Nature and structure of aluminum surface sites grafted on silica from a combination of high-field aluminum-27 solid-state NMR spectroscopy and first-principles calculations

Journal of the American Chemical Society

Volumn 134, Issue 15, 2012, Pages 6767-6775

  Kerber, Rachel Nathaniel ^a   Kermagoret, Anthony ^b   Callens, Emmanuel ^b,c   Florian, Pierre ^d   Massiot, Dominique ^d   Lesage, Anne ^b   Copéret, Christophe ^b,e   Delbecq, Françoise ^a   Rozanska, Xavier ^a,f   Sautet, Philippe ^a  

^a UNIVERSITÉ DE LYON   (France)

^b UNIVERSITÉ LYON 1   (France)

^c KING ABDULLAH UNIVERSITY OF SCIENCE AND TECHNOLOGY   (Saudi Arabia)

^d UNIVERSITÉ D'ORLÉANS   (France)

^e ETH ZURICH   (Switzerland)

^f Materials Design   (France)

Author keywords

[No Author keywords available]

Indexed keywords

ALKYLALUMINUM; ALUMINUM COCATALYST; ALUMINUM SURFACE; ASYMMETRIC PARAMETERS; DINUCLEAR; FIRST-PRINCIPLES CALCULATION; HIGH QUALITY; HIGH-FIELD; ISOTROPIC CHEMICAL SHIFTS; KEYPOINTS; LARGE SURFACE AREA; METHYLALUMINOXANE; QUADRUPOLAR COUPLING; SILICA MATRIX; SILICA SURFACE; SOLID-STATE NMR SPECTROSCOPY; STABLE FIELDS; STRUCTURE OF SURFACES; SURFACE SITES; TETRAHEDRAL SITES; TRIETHYLALUMINUM; ULTRA-FAST;

CALCULATIONS; CHEMICAL MODIFICATION; GRAFTING (CHEMICAL); MAGIC ANGLE SPINNING; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; SILICA; SOLID STATE PHYSICS;

ALUMINUM;

ALUMINUM; SILICON DIOXIDE;

ARTICLE; CALCULATION; CHEMICAL STRUCTURE; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; PROTON NUCLEAR MAGNETIC RESONANCE; SOLID STATE;

EID: 84859991550     PISSN: 00027863     EISSN: 15205126     Source Type: Journal    
DOI: 10.1021/ja3008566     Document Type: Article

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