
4. Ali I (2010) The quest for active carbon adsorbent substitutes: inexpensive adsorbents for toxic metal ions removal from wastewater. Sepn Purfn Rev 39: 95-171.
5. Ali I, Gupta VK (2006) Advances in water treatment by adsorption technology. Nat Protoco 1: 2661-2667.
6. Bozkurt A, Ekinci O, Meyer WH (2003) Synthesis and characterization of proton-conducting copolymers on the basis of vinylpyrrolidone and acrylamido sulfonic acid. J Appl Polym Sci 90: 3347-3353.
7. Cao J, Tan Y, Che Y, Xin H (2010) Novel complex gel beads composed of hydrolyzed polyacrylamide and chitosan: an effective adsorbent for the removal of heavy metal from aqueous solution. Bioresour Technol 101: 2558-2561.
8. 3 catalysts. Appl Catal B-Environ 96: 307-313.
9. El-Hag Ali A, Shawky HA, Abd El Rehim HA, Hegazy EA (2003) Synthesis and characterization of PVP/AAc copolymer hydrogel and its applications in the removal of heavy metals from aqueous solution. Eur Polym J 39: 2337-2344.
10. Essawy HA, Ibrahim HS (2004) Synthesis and characterization of poly (vinylpyrrolidone-co-methylacrylate) hydrogel for removal and recovery of heavy metal ions from wastewater. React Funct Polym 61: 421-432.
11. Freudlich H (1907) Ueber die adsorption in Loesungen. J Phys Chem C 7: 385-470.
12. Gupta VK, Ali I (2000) Utilisation of bagasse fly ash (a sugar industry waste) for the removal of copper and zinc from wastewater. Sepn Purifn Technol 18: 131-140.
13. Gupta VK, Ali I (2004) Removal of lead and chromium from wastewater using bagasse fly ash-a sugar industry waste. J Colloid Interf Sci 271: 321-328.
14. Gupta VK, Rastogi A (2008a) A Sorption and desorption studies of chromium (VI) from nonviable cyano bacterium Nostoc muscorum biomass. J Hazard Mater 154: 347-354.
15. Gupta VK, Rastogi A (2008b) Equilibrium and kinetic modelling of cadmium(II) biosorption by nonliving algal biomass Oedogonium sp. from aqueous phase. J Hazard Mater 153: 759-766.
16. Gupta VK, Rastogi A (2009) Biosorption of hexavalent chromium by raw and acid-treated green alga Oedogonium hatei from aqueous solutions. J Hazard Mater 163: 396-402.
17. Gupta VK, Suhas (2009) Application of low cost adsorbents for dye removal-a review. J Environ Manage 90: 2313-2342.
18. Gupta VK, Mohan D, Sharma S, Park KT (1999) Removal of chromium(VI) from electroplating industry wastewater using bagasse fly ash-a sugar industry waste material. Environmentalist 19: 129-136.
19. Gupta VK, Gupta M, Sharma S (2001) Process development for the removal of lead and chromium from aqueous solutions using red mud-an aluminum industry waste. Water Res 35: 1125-1134.
20. Gupta VK, Jain CK, Ali I, Sharma M, Saini VK (2003) Removal of cadmium and nickel from wastewater using bagasse fly ash-a sugar industry waste. Water Res 37: 4038-4044.
21. Gupta VK, Mittal A, Gajbe V, Mittal J (2006a) Removal and recovery of the hazardous azo dye acid orange 7 through adsorption over waste materials: bottom ash and de-oiled soya. Ind Eng Chem Res 45: 1446-1453.
22. Gupta VK, Mittal A, Kurup L, Mittal J (2006b) Adsorption of a hazardous dye, erythrosine, over hen feathers. J Colloid Interf Sci 304: 52-57.
23. Gupta VK, Ali I, Saini VK (2007a) Adsorption studies on the removal of Vertigo Blue 49 and Orange DNA13 from aqueous solutions using carbon slurry developed from a waste material. J Colloid Interf Sci 315: 87-93.
24. 2 catalyst. J Colloid Interf Sci 309: 464-469.
25. Gupta VK, Jain R, Varshney S (2007c) Electrochemical removal of the hazardous dye Reactofix Red 3 BFN from industrial effluents. Colloid Interf Sci 312: 292-296.
26. Gupta VK, Carrott PJM, Ribeiro Carrott MML (2009) Low cost adsorbents: growing approach to wastewater treatment-a review. Crit Rev Env Sci Tec 39: 783-842.
27. Gupta VK, Rastogi A, Nayak A (2010) Adsorption studies on the removal of hexavalent chromium from aqueous solution using a low cost fertilizer industry waste material. J Colloid Interf Sci 342: 135-141.
28. Gupta VK, Saleh TA, Ali I, Nayak A, Agarwal S (2012) Chemical treatment technologies for waste-water recycling-an overview. RSC Adv. doi: 10. 1039/C2RA20340E.
29. Huang F, Zheng Y, Yang Y (2007) Study on macromolecular metal complexes: synthesis, characterization, and fluorescence properties of stoichiometric complexes for rare earth coordinated with poly (acrylic acid). J Appl Polym Sci 103: 351-357.
30. 2+ removal: equilibrium, kinetics, thermodynamics and regeneration studies. J Hazard Mater 174: 746-755.
31. Ju XJ, Zhang SB, Zhou MY, Xie R, Yang L, Chu LY (2009) Novel heavy metal adsorption material: ion-recognition P(NIPAM-co-BCAm) hydrogels for removal of lead(II) ions. J Hazard Mater 167: 114-118.
32. Kasgoz H, Ozgumus S, Orbay M (2003) Modified polyacrylamide hydrogels and their application in removal of heavy metal ions. Polymer 44: 1785-1793.
33. Kok Yetimoglu E, Kahraman MV, Ercan O, Akdemir ZS, Kayaman Apohan N (2007) N-vinylpyrrolidone/acrylic acid/2-acrylamido-2-methylpropane sulfonic acid based hydrogels: synthesis, characterization and their application in the removal of heavy metals. React Funct Polym 67: 451-460.
34. Langmuir I (1918) The adsorption of gases on plane surfaces of glass, mica and platinum. J Am Chem Soc 40: 1361-1403.
35. Miretzky P, Saralegui A, Cirelli AF (2006) Simultaneous heavy metal removal mechanism by dead macrophytes. Chemosphere 62: 247-254.
36. Mohan S, Sreelakshmi G (2008) Fixed bed column study for heavy metal removal using phosphate treated rice husk. J Hazard Mater 153: 75-82.
37. Ngah WS, Kamari A, Koay YJ (2004) Equilibrium and kinetics studies of adsorption of copper (II) on chitosan and chitosan/PVA beads. Int J Biol Macromol 34: 155-161.
38. Osifo PO, Webster A, van der Merwe H, Neomagus HW, van der Gun MA, Grant DM (2008) The influence of the degree of cross-linking on the adsorption properties of chitosan beads. Bioresour Technol 99: 7377-7382.
39. Pourjavadi A, Barzegar S (2009) Synthesis and evaluation of pH and thermosensitive pectin-based superabsorbent hydrogel for oral drug delivery systems. Starch 61: 161-172.
40. Rivas BL, Castro A (2003) Preparation and adsorption properties of resins containing amine, sulfonic acid, and carboxylic acid moieties. J Appl Polym Sci 90: 700-705.
41. Rueda CJ, Komber H, Cedron JC, Voit B, Shevtsova G (2003) Synthesis of new hydrogels by copolymerization of poly (2-methyl-2-oxazoline) bis (macromonomers) and N-vinylpyrrolidone. Macromol Chem Phys 204: 947-953.
42. Saleh TA, Gupta VK (2012) Column with CNT/magnesium oxide composite for lead (II) removal from water. Environ Sci Pollut Res 19: 1224-1228.
43. Srivastava SK, Gupta VK, Mohan D (1997) Removal of lead and chromium by activated slag-a blast-furnace waste. J Environ Eng 123: 461-468.
44. Wang Q, Xie X, Zhang X, Zhang J, Wang A (2010) Preparation and swelling properties of pH-sensitive composite hydrogel beads based on chitosan-g-poly (acrylic acid)/vermiculite and sodium alginate for diclofenac controlled release. Int J Biol Macromol 46: 356-362.
45. Yildi U, Kemika OF, Hazerb B (2010) The removal of heavy metal ions from aqueous solutions by novel pH-sensitive hydrogels. J Hazard Mater 183: 521-532.
46. Zhao Y, Su H, Fang L, Tan T (2005) Superabsorbent hydrogels from poly (aspartic acid) with salt-, temperature- and pH-responsiveness properties. Polymer 46: 5368-5376.
47. Zheng Y, Wang A (2010) Removal of heavy metals using polyvinyl alcohol semi-IPN poly (acrylic acid)/tourmaline composite optimized with response surface methodology. Chem Eng J 162: 186-193.
48. 2+ recovery. Anal Chim Acta 687: 193-200.