Principles of sustained enzymatic hydrogen oxidation in the presence of oxygen -the crucial influence of high potential Fe-S clusters in the electron relay of [NiFe]-hydrogenases

Journal of the American Chemical Society

Volumn 135, Issue 7, 2013, Pages 2694-2707

  Evans, Rhiannon M ^a   Parkin, Alison ^a   Roessler, Maxie M ^a,b   Murphy, Bonnie J ^a   Adamson, Hope ^a   Lukey, Michael J ^a   Sargent, Frank ^c   Volbeda, Anne ^d   Fontecilla Camps, Juan C ^d   Armstrong, Fraser A ^a,b  

^a Department of Chemistry ^*  (United Kingdom)

^b Centre for Advanced Electron Spin Resonance   (United Kingdom)

^c UNIVERSITY OF DUNDEE   (United Kingdom)

^d CNRS   (France)

Author keywords

[No Author keywords available]

Indexed keywords

[NIFE]-HYDROGENASE; ACTIVE SITE; ELECTROCATALYTIC ACTIVITY; ELECTRON RELAY; ELECTRON-RICH; HIGH POTENTIAL; HYDROGEN OXIDATION; HYDROGENASES; IRREVERSIBLE INACTIVATION; OXIDATION ACTIVITIES; POTENTIOMETRIC TITRATIONS; PROTEIN FILMS; RICH PICTURE; SPECIAL CLASS; TOLERANCE MECHANISMS;

CATALYTIC OXIDATION; ENZYMES; ESCHERICHIA COLI; HYDROGEN; NICKEL; OXIDATION; TITRATION;

ELECTRONS;

ENZYME VARIANT; HYDROGEN; HYDROGENASE; IRON; NICKEL; OXIDOREDUCTASE; OXYGEN; SULFUR;

ARTICLE; CATALYSIS; ELECTROCHEMISTRY; ELECTRON TRANSPORT; ENZYME ACTIVE SITE; ENZYME ACTIVITY; ENZYME MECHANISM; ENZYME STRUCTURE; ESCHERICHIA COLI; NONHUMAN; OXIDATION; POTENTIOMETRIC TITRATION; PROTEIN FILM ELECTROCHEMISTRY; REACTION ANALYSIS; REDUCTION;

AMINO ACID SEQUENCE; CRYSTALLOGRAPHY, X-RAY; ESCHERICHIA COLI; GENETIC VARIATION; HYDROGEN; HYDROGENASE; IRON-SULFUR PROTEINS; MODELS, BIOLOGICAL; MOLECULAR SEQUENCE DATA; OXIDATION-REDUCTION; OXYGEN; SEQUENCE ALIGNMENT;

EID: 84874101282     PISSN: 00027863     EISSN: 15205126     Source Type: Journal    
DOI: 10.1021/ja311055d     Document Type: Article

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