-
2
-
-
0242383973
-
-
Kobayashi, N.; Ogata, H.; Nonaka, N.; Luk'yanets, E. A. Chem. - Eur. J. 2003, 9, 5123-5134
-
(2003)
Chem. - Eur. J.
, vol.9
, pp. 5123-5134
-
-
Kobayashi, N.1
Ogata, H.2
Nonaka, N.3
Luk'yanets, E.A.4
-
3
-
-
78149244690
-
-
E970
-
Peng, X.; Draney, D. R.; Volcheck, W. M.; Bashford, G. R.; Lamb, D. T.; Grone, D. L.; Zhang, Y.; Johnson, C. M. Proc. SPIE 2006, 6097 E970
-
(2006)
Proc. SPIE
, vol.6097
-
-
Peng, X.1
Draney, D.R.2
Volcheck, W.M.3
Bashford, G.R.4
Lamb, D.T.5
Grone, D.L.6
Zhang, Y.7
Johnson, C.M.8
-
4
-
-
0001686369
-
-
Lippel, P. H.; Wilson, R. J.; Miller, M. D.; Wöll, C.; Chiang, S. Phys. Rev. Lett. 1989, 62, 171-174
-
(1989)
Phys. Rev. Lett.
, vol.62
, pp. 171-174
-
-
Lippel, P.H.1
Wilson, R.J.2
Miller, M.D.3
Wöll, C.4
Chiang, S.5
-
5
-
-
0027690405
-
-
Watanabe, F.; Mcclelland, G. M.; Heinzelmann, H. Science 1992, 262, 1244-1247
-
(1992)
Science
, vol.262
, pp. 1244-1247
-
-
Watanabe, F.1
McClelland, G.M.2
Heinzelmann, H.3
-
6
-
-
77951941816
-
-
Pan, S.; Zhao, A.; Wang, B.; Yang, J.; Hou, J. Adv. Mater. 2010, 22, 1967-1971
-
(2010)
Adv. Mater.
, vol.22
, pp. 1967-1971
-
-
Pan, S.1
Zhao, A.2
Wang, B.3
Yang, J.4
Hou, J.5
-
7
-
-
77951550074
-
-
Wang, Y. F.; Kröger, J.; Berndt, R.; Vázquez, H.; Brandbyge, M.; Paulsson, M. Phys. Rev. Lett. 2010, 104, 176802
-
(2010)
Phys. Rev. Lett.
, vol.104
, pp. 176802
-
-
Wang, Y.F.1
Kröger, J.2
Berndt, R.3
Vázquez, H.4
Brandbyge, M.5
Paulsson, M.6
-
8
-
-
4544370376
-
-
Wu, S. W.; Nazin, G. V.; Chen, X.; Qiu, X. H.; Ho, W. Phys. Rev. Lett. 2004, 93, 236802
-
(2004)
Phys. Rev. Lett.
, vol.93
, pp. 236802
-
-
Wu, S.W.1
Nazin, G.V.2
Chen, X.3
Qiu, X.H.4
Ho, W.5
-
9
-
-
34547853629
-
-
Mikaelian, G.; Ogawa, N.; Tu, X. W.; Ho, W. J. Chem. Phys. 2006, 124, 131101
-
(2006)
J. Chem. Phys.
, vol.124
, pp. 131101
-
-
Mikaelian, G.1
Ogawa, N.2
Tu, X.W.3
Ho, W.4
-
11
-
-
0000762326
-
-
Kerp, H. R.; Donker, H.; Koehorst, R. B. M.; Schaafsma, T. J.; van Faassen, E. E. Chem. Phys. Lett. 1998, 298, 302-308
-
(1998)
Chem. Phys. Lett.
, vol.298
, pp. 302-308
-
-
Kerp, H.R.1
Donker, H.2
Koehorst, R.B.M.3
Schaafsma, T.J.4
Van Faassen, E.E.5
-
13
-
-
67650745416
-
-
023305
-
Kim, I.; Haverinen, H. M.; Wang, Z.; Madakuni, S.; Li, J.; Jabbour, G. E. Appl. Phys. Lett. 2009, 95 023305
-
(2009)
Appl. Phys. Lett.
, vol.95
-
-
Kim, I.1
Haverinen, H.M.2
Wang, Z.3
Madakuni, S.4
Li, J.5
Jabbour, G.E.6
-
14
-
-
75149174639
-
-
Xi, X.; Meng, Q.; Li, F.; Ding, Y.; Ji, J.; Shi, Z.; Li, G. Sol. Energy Mater. Sol. Cells 2010, 94, 623-628
-
(2010)
Sol. Energy Mater. Sol. Cells
, vol.94
, pp. 623-628
-
-
Xi, X.1
Meng, Q.2
Li, F.3
Ding, Y.4
Ji, J.5
Shi, Z.6
Li, G.7
-
15
-
-
21844450216
-
-
Nazeeruddin, Md. K.; Humphry-Baker, R.; Grätzel, M.; Murrer, B. A. Chem. Commun. 1998, 719-720
-
(1998)
Chem. Commun.
, pp. 719-720
-
-
Nazeeruddin, Md.K.1
Humphry-Baker, R.2
Grätzel, M.3
Murrer, B.A.4
-
16
-
-
1942521169
-
-
Clifford, J. N.; Palomares, E.; Nazeeruddin, Md. K.; Grätzel, M.; Nelson, J.; Li, X.; Long, N. J.; Durrant, J. R. J. Am. Chem. Soc. 2004, 126, 5225-5233
-
(2004)
J. Am. Chem. Soc.
, vol.126
, pp. 5225-5233
-
-
Clifford, J.N.1
Palomares, E.2
Nazeeruddin, Md.K.3
Grätzel, M.4
Nelson, J.5
Li, X.6
Long, N.J.7
Durrant, J.R.8
-
17
-
-
20444439555
-
-
Levitsky, I. A.; Euler, W. B.; Tokranova, N.; Xu, B.; Castracane, J. Appl. Phys. Lett. 2004, 85, 6245-6247
-
(2004)
Appl. Phys. Lett.
, vol.85
, pp. 6245-6247
-
-
Levitsky, I.A.1
Euler, W.B.2
Tokranova, N.3
Xu, B.4
Castracane, J.5
-
18
-
-
0042225050
-
-
Tamarat, Ph.; Maali, A.; Lounis, B.; Orrit, M. J. Phys. Chem. B 2000, 104, 1-16
-
(2000)
J. Phys. Chem. B
, vol.104
, pp. 1-16
-
-
Tamarat, Ph.1
Maali, A.2
Lounis, B.3
Orrit, M.4
-
19
-
-
18844423055
-
-
Tinnefeld, P.; Sauer, M. Angew. Chem., Int. Ed. 2005, 44, 2642-2671
-
(2005)
Angew. Chem., Int. Ed.
, vol.44
, pp. 2642-2671
-
-
Tinnefeld, P.1
Sauer, M.2
-
20
-
-
33646937406
-
-
Michalet, X.; Weiss, S.; Jäger, M. Chem. Rev. 2006, 106, 1785-1813
-
(2006)
Chem. Rev.
, vol.106
, pp. 1785-1813
-
-
Michalet, X.1
Weiss, S.2
Jäger, M.3
-
21
-
-
67650269841
-
-
Wöll, D.; Braeken, E.; Deres, A.; De Schryver, F. C.; Uji-i, H.; Hofkens, J. Chem. Soc. Rev. 2009, 38, 313-328
-
(2009)
Chem. Soc. Rev.
, vol.38
, pp. 313-328
-
-
Wöll, D.1
Braeken, E.2
Deres, A.3
De Schryver, F.C.4
Uji-I, H.5
Hofkens, J.6
-
22
-
-
0038674868
-
-
Bosman, A. W.; Janssen, H. M.; Meijer, E. W. Chem. Rev. 1999, 99, 1665-1688
-
(1999)
Chem. Rev.
, vol.99
, pp. 1665-1688
-
-
Bosman, A.W.1
Janssen, H.M.2
Meijer, E.W.3
-
23
-
-
77951234285
-
-
Astruc, D.; Boisselier, E.; Ornelas, C. Chem. Rev. 2010, 110, 1857-1959
-
(2010)
Chem. Rev.
, vol.110
, pp. 1857-1959
-
-
Astruc, D.1
Boisselier, E.2
Ornelas, C.3
-
24
-
-
0021586266
-
-
Tomalia, D. A.; Baker, H.; Dewald, J.; Hall, M.; Kallos, G.; Martin, S.; Roeck, J.; Ryder, J.; Smith, P. Polymer J. 1985, 17, 117-132
-
(1985)
Polymer J.
, vol.17
, pp. 117-132
-
-
Tomalia, D.A.1
Baker, H.2
Dewald, J.3
Hall, M.4
Kallos, G.5
Martin, S.6
Roeck, J.7
Ryder, J.8
Smith, P.9
-
25
-
-
0034696613
-
-
Wang, J.; Chen, J.; Jia, X.; Cao, W.; Li, M. Chem. Commun. 2000, 511-512
-
(2000)
Chem. Commun.
, pp. 511-512
-
-
Wang, J.1
Chen, J.2
Jia, X.3
Cao, W.4
Li, M.5
-
26
-
-
0036062532
-
-
Wang, J.; Jia, X.; Zhong, H.; Luo, Y.; Zhao, X.; Cao, W.; Li, M. Chem. Mater. 2002, 14, 2854-2858
-
(2002)
Chem. Mater.
, vol.14
, pp. 2854-2858
-
-
Wang, J.1
Jia, X.2
Zhong, H.3
Luo, Y.4
Zhao, X.5
Cao, W.6
Li, M.7
-
30
-
-
40949138803
-
-
Moraes, M. L.; Baptista, M. S.; Itri, R.; Zucolotto, V.; Oliveira, O. N., Jr. Mater. Sci. Eng., C 2008, 28, 467-471
-
(2008)
Mater. Sci. Eng., C
, vol.28
, pp. 467-471
-
-
Moraes, M.L.1
Baptista, M.S.2
Itri, R.3
Zucolotto, V.4
Oliveira Jr., O.N.5
-
31
-
-
13444252774
-
-
Srivastava, S.; Frankamp, B. L.; Rotello, V. M. Chem. Mater. 2005, 17, 487-490
-
(2005)
Chem. Mater.
, vol.17
, pp. 487-490
-
-
Srivastava, S.1
Frankamp, B.L.2
Rotello, V.M.3
-
32
-
-
67649277235
-
-
Park, M.-H.; Ofir, Y.; Samanta, B.; Rotello, V. M. Adv. Mater. 2009, 21, 2323-2327
-
(2009)
Adv. Mater.
, vol.21
, pp. 2323-2327
-
-
Park, M.-H.1
Ofir, Y.2
Samanta, B.3
Rotello, V.M.4
-
33
-
-
27844474655
-
-
Qiana, L.; Liua, Y.; Songa, Y.; Lia, Z.; Yang, X. Electrochem. Commun. 2005, 7, 1209-1212
-
(2005)
Electrochem. Commun.
, vol.7
, pp. 1209-1212
-
-
Qiana, L.1
Liua, Y.2
Songa, Y.3
Lia, Z.4
Yang, X.5
-
34
-
-
33748807729
-
-
Crespilho, F. N.; Zucolotto, V.; Brett, C. M. A.; Oliveira, O. N., Jr.; Nart, F. C. J. Phys. Chem. B 2006, 110, 17478-17483
-
(2006)
J. Phys. Chem. B
, vol.110
, pp. 17478-17483
-
-
Crespilho, F.N.1
Zucolotto, V.2
Brett, C.M.A.3
Oliveira Jr., O.N.4
Nart, F.C.5
-
35
-
-
53549110003
-
-
Siqueira, J. R., Jr.; Gasparotto, L. H. S.; Oliveira, O. N., Jr.; Zucolotto, V. J. Phys. Chem. C 2008, 112, 9050-9055
-
(2008)
J. Phys. Chem. C
, vol.112
, pp. 9050-9055
-
-
Siqueira Jr., J.R.1
Gasparotto, L.H.S.2
Oliveira Jr., O.N.3
Zucolotto, V.4
-
36
-
-
33846152890
-
-
Ogasawara, S.; Ikeda, A.; Kikuchi, J.-i. Chem. Mater. 2006, 18, 5982-5987
-
(2006)
Chem. Mater.
, vol.18
, pp. 5982-5987
-
-
Ogasawara, S.1
Ikeda, A.2
Kikuchi, J.-I.3
-
38
-
-
67349108710
-
-
Li, G.; Li, X.; Wan, J.; Zhang, S. Biosens. Bioelectron. 2009, 24, 3281-3287
-
(2009)
Biosens. Bioelectron.
, vol.24
, pp. 3281-3287
-
-
Li, G.1
Li, X.2
Wan, J.3
Zhang, S.4
-
39
-
-
69949142854
-
-
Siqueira, J. R., Jr.; Abouzarb, M. H.; Poghossianb, A.; Zucolottoa, V.; Oliveira, O. N., Jr.; Schöning, M. J. Biosens. Bioelectron. 2009, 25, 497-501
-
(2009)
Biosens. Bioelectron.
, vol.25
, pp. 497-501
-
-
Siqueira Jr., J.R.1
Abouzarb, M.H.2
Poghossianb, A.3
Zucolottoa, V.4
Oliveira Jr., O.N.5
Schöning, M.J.6
-
40
-
-
69049103277
-
-
Siqueira, J. R., Jr.; Werner, C. F.; Bäcker, M.; Poghossian, A.; Zucolotto, V.; Oliveira, O. N., Jr.; Schöning, M. J. J. Phys. Chem. C 2009, 113, 14765-14770
-
(2009)
J. Phys. Chem. C
, vol.113
, pp. 14765-14770
-
-
Siqueira Jr., J.R.1
Werner, C.F.2
Bäcker, M.3
Poghossian, A.4
Zucolotto, V.5
Oliveira Jr., O.N.6
Schöning, M.J.7
-
41
-
-
49749105600
-
-
Tomita, S.; Sato, K.; Anzai, J.-i. J. Colloid Interface Sci. 2008, 326, 35-40
-
(2008)
J. Colloid Interface Sci.
, vol.326
, pp. 35-40
-
-
Tomita, S.1
Sato, K.2
Anzai, J.-I.3
-
42
-
-
62649166347
-
-
Singha, P.; Onoderaa, T.; Mizutaa, Y.; Matsumoto, K.; Miura, N.; Toko, K. Sens. Actuators B 2009, 137, 403-409
-
(2009)
Sens. Actuators B
, vol.137
, pp. 403-409
-
-
Singha, P.1
Onoderaa, T.2
Mizutaa, Y.3
Matsumoto, K.4
Miura, N.5
Toko, K.6
-
43
-
-
0345547747
-
-
Paulo, P. M. R.; Gronheid, R.; De Schryver, F. C.; Costa, S. M. B. Macromolecules 2003, 36, 9135-9144
-
(2003)
Macromolecules
, vol.36
, pp. 9135-9144
-
-
Paulo, P.M.R.1
Gronheid, R.2
De Schryver, F.C.3
Costa, S.M.B.4
-
45
-
-
2942704100
-
-
Laia, C. A. T.; Costa, S. M. B.; Phillips, D.; Beeby, A. J. Phys. Chem. B 2004, 108, 7506-7514
-
(2004)
J. Phys. Chem. B
, vol.108
, pp. 7506-7514
-
-
Laia, C.A.T.1
Costa, S.M.B.2
Phillips, D.3
Beeby, A.4
-
46
-
-
33745751393
-
-
Laia, C. A. T.; Costa, S. M. B.; Ferreira, L. F. V. Biophys. Chem. 2006, 122, 143-155
-
(2006)
Biophys. Chem.
, vol.122
, pp. 143-155
-
-
Laia, C.A.T.1
Costa, S.M.B.2
Ferreira, L.F.V.3
-
47
-
-
30844441178
-
-
Togashi, D. M.; Costa, S. M. B.; Sobral, A. J. F. N. Biophys. Chem. 2006, 119, 121-126
-
(2006)
Biophys. Chem.
, vol.119
, pp. 121-126
-
-
Togashi, D.M.1
Costa, S.M.B.2
Sobral, A.J.F.N.3
-
48
-
-
0035326346
-
-
Maus, M.; Cotlet, M.; Hofkens, J.; Gensch, T.; De Schryver, F. C. Anal. Chem. 2001, 73, 2078-2086
-
(2001)
Anal. Chem.
, vol.73
, pp. 2078-2086
-
-
Maus, M.1
Cotlet, M.2
Hofkens, J.3
Gensch, T.4
De Schryver, F.C.5
-
49
-
-
78149262504
-
-
No changes are observed in the absorption spectra of phthalocyanine upon association with the dendrimer in the region of the Q-band (transition to S1 state); however, in the region of the Soret band (transition to S2 state), a shift and broadening of this band toward longer wavelengths is observed
-
No changes are observed in the absorption spectra of phthalocyanine upon association with the dendrimer in the region of the Q-band (transition to S1 state); however, in the region of the Soret band (transition to S2 state), a shift and broadening of this band toward longer wavelengths is observed.
-
-
-
-
50
-
-
78149233660
-
-
note
-
The Rehm-Weller expression can be written as I" G 0 = (E D ox - E A red) B + (1 - 1 Iμ B) (S p - S r) - W r + W p - h I1/2 where E D ox and E A red stand for the oxidation and reduction potential of the donor and acceptor, respectively, in a medium of permittivity Iμ B; S p,r are the solvation energies of individual reactant and product ions in vacuum; W r,p are the solvation energies and Coulomb interaction of the ions, and h I1/2 is the excited-state energy. The expressions for S p,r and W r,p can be found in
-
-
-
-
51
-
-
0000374452
-
-
Tavernier, H. L.; Barzykin, A. V.; Tachiya, M.; Fayer, M. D. J. Phys. Chem. B 1998, 102, 6078-6088
-
(1998)
J. Phys. Chem. B
, vol.102
, pp. 6078-6088
-
-
Tavernier, H.L.1
Barzykin, A.V.2
Tachiya, M.3
Fayer, M.D.4
-
52
-
-
78149267793
-
-
For E D ox, we used a value of 0.97 V (vs. SCE) for the oxidation potential of triethylamine in water taken from
-
For E D ox, we used a value of 0.97 V (vs. SCE) for the oxidation potential of triethylamine in water taken from
-
-
-
-
53
-
-
0034688414
-
-
Okutsu, T.; Ooyama, M.; Hiratsuka, H.; Tsuchiya, J.; Obi, K. J. Phys. Chem. A 2000, 104, 288-292
-
(2000)
J. Phys. Chem. A
, vol.104
, pp. 288-292
-
-
Okutsu, T.1
Ooyama, M.2
Hiratsuka, H.3
Tsuchiya, J.4
Obi, K.5
-
54
-
-
78149243400
-
-
red, we used a value of -0.5 V (vs. SCE) for the reduction potential of aluminum phthalocyanine in DMSO taken from
-
red, we used a value of -0.5 V (vs. SCE) for the reduction potential of aluminum phthalocyanine in DMSO taken from
-
-
-
-
55
-
-
33751379099
-
-
The excited-state energy of the phthalocyanine is around 1.82 eV
-
Ou, Z.; Shen, J.; Kadish, K. M. Inorg. Chem. 2006, 45, 9569-9579. The excited-state energy of the phthalocyanine is around 1.82 eV
-
(2006)
Inorg. Chem.
, vol.45
, pp. 9569-9579
-
-
Ou, Z.1
Shen, J.2
Kadish, K.M.3
-
56
-
-
0022418081
-
-
Albery, W. J.; Bartlett, P. N.; Wilde, C. P.; Darwent, J. R. J. Am. Chem. Soc. 1985, 107, 1854-1858
-
(1985)
J. Am. Chem. Soc.
, vol.107
, pp. 1854-1858
-
-
Albery, W.J.1
Bartlett, P.N.2
Wilde, C.P.3
Darwent, J.R.4
-
57
-
-
57449108708
-
-
Paulo, P. M. R.; Canongia Lopes, J. N.; Costa, S. M. B. J. Phys. Chem. B 2008, 112, 14779-14792
-
(2008)
J. Phys. Chem. B
, vol.112
, pp. 14779-14792
-
-
Paulo, P.M.R.1
Canongia Lopes, J.N.2
Costa, S.M.B.3
-
60
-
-
78149270573
-
-
note
-
The value of V 0 2 = 10 cm-1 is small enough to justify the nonadiabatic approximation in eq 2 but at the same time large enough to quench the excited-state lifetime of the phthalocyanine down to subnanosecond values. The value of I = 1 A-1 is typical for electron tunneling through an aliphatic carbon donor-acceptor bridge and therefore is appropriate for the PAMAM dendrimer systems.
-
-
-
-
61
-
-
0035800279
-
-
Prosa, T. J.; Bauer, B. J.; Amis, E. J. Macromolecules 2001, 34, 4897-4906
-
(2001)
Macromolecules
, vol.34
, pp. 4897-4906
-
-
Prosa, T.J.1
Bauer, B.J.2
Amis, E.J.3
-
63
-
-
13444265936
-
-
Vallée, R. A. L.; Van der Auweraer, M.; De Schryver, F. C.; Beljonne, D.; Orrit, M. ChemPhysChem 2005, 6, 81-91
-
(2005)
ChemPhysChem
, vol.6
, pp. 81-91
-
-
Vallée, R.A.L.1
Van Der Auweraer, M.2
De Schryver, F.C.3
Beljonne, D.4
Orrit, M.5
-
64
-
-
13444266498
-
-
Maiti, P. K.; CagIın, T.; Lin, S.-T.; Goddard, W. A., III. Macromolecules 2005, 38, 979-991
-
(2005)
Macromolecules
, vol.38
, pp. 979-991
-
-
Maiti, P.K.1
Cagiän, T.2
Lin, S.-T.3
Goddard III, W.A.4
-
65
-
-
0000326062
-
-
Hou, Y.; Bardo, A. M.; Martinez, C.; Higgins, D. A. J. Phys. Chem. B 2000, 104, 212-219
-
(2000)
J. Phys. Chem. B
, vol.104
, pp. 212-219
-
-
Hou, Y.1
Bardo, A.M.2
Martinez, C.3
Higgins, D.A.4
-
66
-
-
34547277266
-
-
Clifford, J. N.; Bell, T. D. M.; Tinnefeld, P.; Heilemann, M.; Melnikov, S. M.; Hotta, J.-i.; Sliwa, M.; Dedecker, P.; Sauer, M.; Hofkens, J.; Yeow, E. K. L. J. Phys. Chem. B 2007, 111, 6987-6991
-
(2007)
J. Phys. Chem. B
, vol.111
, pp. 6987-6991
-
-
Clifford, J.N.1
Bell, T.D.M.2
Tinnefeld, P.3
Heilemann, M.4
Melnikov, S.M.5
Sliwa, M.6
Dedecker, P.7
Sauer, M.8
Hofkens, J.9
Yeow, E.K.L.10
-
67
-
-
0032187986
-
-
Bliznyuk, V. N.; Rinderspachert, F.; Tsukruk, V. V. Polymer 1998, 39, 5249-5252
-
(1998)
Polymer
, vol.39
, pp. 5249-5252
-
-
Bliznyuk, V.N.1
Rinderspachert, F.2
Tsukruk, V.V.3
-
68
-
-
0035353442
-
-
Betley, T. A.; Banaszak Holl, M. M.; Orr, B. G.; Swanson, D. R.; Tomalia, D. A.; Baker, J. R., Jr. Langmuir 2001, 17, 2768-2773
-
(2001)
Langmuir
, vol.17
, pp. 2768-2773
-
-
Betley, T.A.1
Banaszak Holl, M.M.2
Orr, B.G.3
Swanson, D.R.4
Tomalia, D.A.5
Baker Jr., J.R.6
-
69
-
-
0141993702
-
-
Yang, H.; Luo, G.; Karnchanaphanurach, P.; Louie, T.-M.; Rech, I.; Cova, S.; Xun, L.; Xie, X. S. Science 2003, 302, 262-266
-
(2003)
Science
, vol.302
, pp. 262-266
-
-
Yang, H.1
Luo, G.2
Karnchanaphanurach, P.3
Louie, T.-M.4
Rech, I.5
Cova, S.6
Xun, L.7
Xie, X.S.8
-
70
-
-
0030878722
-
-
Jia, Y.; Sytnik, A.; Li, L.; Vladimirov, S.; Cooperman, B. S.; Hochstrasser, R. M. Proc. Natl. Acad. Sci. U.S.A. 1997, 94, 7932-7936
-
(1997)
Proc. Natl. Acad. Sci. U.S.A.
, vol.94
, pp. 7932-7936
-
-
Jia, Y.1
Sytnik, A.2
Li, L.3
Vladimirov, S.4
Cooperman, B.S.5
Hochstrasser, R.M.6
-
71
-
-
78149270313
-
-
Besides fluorescence quenching by electron transfer, other factors can change the intensity of the "ona" level in single-molecule fluorescence traces (rotational dynamics, spectral diffusion, and so forth). Indeed, we observe intensity fluctuations in traces of unquenched single phthalocyanine molecules that have monoexponential decays. This is probably related to rotational dynamics of phthalocyanine in more flexible environments. This effect is more pronounced here, because the excitation light is not circularly polarized, and in-plane rotation is enough to change emission intensity. Spectral diffusion does not seem plausible, because the emission light is collected through a filter with a broad wavelength window
-
Besides fluorescence quenching by electron transfer, other factors can change the intensity of the "ona" level in single-molecule fluorescence traces (rotational dynamics, spectral diffusion, and so forth). Indeed, we observe intensity fluctuations in traces of unquenched single phthalocyanine molecules that have monoexponential decays. This is probably related to rotational dynamics of phthalocyanine in more flexible environments. This effect is more pronounced here, because the excitation light is not circularly polarized, and in-plane rotation is enough to change emission intensity. Spectral diffusion does not seem plausible, because the emission light is collected through a filter with a broad wavelength window.
-
-
-
-
72
-
-
0037452963
-
-
Rhoades, E.; Gussakovsky, E.; Haran, G. Proc. Natl. Acad. Sci. U.S.A. 2003, 100, 3197-3202
-
(2003)
Proc. Natl. Acad. Sci. U.S.A.
, vol.100
, pp. 3197-3202
-
-
Rhoades, E.1
Gussakovsky, E.2
Haran, G.3
-
73
-
-
33847254454
-
-
Nettels, D.; Gopich, I. V.; Hoffmann, A.; Schuler, B. Proc. Natl. Acad. Sci. U.S.A. 2007, 104, 2655-2660
-
(2007)
Proc. Natl. Acad. Sci. U.S.A.
, vol.104
, pp. 2655-2660
-
-
Nettels, D.1
Gopich, I.V.2
Hoffmann, A.3
Schuler, B.4
|