Mechanistic insight into the N=N bond-cleavage of Azo-compounds that was induced by an Al-Al-bonded compound [L 2-Al II-Al IIL 2-]

Chemistry - A European Journal

Volumn 18, Issue 19, 2012, Pages 6022-6030

  Zhao, Yanxia ^a,d   Liu, Yanyan ^a   Yang, Ling ^b,c   Yu, Jian Guo ^c   Li, Shaoguang ^a,d   Wu, Biao ^a   Yang, Xiao Juan ^a  

^a LANZHOU INSTITUTE OF CHEMICAL PHYSICS   (China)

^b HARBIN INSTITUTE OF TECHNOLOGY   (China)

^c BEIJING NORMAL UNIVERSITY   (China)

^d UNIVERSITY OF CHINESE ACADEMY OF SCIENCES   (China)

Author keywords

aluminum; azo compounds; cleavage reactions; reaction mechanisms; reduction

Indexed keywords

AZO COMPOUND; CLEAVAGE REACTION; DFT CALCULATION; DIANIONIC LIGANDS; DIANIONS; DIIMINE LIGAND; DOUBLE BONDS; MONOANIONS; MULTI-ELECTRON; REACTION MECHANISM; REACTION PROCESS; REDUCTANTS; REDUCTIVE CLEAVAGE;

DENSITY FUNCTIONAL THEORY; LIGANDS; REDUCTION; SODIUM COMPOUNDS;

ALUMINUM;

EID: 84860742385     PISSN: 09476539     EISSN: 15213765     Source Type: Journal    
DOI: 10.1002/chem.201103607     Document Type: Article

References (58)

1. J. Du Bois, C. S. Tomooka, J. Hong, E. M. Carreira, Acc. Chem. Res. 1997, 30, 364-372.
2. K. Kaleta, P. Arndt, T. Beweries, A. Spannenberg, O. Theilmann, U. Rosenthal, Organometallics 2010, 29, 2604-2609
3. W. J. Evans, C. A. Traina, J. W. Ziller, J. Am. Chem. Soc. 2009, 131, 17473-17481
4. W. H. Monillas, G. P. A. Yap, L. A. MacAdams, K. H. Theopold, J. Am. Chem. Soc. 2007, 129, 8090-8091
5. P. L. Diaconescu, P. L. Arnol, T. A. Baker, D. J. Mindiola, C. C. Cummins, J. Am. Chem. Soc. 2000, 122, 6108-6109
6. W. J. Evans, K. A. Miller, J. W. Ziller, Angew. Chem. 2008, 120, 599-602
7. Angew. Chem. Int. Ed. 2008, 47, 589-592
8. Y.-C. Tsai, P.-Y. Wang, K.-M. Lin, S.-A. Chen, J.-M. Chen, Chem. Commun. 2008, 205-207
9. F. A. Cotton, S. A. Duraj, W. J. Roth, J. Am. Chem. Soc. 1984, 106, 4749-4751.
10. S. S. Sen, D. Kratzert, D. Stern, H. W. Roesky, D. Stalke, Inorg. Chem. 2010, 49, 5786-5788.
11. R. J. Wright, M. Brynda, J. C. Fettinger, A. R. Betzer, P. P. Power, J. Am. Chem. Soc. 2006, 128, 12498-12509.
12. S. J. Bonyhady, S. P. Green, C. Jones, S. Nembenna, A. Stasch, Angew. Chem. 2009, 121, 3017-3021
13. Angew. Chem. Int. Ed. 2009, 48, 2973-2977.
14. C. Cui, M. M. Olmstead, J. C. Fettinger, G. H. Spikes, P. P. Power, J. Am. Chem. Soc. 2005, 127, 17530-17541.
15. K. Takeuchi, M. Ichinohe, A. Sekiguchi, J. Am. Chem. Soc. 2011, 133, 12478-12481.
16. W. Uhl, Z. Naturforsch. B 1988, 43, 1113-1118.
17. N. Wiberg, K. Amelunxen, T. Blank, H. Noth, J. Knizek, Organometallics 1998, 17, 5431-5433.
18. R. J. Wehmschulte, K. Ruhlandt-Senge, M. M. Olmstead, H. Hope, B. E. Sturgeon, P. P. Power, Inorg. Chem. 1993, 32, 2983-2984.
19. R. J. Wright, M. Brynda, P. P. Power, Angew. Chem. 2006, 118, 6099-6102
20. Angew. Chem. Int. Ed. 2006, 45, 5953-5956.
21. S. G. Minasian, J. Arnold, Chem. Commun. 2008, 4043-4045.
22. S. J. Bonyhady, D. Collis, G. Frenking, N. Holzmann, C. Jones, A. Stasch, Nat. Chem. 2010, 2, 865-869.
23. K. R. Compaan, J. J. Wilke, H. F. Schaefer, J. Am. Chem. Soc. 2011, 133, 13387-13396.
24. R. J. Wright, A. D. Phillips, P. P. Power, J. Am. Chem. Soc. 2003, 125, 10784-10785.
25. W. Uhl, Coord. Chem. Rev. 1997, 163, 1-32.
26. Y. Mori, Y. Kumakura, Y. Sugahara, J. Organomet. Chem. 2006, 691, 4289-4296
27. Y. Saito, Y. Sugahara, K. Kuroda, J. Am. Ceram. Soc. 2004, 83, 2436-2440.
28. A. Y. Timoshkin, Coord. Chem. Rev. 2005, 249, 2094-2131
29. W. Uhl, A. Vogelpohl, Eur. J. Inorg. Chem. 2009, 93-97
30. W. Uhl, T. Abel, A. Hepp, T. Nilges, F. Rogel, E.-U. Würthwein, N. Ghavtadze, Inorg. Chem. 2009, 48, 752-759
31. W. Uhl, T. Abel, A. Hepp, S. Grimme, M. Steinmetz, Eur. J. Inorg. Chem. 2008, 543-551.
32. R. J. Wright A. D. Phillips T. L. Allen W. H. Fink, P. P. Power, J. Am. Chem. Soc. 2003, 125, 1694-1695.
33. H. Zhu, J. Chai, H. Fan, H. W. Roesky, U. N. Nehete, H.-G. Schmidt, M. Noltemeyer, Eur. J. Inorg. Chem. 2005, 2147-2150.
34. X.-J. Yang, J. Yu, Y. Liu, Y. Xie, H. F. Schaefer, Y. Liang, B. Wu, Chem. Commun. 2007, 2363-2365
35. Y. Liu, S. Li, X.-J. Yang, P. Yang, B. Wu, J. Am. Chem. Soc. 2009, 131, 4210-4211.
36. Y. Liu, P. Yang, J. Yu, X.-J. Yang, J. D. Zhang, Z. Chen, H. F. Schaefer, B. Wu, Organometallics 2008, 27, 5830-5835.
37. J. Yu, X.-J. Yang, Y. Liu, Z. Pu, Q.-S. Li, Y. Xie, H. F. Schaefer, B. Wu, Organometallics 2008, 27, 5800-5805
38. Y. Liu, S. Li, X.-J. Yang, P. Yang, J. Gao, Y. Xia, B. Wu, Organometallics 2009, 28, 5270-5272
39. P. Yang, X.-J. Yang, J. Yu, Y. Liu, C. Zhang, Y.-H. Deng, B. Wu, Dalton Trans. 2009, 5773-5779
40. Y. Liu, Y. Zhao, X.-J. Yang, S. Li, J. Gao, P. Yang, Y. Xia, B. Wu, Organometallics 2011, 30, 1599-1606.
41. E. K. Styron, C. H. Lake, D. H. Powell, C. L. Watkins, L. K. Krannich, Polyhedron 2002, 21, 1747-1753
42. R. J. Wehmschulte, P. P. Power, J. Am. Chem. Soc. 1996, 118, 791-797
43. C. J. Carmalt, J. D. Mileham, A. J. P. White, D. J. Williams, Organometallics 2003, 22, 1554-1557.
44. S. P. Green, C. Jones, A. Stasch, Angew. Chem. 2008, 120, 9219-9223
45. Angew. Chem. Int. Ed. 2008, 47, 9079-9083.
46. S. Schulz, L. Häming, R. Herbst-Irmer, H. W. Roesky, G. M. Sheldrick, Angew. Chem. 1994, 106, 1052-1054
47. Angew. Chem. Int. Ed. Engl. 1994, 33, 969-970.
48. J. D. Fisher, P. J. Shapiro, G. P. A. Yap, A. L. Rheingold, Inorg. Chem. 1996, 35, 271-272.
49. R. D. Davy, H. F. Schaefer, Inorg. Chem. 1998, 37, 2291-2295.
50. G. Fochi, C. Floriani, J. Chem. Soc. Dalton Trans. 1983, 1515-1521.
51. Z. Padělková, M. S. Nechaev, A. Lyčka, J. Holubová, T. A. Zevaco, A. Růžička, Eur. J. Inorg. Chem. 2009, 2058-2061.
52. R. J. Doedens, J. A. Ibers, Inorg. Chem. 1969, 8, 2709-2714.
53. Y. Ohki, Y. Takikawa, T. Hatanaka, K. Tatsumi, Organometallics 2006, 25, 3111-3113.
54. P. v. R. Schleyer, C. Maerker, A. Dransfeld, H. Jiao, N. J. R. v. E. Hommes, J. Am. Chem. Soc. 1996, 118, 6317-6318
55. Z. Chen, C. S. Wannere, C. Corminboeuf, R. Puchta, P. v. R. Schleyer, Chem. Rev. 2005, 105, 3842-3888.
56. H. A. Zhong, J. A. Labinger, J. E. Bercaw, J. Am. Chem. Soc. 2002, 124, 1378-1399.
57. G. M. Sheldrick, Program SADABS: Area-Detector Absorption Correction; University of Göttingen, Göttingen, Germany, 1996.
58. G. M. Sheldrick, SHELXS-97 and SHELXL-97, Programs for Crystal Structure Analysis; University of Göttingen, Göttingen, Germany, 1997.