High temporal resolution Br2, BrCl and BrO observations in coastal Antarctica

Atmospheric Chemistry and Physics

Volumn 13, Issue 3, 2013, Pages 1329-1343

  Buys, Z ^a,b   Brough, N ^a   Huey, L G ^c   Tanner, D J ^c   Von Glasow, R ^b   Jones, A E ^a  

^a BRITISH ANTARCTIC SURVEY   (United Kingdom)

^b UNIVERSITY OF EAST ANGLIA   (United Kingdom)

^c GEORGIA INSTITUTE OF TECHNOLOGY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

AIR MASS; ATMOSPHERIC CHEMISTRY; BROMINE COMPOUND; HALOGEN; IMAGE RESOLUTION; MASS SPECTROMETRY; MASS TRANSPORT; MIXING RATIO; OZONE DEPLETION; PHOTOLYSIS; POLAR REGION;

ANTARCTICA; BELLINGSHAUSEN SEA; SOUTHERN OCEAN;

EID: 84873639584     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-13-1329-2013     Document Type: Article

References (53)

1. Abbatt, J. P. D.: Heterogeneous reaction of HOBr with HBr and HCl on ice surfaces at 228 K, Geophys. Res. Lett., 21, 665-668, doi:10.1029/94GL00775, 1994. (Pubitemid 24406046)
2. Abbatt, J. P. D., Thomas, J. L., Abrahamsson, K., Boxe, C., Gran-fors, A., Jones, A. E., King, M. D., Saiz-Lopez, A., Shep-son, P. B., Sodeau, J., Toohey, D. W., Toubin, C., von Glasow, R., Wren, S. N., and Yang, X.: Halogen activation via interactions with environmental ice and snow in the polar lower troposphere and other regions, Atmos. Chem. Phys., 12, 6237-6271, doi:10.5194/acp-12-6237-2012, 2012.
3. Adams, J. W., Holmes, N. S., and Crowley, J. N.: Uptake and reaction of HOBr on frozen and dry NaCl/NaBr surfaces between 253 and 233K, Atmos. Chem. Phys., 2, 79-91, doi:10.5194/acp-2-79-2002, 2002.
4. Anderson, P. S. and Neff, W. D.: Boundary layer physics over snow and ice, Atmos. Chem. Phys., 8, 3563-3582, doi:10.5194/acp-8-3563-2008, 2008.
5. 5OH from 50 to 500 torr, J. Phys. Chem. A 105, 3527-3531, 2001.
6. Barrie, L. A., Bottenheim, J. W., Schnell, R. C., Crutzen, P. J., and Rasmussen, R. A.: Ozone Destruction and Photochemical-Reactions at Polar Sunrise in the Lower Arctic Atmosphere, Nature, 334, 138-141, 1988. (Pubitemid 19296595)
7. 4 Int. J. Mass Spec-trom., 202, 91-109, 2000.
8. ? N Latitude, Geophys. Res. Lett., 13, 113-116, 1986.
9. Bromwich, D. H., Carrasco J. F., and Turner J.: A Downward Developing Mesoscale Cyclone Over the Ross Ice Shelf During Winter, Global Atmos. Ocean Syst., 4, 125-147, 1996. (Pubitemid 29303401)
10. Damian, V., Sandu, A., Damien, M., Potra, F., and Carmichael, G. R.: The kinetic preprocessor kpp-a software environment for solving chemical kinetics, Comp. Chem. Eng., 26, 1567-1579, 2002. (Pubitemid 35192177)
11. Draxler, R. R. and Rolph, G. D.: HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website (http://ready.arl.noaa.gov/HYSPLIT. php), NOAA Air Resources Laboratory, Silver Spring, MD, 2012.
12. 2 and BrCl via uptake of HOBr onto aqueous salt solutions, J. Geophys. Res., 104, 23719-23727, doi:10.1029/1999JD900359, 1999.
13. 2 and BrCl in surface ozone destruction at polar sunrise Science, Science, 291, 471-474, 2001. (Pubitemid 32097068)
14. Gilman, J. B., Burkhart, J. F., Lerner, B. M., Williams, E. J., Kuster, W. C., Goldan, P. D., Murphy, P. C., Warneke, C., Fowler, C., Montzka, S. A., Miller, B. R., Miller, L., Oltmans, S. J., Ry-erson, T. B., Cooper, O. R., Stohl, A., and de Gouw, J. A.: Ozone variability and halogen oxidation within the Arctic and sub-Arctic springtime boundary layer, Atmos. Chem. Phys., 10, 10223-10236, doi:10.5194/acp-10-10223-2010, 2010.
15. - with Atmospheric Trace Gases, J. Phys. Chem., 99, 5001-5008, doi:10.1021/j100014a021, 1995.
16. 3 in air with a chemical ionization mass spectrometer, J. Geophys. Res.-Atmos., 103, 3355-3360, 1998. (Pubitemid 28392512)
17. 2 at the South Pole during ISCAT 2000, Atmos. Environ., 38, 5411-5421, doi:10.1016/j.atmosenv.2004.04.037, 2004. (Pubitemid 39185845)
18. Jacobi, H.-W., Morin, S., and Bottenheim, J. W.: Observation of widespread depletion of ozone in the springtime boundary layer of the central Arctic linked to mesoscale synoptic conditions, J. Geophys. Res., 115, D17302, doi:10.1029/2010JD013940, 2010.
19. Jones, A. E., Anderson, P. S., Wolff, E. W., Turner, J., Rankin, A. M., and Colwell, S. R.: A role for newly forming sea ice in springtime polar tropospheric ozone loss? Observational evidence from Halley station, Antarctica, J. Geophys. Res., 111, D08306, doi:10.1029/2005JD006566, 2006.
20. Jones, A. E., Wolff, E. W., Salmon, R. A., Bauguitte, S. J.-B., Roscoe, H. K., Anderson, P. S., Ames, D., Clemitshaw, K. C., Fleming, Z. L., Bloss, W. J., Heard, D. E., Lee, J. D., Read, K. A., Hamer, P., Shallcross, D. E., Jackson, A. V., Walker, S. L., Lewis, A. C., Mills, G. P., Plane, J. M. C., Saiz-Lopez, A., Sturges, W. T., and Worton, D. R.: Chemistry of the Antarctic Boundary Layer and the Interface with Snow: an overview of the CHABLIS campaign, Atmos. Chem. Phys., 8, 3789-3803, doi:10.5194/acp-8-3789-2008, 2008.
21. Jones, A. E., Anderson, P. S., Begoin, M., Brough, N., Hutterli, M. A., Marshall, G. J., Richter, A., Roscoe, H. K., and Wolff, E. W.: BrO, blizzards, and drivers of polar tropospheric ozone depletion events, Atmos. Chem. Phys., 9, 4639-4652, doi:10.5194/acp-9-4639-2009, 2009.
22. Kirchner, U., Benter, T. H., and Schindler, R. N.: Experimental verification of gas phase bromine enrichment in reactions of HOBr with sea salt doped ice surfaces, Ber. Bunsen Ges. Phys. Chem., 101, 975-977, 1997. (Pubitemid 127746066)
23. König-Langlo, G., King, J. C., and Pettre, P.: Climatology of the three coastal Antarctic stations Dumont d'Urville, Neu-mayer, and Halley, J. Geophys. Res.-Atmos., 103, 10935-10946, doi:10.1029/97jd00527, 1998. (Pubitemid 128718599)
24. Kreher, K., Keys, J. G., Johnston, P. V., Platt, U., and Liu, X.: Ground-based measurements of OClO and HCl in austral spring 1993 at Arrival Heights, Antarctica, Geophys. Res. Lett., 23, 1545-1548, doi:10.1029/96gl01318, 1996.
25. Kreher, K., Johnston, P. V., Wood, S. W., Nardi, B., and Platt, U.: Ground-based measurements of tropospheric and stratospheric BrO at Arrival Heights, Antarctica, Geophys. Res. Lett., 24, 3021-3024, doi:10.1029/97gl02997, 1997. (Pubitemid 127686527)
26. Landgraf, J. and Crutzen, P. J.: An Efficient Method for Online Calculations of Photolysis and Heating Rates, J. Atmos. Sci., 55, 863-878, doi:10.1175/1520-0469(1998)0552.0.CO;2, 1998.
27. Leibrock, E. and Huey, L. G.: Ion chemistry for the detection of isoprene and other volatile organic compounds in ambient air, Geophys. Res. Lett., 27, 1719-1722, 2000. (Pubitemid 32040465)
28. Liao, J., Huey, L. G., Tanner, D. J., Brough, N., Brooks, S., Dibb, J. E., Stutz, J., Thomas, J. L., Lefer, B., Haman, C., and Gorham, K.: Observations of hydroxyl and peroxy radicals and the impact of BrO at Summit, Greenland in 2007 and 2008, Atmos. Chem. Phys., 11, 8577-8591, doi:10.5194/acp-11-8577-2011, 2011a.
29. Liao, J., Sihler, H., Huey, L. G., Neuman, J. A., Tanner, D. J., Friess, U., Platt, U., Flocke, F. M., Orlando, J. J., Shepson, P. B., Beine, H. J., Weinheimer, A. J., Sjostedt, S. J., Nowak, J. B., Knapp, D. J., Staebler, R. M., Zheng, W., Sander, R., Hall, S. R., and Ullmann, K.: A comparison of Arctic BrO measurements by chemical ionization mass spectrometry and long path-differential optical absorption spectroscopy, J. Geophys. Res.-Atmos., 116, D00r02, doi:10.1029/2010jd014788, 2011b.
30. Liao, J., Huey, L. G., Scheuer, E., Dibb, J. E., Stickel, R. E., Tanner, D.J., Neuman, J. A., Nowak, J. B., Choi, S., Wang, Y., Salawitch, R. J., Canty, T., Chance, K., Kurosu, T., Suleiman, R., Weinheimer, A. J., Shetter, R. E., Fried, A., Brune, W., Anderson, B., Zhang, X., Chen, G., Crawford, J., Hecobian, A., and Ingall, E.D.: Characterization of soluble bromide measurements and a case study of BrO observations during ARCTAS, Atmos. Chem. Phys., 12, 1327-1338, doi:10.5194/acp-12-1327-2012, 2012a.
31. 2) speciation at Barrow, Alaska, in spring 2009, J. Geophys. Res., 117, D00R16, doi:10.1029/2011JD016641, 2012b.
32. Neuman, J. A., Nowak, J. B., Huey, L. G., Burkholder, J. B., Dibb, J. E., Holloway, J. S., Liao, J., Peischl, J., Roberts, J. M., Ryer-son, T. B., Scheuer, E., Stark, H., Stickel, R. E., Tanner, D. J., and Weinheimer, A.: Bromine measurements in ozone depleted air over the Arctic Ocean, Atmos. Chem. Phys., 10, 6503-6514, doi:10.5194/acp-10-6503-2010, 2010.
33. Oltmans, S. J.: Surface Ozone Measurements in Clean Air, J. Geo-phys. Res., 86, 1174-1180, 1981.
34. Piot, M. and von Glasow, R.: The potential importance of frost flowers, recycling on snow, and open leads for ozone depletion events, Atmos. Chem. Phys., 8, 2437-2467, doi:10.5194/acp-8-2437-2008, 2008.
35. Pöhler, D., Vogel, L., Friess, U., and Platt, U.: Observation of halogen species in the Amundsen Gulf, Arctic, by active long-path differential optical absorption spectroscopy, P. Natl. Acad. Sci. USA, 107, 6582-6587, doi:10.1073/pnas.0912231107, 2010.
36. Rankin, A. M. and Wolff, E. W.: A year-long record of size-segregated aerosol composition at Halley, Antarctica, J. Geo-phys. Res.-Atmos., 108, 4775, doi:10.1029/2003jd003993, 2003.
37. Rankin, A. M., Wolff, E. W., and Martin, S.: Frost flowers: Implications for tropospheric chemistry and ice core interpretation, J. Geophys. Res.-Atmos., 107, 4683, doi:10.1029/2002jd002492, 2002. (Pubitemid 43197276)
38. 3 to 12km altitude during the summer monsoon season over New Mexico, J. Geophys. Res., 99, 25529-25534, doi:10.1029/94JD02210, 1994.
39. Rolph, G. D.: Real-time Environmental Applications and Display system (READY) Website (http://ready.arl.noaa.gov), NOAA Air Resources Laboratory, Silver Spring, MD, 2012.
40. Roscoe, H. K. and Roscoe, J.: Polar tropospheric ozone depletion events observed in the International Geophysical Year of 1958, Atmos. Chem. Phys., 6, 3303-3314, doi:10.5194/acp-6-3303-2006, 2006. (Pubitemid 44221575)
41. Saiz-Lopez, A., Mahajan, A. S., Salmon, R. A., Bauguitte, S. J. B., Jones, A. E., Roscoe, H. K., and Plane, J. M. C.: Boundary layer halogens in coastal Antarctica, Science, 317, 348-351, doi:10.1126/science.1141408, 2007. (Pubitemid 47106370)
42. Simpson, W. R., von Glasow, R., Riedel, K., Anderson, P., Ariya, P., Bottenheim, J., Burrows, J., Carpenter, L. J., Frieß, U., Good-site, M. E., Heard, D., Hutterli, M., Jacobi, H.-W., Kaleschke, L., Neff, B., Plane, J., Platt, U., Richter, A., Roscoe, H., Sander, R., Shepson, P., Sodeau, J., Steffen, A., Wagner, T., and Wolff, E.: Halogens and their role in polar boundary-layer ozone depletion, Atmos. Chem. Phys., 7, 4375-4418, doi:10.5194/acp-7-4375-2007, 2007. (Pubitemid 47325998)
43. Sjostedt, S. J. and Abbatt, J. P. D.: Release of gas-phase halogens from sodium halide substrates: heterogeneous oxidation of frozen solutions and dessicated salts by hydroxyl radicals, Environ. Res. Lett., 3, 045007, doi:10.1088/1748-9326/3/4/045007, 2008.
44. Slusher, D. L., Pitteri, S. J., Haman, B. J., Tanner, D. J., and Huey, L. G.: A chemical ionization technique for measurement of per-nitric acid in the upper troposphere and the polar boundary layer, Geophys. Res. Lett., 28, 3875-3878, 2001. (Pubitemid 33056413)
45. Slusher, D. L., Huey, L. G., Tanner, D. J., Flocke, F. M., and Roberts, J. M.: A thermal dissociation-chemical ionization mass spectrometry (td-cims) technique for the simultaneous measurement of peroxyacyl nitrates and dinitrogen pentoxide, J. Geo-phys. Res., 109, D19315, doi:10.1029/2004JD004670, 2004. (Pubitemid 39660694)
46. Spicer, C. W., Plastridge, R. A., Foster, K. L., Finlayson-Pitts, B. J., Bottenheim, J. W., Grannas, A. M., and Shepson, P. B.: Molecular halogens before and during ozone depletion events in the Arctic at polar sunrise: concentrations and sources, Atmos. Environ., 36, 2721-2731, 2002. (Pubitemid 34628362)
47. Spreen, G., Kaleschke, L., and Heygster, G.: Sea ice remote sensing using AMSR-E 89-GHz channels, J. Geophys. Res.-Oceans, 113, C02s03, doi:10.1029/2005jc003384, 2008.
48. Toyota, K., McConnell, J. C., Lupu, A., Neary, L., McLinden, C. A., Richter, A., Kwok, R., Semeniuk, K., Kaminski, J. W., Gong, S.-L., Jarosz, J., Chipperfield, M. P., and Sioris, C. E.: Analysis of reactive bromine production and ozone depletion in the Arctic boundary layer using 3-D simulations with GEM-AQ: inference from synoptic-scale patterns, Atmos. Chem. Phys., 11, 3949-3979, doi:10.5194/acp-11-3949-2011, 2011.
49. von Glasow, R., Sander, R., Bott, A., and Crutzen, P. J.: Modeling halogen chemistry in the marine boundary layer-1. Cloud-free MBL, J. Geophys. Res.-Atmos., 107, 4341, doi:10.1029/2001JD000942, 2002. (Pubitemid 43206147)
50. Wesely, M. L.: Parameterization of surface resistances to gaseous dry deposition in regional-scale numerical models, Atmos. Environ., 23, 1293-1304, 1989.
51. Wessel, S., Aoki, S., Winkler, P., Weller, R., Herber, A., Gernandt, H., and Schrems, O.: Tropospheric ozone depletion in polar regions-A comparison of observations in the Arctic and Antarctic, Tellus B, 50, 34-50, 1998.
52. Wilson, K. L. and Birks, J. W.: Mechanism and Elimination of a Water Vapour Interference in the Measurement of Ozone by UV Absorbance, Environ. Sci. Technol., 40, 6361-6367, doi:10.1021/es052590c, 2006. (Pubitemid 44630902)
53. Yang, X., Pyle, J. A., and Cox, R. A.: Sea salt aerosol production and bromine release: Role of snow on sea ice, Geophys. Res. Lett., 35, L16815, doi:10.1029/2008GL034536, 2008.