SMX degradation by ozonation and UV radiation: A kinetic study

Chemosphere

Volumn 87, Issue 10, 2012, Pages 1134-1140

  Liu, Xiaowei ^a   Garoma, Temesgen ^b   Chen, Zhonglin ^a   Wang, Lili ^a   Wu, Youxian ^b  

^a HARBIN INSTITUTE OF TECHNOLOGY   (China)

^b AGC Paul S Roel Chair in Construction Engineering and Management   (United States)

Author keywords

Kinetic model; Operational parameters; Ozonation; SMX; UV radiation

Indexed keywords

ALKALINITY; IONIC STRENGTH; KINETIC PARAMETERS; KINETIC THEORY; OZONE WATER TREATMENT; OZONIZATION; RATE CONSTANTS; SULFUR COMPOUNDS; ULTRAVIOLET RADIATION; WATER QUALITY;

DOMINANT FACTOR; KINETIC MODELING; OPERATIONAL PARAMETERS; PSEUDO-FIRST ORDER KINETIC MODEL; SECOND-ORDER RATE CONSTANTS; SULFAMETHOXAZOLE (SMX); UV DEGRADATION; UV LIGHT INTENSITY;

OZONE;

BICARBONATE; HUMIC ACID; NITRATE; OZONE; SULFAMETHOXAZOLE; SULFATE; WATER;

HUMIC ACID; IONIC COMPOSITION; LIGHT INTENSITY; OZONE; PH; REACTION KINETICS; ULTRAVIOLET RADIATION;

ACIDITY; ALKALINITY; AQUEOUS SOLUTION; ARTICLE; CONCENTRATION (PARAMETERS); CONTROLLED STUDY; DRUG DEGRADATION; IONIC STRENGTH; LIGHT INTENSITY; OZONATION; RADIATION DOSE; ULTRAVIOLET RADIATION; WATER QUALITY;

EID: 84862802115     PISSN: 00456535     EISSN: 18791298     Source Type: Journal    
DOI: 10.1016/j.chemosphere.2012.02.007     Document Type: Article

References (53)

1. Andreozzi R., Marotta R. Ozonation of p-chlorophenol in aqueous solution. J. Hazard. Mater. 1999, 69:303-317.
2. Andreozzi R., Canterino M., Marotta R., Paxeus N. Antibiotic removal from wastewaters: the ozonation of amoxicillin. J. Hazard. Mater. 2005, 122:243-250.
3. APHA Standard Methods for Examination of Water and Wastewater 1998, American Public Health Association, Washington, DC.
4. Bader H., Hoigne J. Determination of ozone in water by the indigo method. Water Res. 1981, 15:449-456.
5. Beltran F.J. Ozone Reaction Kinetics for Water and Wastewater Systems 2004, Lewis Publishers, Boca Raton, FL. first ed.
6. Beltran F.J., Aguinaco A., Garcia-Araya J.F. Mechanism and kinetics of sulfamethoxazole photocatalytic ozonation in water. Water Res. 2009, 43:1359-1369.
7. Beltran F.J., Pocostales P., Alvarez P.M., Lopez-Pineiro F. Catalysts to improve the abatement of sulfamethoxazole and the resulting organic carbon in water during ozonation. Appl. Catal. B-Environ. 2009, 92:262-270.
8. Boreen A.L., Arnold W.A., McNeill K. Photochemical fate of sulfa drugs in the aquatic environment: Sulfa drugs containing five-membered heterocyclic groups. Environ. Sci. Technol. 2004, 38:3933-3940.
9. Buchanan W., Roddick F., Porter N., Drikas M. Enhanced biodegradability of UV and VUV pre-treated natural organic matter. Water Sci. Tech. Water Supply 2004, 4:103-111.
10. Buchanan W., Roddick F., Porter N., Drikass M. Fractionation of UV and VUV pretreated natural organic matter from drinking water. Environ. Sci. Technol. 2005, 39:4647-4654.
11. Burns R.A., Crittenden J.C., Hand D.W., Selzer V.H., Sutter L.L., Salman S.R. Effect of inorganic ions in heterogeneous photocatalysis of TCE. J. Environ. Eng. 1999, 125:77.
12. -) in aqueous solution. J. Phys. Chem. Ref. Data 1988, 17:513-886.
13. Chin Y.P., Miller P.L., Zeng L., Cawley K., Weavers L.K. Photosensitized degradation of bisphenol A by dissolved organic matter. Environ. Sci. Technol. 2004, 38:5888-5894.
14. Dantas R.F., Contreras S., Sans C., Esplugas S. Sulfamethoxazole abatement by means of ozonation. J. Hazard. Mater. 2008, 150:790-794.
15. Dodd M.C., Buffle M.O., Von Gunten U. Oxidation of antibacterial molecules by aqueous ozone: Moiety-specific reaction kinetics and application to ozone-based wastewater treatment. Environ. Sci. Technol. 2006, 40:1969-1977.
16. Drewes J.E., Heberer T., Rauch T., Reddersen K. Fate of pharmaceuticals during ground water recharge. Ground Water Monit. Remed. 2003, 23:64-72.
17. 2) treatment. J. Hazard. Mater. 2009, 164:640-645.
18. 3/UV Process. Environ. Sci. Technol. 2004, 38:5246-5252.
19. Garoma T., Umamaheshwar S., Mumper A. Removal of sulfadiazine, sulfamethizole, sulfamethoxazole, and sulfathiazole from aqueous solution by ozonation. Chemosphere 2010, 79:814-820.
20. Gonzalez M.C., Braun A.M. VUV photolysis of aqueous-solution of nitrate and nitrite. Res. Chem. Intermed. 1995, 21:837-859.
21. Guittonneau S., Thibaudeau D., Meallier P. Free radicals formation induced by the ozonation of humic substances in aqueous medium. Catal. Today 1996, 29:323-327.
22. Hassan I., Robinson C.W. Mass transfer coefficients in mechanically agitated gas-aqueous electrolyte dispersions. Can. J. Chem. Eng. 1980, 58:198-205.
23. Hatchard C., Parker C. A new sensitive chemical actinometer. II. Potassium ferrioxalate as a standard chemical actinometer. Proc. R. Soc. Lond. A Math. Phys. Sci. 1956, 235:518-536.
24. Hirsch R., Ternes T., Haberer K., Mehlich A., Ballwanz F., Kratz K. Determination of antibiotics in different water compartments via liquid chromatography-electrospray tandem mass spectrometry. J. Chromatogr. A 1998, 815:213-223.
25. Hirsch R., Ternes T., Haberer K., Kratz K.-L. Occurrence of antibiotics in the aquatic environment. Sci. Total. Environ. 1999, 225:109-118.
26. Hoigne J., Bader H., Haag W.R., Staehelin J. Rate constants of reactions of ozone with organic and inorganic compounds in water. III. Inorganic compounds and radicals. Water Res. 1985, 19:993-1004.
27. Huber M.M., Canonica S., Park G.Y., Von Gunten U. Oxidation of pharmaceuticals during ozonation and advanced oxidation processes. Environ. Sci. Technol. 2003, 37:1016-1024.
28. Jiang, J., 2009. Characteristics and Mechanism for Oxidative Degradation of Typical Organic Compounds in Aqueous Solution by High Valent Manganese and Iron Species. PhD thesis, Harbin Institute of Technology, Harbin.
29. Kim S.D., Cho J., Kim I.S., Vanderford B.J., Snyder S.A. Occurrence and removal of pharmaceuticals and endocrine disruptors in South Korean surface, drinking, and waste waters. Water Res. 2007, 41:1013-1021.
30. 2 processes for the removal of pharmaceuticals detected in secondary effluent of a sewage treatment plant in Japan. J. Hazard. Mater. 2009, 166:1134-1140.
31. 2 treatments. Chemosphere 2009, 77:518-525.
32. Kimura K., Toshima S., Amy G., Watanabe Y. Rejection of neutral endocrine disrupting compounds (EDCs) and pharmaceutical active compounds (PhACs) by RO membranes. J. Membrane Sci. 2004, 245:71-78.
33. Lam M., Tantuco K., Mabury S. PhotoFate: a new approach in accounting for the contribution of indirect photolysis of pesticides and pharmaceuticals in surface waters. Environ. Sci. Technol 2003, 37:899-907.
34. Larsson D.G.J., de Pedro C., Paxeus N. Effluent from drug manufactures contains extremely high levels of pharmaceuticals. J. Hazard. Mater. 2007, 148:751-755.
35. Leo A., Hansch C., Elkins D. Partition coefficients and their uses. Chem. Rev. 1971, 71:525-616.
36. Liu Y., Shen J., Chen Z., Yang L., Han Y. Effects of amorphous-zinc-silicate-catalyzed ozonation on the degradation of p-chloronitrobenzene in drinking water. Appl. Catal. A-Gen. 2011, 403:112-118.
37. 2 degradations of pharmaceutical intermediates in aqueous solution. J. Photochem. Photobiol. Chem. 2003, 156:121-126.
38. Ma J., Graham N. Degradation of atrazine by manganese-catalysed ozonation: Influence of humic substances. Water Res. 1999, 33:785-793.
39. Martinez Bueno M.J., Aguera A., Gomez M.J., Hernando M.D., Garcia-Reyes J.F., Fernandez-Alba A.R. Application of liquid chromatography/quadrupole-linear Ion trap mass spectrometry and time-of-flight mass spectrometry to the determination of pharmaceuticals and related contaminants in wastewater. Anal. Chem. 2007, 79:9372-9384.
40. max=254nm). J. Hazard. Mater. 2011, 186:67-75.
41. Ngouyap Mouamfon M.V., Li W., Lu S., Qiu Z., Chen N., Lin K. Photodegradation of sulphamethoxazole under UV-light irradiation at 254nm. Environ. Technol. 2010, 31:489-494.
42. Nicolle L.E. Urinary tract infection: Traditional pharmacologic therapies. Am. J. Med. 2002, 113:35-44.
43. Staehelin J., Hoigne J. Decomposition of ozone in water in the presence of organic solutes acting as promoters and inhibitors of radical chain reactions. Environ. Sci. Technol. 1985, 19:1206-1213.
44. Tercero Espinoza L.A., Neamtu M., Frimmel F.H. The effect of nitrate, Fe(III) and bicarbonate on the degradation of bisphenol A by simulated solar UV-irradiation. Water Res. 2007, 41:4479-4487.
45. Ternes T., Stuber J., Herrmann N., McDowell D., Ried A., Kampmann M., Teiser B. Ozonation: a tool for removal of pharmaceuticals, contrast media and musk fragrances from wastewater?. Water Res. 2003, 37:1976-1982.
46. Trovo A.G., Nogueira R.F.P., Aguera A., Sirtori C., Fernadez-Alba A.R. Photodegradation of sulfamethoxazole in various aqueous media: Persistence, toxicity and photoproducts assessment. Chemosphere 2009, 77:1292-1298.
47. Vione D., Falletti G., Maurino V., Minero C., Pelizzetti E., Malandrino M., Ajassa R., Olariu R.-I., Arsene C. Sources and sinks of hydroxyl radicals upon irradiation of natural water samples. Environ. Sci. Technol. 2006, 40:3775-3781.
48. Walter M.V., Vennes J.W. Occurrence of multiple-antibiotic-resistant enteric bacteria in domestic sewage and oxidation lagoons. Appl. Environ. Microb. 1985, 50:930-933.
49. Westerhoff, P., 1995. Ozone oxidation of bromide and natural organic matter. PhD thesis, University of Colorado.
50. Westerhoff P., Yoon Y., Snyder S., Wert E. Fate of endocrine-disruptor, pharmaceutical, and personal care product chemicals during simulated drinking water treatment processes. Environ. Sci. Technol. 2005, 39:6649-6663.
51. Xiong F., Graham N. Removal of atrazine through ozonation in the presence of humic substances. Ozone Sci. Eng. 1992, 14:263-268.
52. Xu W., Zhang G., Li X., Zou S., Li P., Hu Z., Li J. Occurrence and elimination of antibiotics at four sewage treatment plants in the Pearl River Delta (PRD). South China. Water Res. 2007, 41:4526-4534.
53. Zuccato E., Calamari D., Natangelo M., Fanelli R. Presence of therapeutic drugs in the environment. Lancet 2000, 355:1789-1790.