Interdiffusion/reaction at the polymer/polymer interface in multilayer systems probed by linear viscoelasticity coupled to FTIR and NMR measurements

European Polymer Journal

Volumn 46, Issue 7, 2010, Pages 1604-1622

  Lamnawar, Khalid ^a   Baudouin, Anne ^b   Maazouz, Abderrahim ^a,c  

^a UNIVERSITÉ DE LYON   (France)

^b UNIVERSITÉ LYON 1   (France)

^c HASSAN II ACADEMY OF SCIENCE AND TECHNOLOGY   (Morocco)

Author keywords

Coextrusion; FTIR; Interphase; NMR; Reactive multilayer; Rheology

Indexed keywords

COEXTRUSION; ELASTICITY; MULTILAYERS; NUCLEAR MAGNETIC RESONANCE; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; POLYMERS; RHEOLOGY; VISCOELASTICITY;

EXPERIMENTAL INVESTIGATIONS; FTIR; INTERPHASE; IR AND NMR SPECTROSCOPY; LINEAR VISCOELASTICITY; PHYSICOCHEMICAL PHENOMENA; POLYMER-POLYMER INTERFACES; RHEOLOGICAL MEASUREMENTS;

CROSSLINKING;

EID: 77953684649     PISSN: 00143057     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.eurpolymj.2010.03.019     Document Type: Article

References (61)

1. Riemann R.E., Cantow H.J., and Friedrich C. Interpretation of a new interface-governed relaxation process in compatibilized polymer blends. Macromolecules 30 (1997) 5476
2. Muller R., Cirman C., Bouquey M., and Terrisse J. Rheological study of the interfacial crosslinking reaction in reactive polymer blends. Appl Rheol 9 3 (1999) 108-115
3. Muller R., Bouquey M., Mauguière F., Schlatter G., Serra C., and Terrisse J. Rheology of reactive polymer blends: separation of mixing and reaction steps. Appl Rheol 11 2 (2001) 141-152
4. Serra C., Bouquey M., Schlatter G., and Muller R. Rheological behavior of reactive miscible polymer blends: influence of mixing and annealing before crosslinking. J Appl Polym Sci 98 (2005) 1978-1995
5. Levitt L., Macosko C.W., Schmeizer T., and Meisner J. Extensional rheometry of polymer multilayers: a sensitive probe of interfaces. J Rheol 41 (1997) 671
6. Bousmina M., Qiu Hua., Grmela M., and Klemberg-Sapieha J.E. Diffusion at Polymer/polymer interfaces probed by rheological tools. Macromolecules 31 (1998) 8273
7. Qiu H., and Bousmina M. Determination of mutual diffusion coefficients at Nonsymmetric Polymer/Polymer interfaces from rheometrys. Macromolecules 33 (2000) 6588-6594
8. de Gennes P.G. Reptation of a polymer chain in the presence of fixed obstacles. J Chem Phys 55 (1971) 572
9. de Gennes P.G. Kinetics of diffusion - controlled processes in dense polymer systems. II. Effects of entanglements. J Chem Phys 76 (1982) 3322
10. Scheinhardt-Engels S.M., Leermakers F.A.M., and Fleer G. Lattice mean-field method for stationary polymer diffusion. J Phys Rev 68 (2003) 011802
11. Lamnawar K., and Maazouz A. Rheological study of multilayer functionalized polymers: Characterization of interdiffusion and reaction at polymer/polymer interface. Rheol Acta 45 (2006) 411-424
12. Lamnawar K., and Maazouz A. Rheology and morphology of multilayer reactive polymers: effect of interfacial area in interdiffusion/reaction phenomena. Rheol Acta 47 (2008) 383-397
13. Lamnawar K., and Maazouz A. Reactive functionalized multilayer polymers in coextrusion process. AIP Conf Proc 907 (2007) 908-914
14. Lyu S., Cernohous J.J., Macosko C.W., and Bates F.S. Interfacial reaction induced roughening in polymer blends. Macromolecules 32 (1999) 106-110
15. Lamnawar K., Vion-Loisel F., and Maazouz A. Rheological, morphological and heat seal properties of linear low density polyethylene and cyclo-olefine copolymer (LLDPE/COC) blends. J Appl Polym Sci 116 4 (2010) 2015-2022
16. Jiao J., Kramer E.J., Sicco d.V., Moller M., and Koning C. Morphological changes of a molten polymer/polymer interface driven by grafting. Macromolecules 32 (1999) 6261-6269
17. Schulze J.S., Lodge T.P., and Macosko C.W. The reactive formation of diblock copolymer at a polymer/polymer interface and its effect on interfacial structure. Mater Res Soc Symp 629 (2000) FF2.2.1-FF2.2.6
18. Yin Z., Koulic C., Pagnoulle C., and Jerome R. Probing of the reaction progress at a PMMA/PS interface by using anthracene-labeled reactive PS chains. Langmuir 19 (2003) 453-457
19. Fredrickson G.H., and Scott M.T. Time-dependent reactive coupling at polymer-polymer interfaces. Macromolecules 29 (1996) 7386-7390
20. O'Shaughnessy B., and Vavylonis D. Reactive polymer interfaces: how reaction kinetics depend on reactivity and density of chemical group. Macromolecules 32 (1999) 1785-1796
21. Fredrickson G.H. Diffusion-controlled reactions at polymer-polymer Interfaces. Phys Rev Lett 76 (1996) 3440
22. Wool P.R. Polymer interface. Structure development at semicrystalline interfaces (1995), Hansers, Munich 383
23. Jones T.D., Schulze J.S., Macosko C.W., and Lodge T.P. Effect of thermodynamic interactions on reactions at polymer/polymer interfaces. Macromolecules 36 (2003) 7212-7219
24. Kim J.B., Kang H., Char K., Katsow K., Fredrikson G.H., and Kramer E. Interfacial roughening induced by the reaction of end-functionalized polymers at a PS/P2VP interface: quantitative analysis by DSIMS. Macromolecules 38 (2005) 6106-6114
25. Zhang X.M., Li X.L., Wang D.M., Yin Z.H., and Yin J.H. Morphology, thermal behavior, and mechanical properties of PA1010/PP and PA 1010/PP-g-GMA blends. J Appl Polym Sci 64 (1997) 1489
26. Kuroda T., Torikai K., Oyama H.T., Ougizawa T., Inoue T., and Weber M. Reaction-induced pattern formation at the polymer-polymer interface. Kobunshi Ronbunshu 56 (1999) 860
27. Xie F., Zhou C., Yu W., and Wu D. Reaction kinetics study of asymmetric polymer-polymer interface. Polymer 46 (2005) 8410-8415
28. Harton S.E., Stevie F.A., and Ade H. Diffusion-controlled reactive coupling at polymer-polymer interfaces. Macromolecules 38 (2005) 3543-3546
29. Schulze S.J., Jeffrey J.C., Hiraro A., Lodge T.P., and Macosko C.W. Reaction kinetics of end-functionalized chains at a polystyrene/poly(methyl methacrylate) interface. Macromolecules 33 (2000) 1191-1198
30. Xiaobo Y., Yang W., Binyao L., and Yanchun H. Studies on interfacial reaction kinetics and properties at a reactive compatibilization interface. Polymer 46 (2005) 3337-3342
31. Kim H.Y., Jeong U., and Kim J.K. Reaction kinetics and morphological changes of reactive polymer-polymer interface. Macromolecules 36 (2003) 1594-1602
32. Lamnawar K., and Maazouz A. Role of the interphase in the flow stability of reactive coextruded multilayer polymers. Polym Eng Sci 49 (2009) 727-739
33. Baker M., Scott C., and Hu G.-H. Reactive polymer blending (2001), Hanser Publishers, Munich
34. Koulouri E.G., Georgaki A.X., and Kallitsis J.K. Reactive compatibilization of aliphatic polyamides with functionalized polyethylenes. Polymer 38 (1997) 4185-4192
35. Zhang X.M., Yin Z.H., Li L.X., and Yin J.H. Grafting of glycidyl methacrylate onto ethylene-propylene copolymer: Preparation and characterization. J Appl Polym Sci 61 (1996) 2253
36. Filippi S., Chiono V., Polacco G., Paci M., Minkova L., and Magagnini P. Reactive compatibilizer precursors for LDPE/PA6 blends, 1. Ethylene/Acrylic Acid Copolymers. Macromol Chem Phys 203 (2002) 1512
37. Chiono V., Filippi S., Yordanov H., Minkova L., and Magagnini P. Reactive compatibilizer precursors for LDPE/PA6 blends. III: ethylene-glycidylmethacrylate copolymer. Polymer 44 (2003) 2423
38. Jiang C., Filippi S., and Magagnini P. Reactive compatibilizer precursors for LDPE/PA6 blends. II: maleic anhydride grafted polyethylenes. Polymer 44 (2003) 2411-2422
39. Wei Q., Chionna D., and Pracella M. Reactive compatibilization of PA6/LDPE blends with glycidyl methacrylate functionalized polyolefins. Macromol Chem Phys 206 (2005) 777-786
40. Coote M.L., Gordon D.H., Hutchings L.R., and Richards R.W. Neutron reflectometry investigation of polymer-polymer reactions at the interface between immiscible polymers. Polymer 44 (2003) 7689-7700
41. Yokoyama H., and Kramer E.J. Mutual diffusion of asymmetric block copolymers with homopolymers. Macromolecules 33 (2000) 1871-1877
42. Lamnawar K., and Maazouz A. Interfacial Rheology of multilayer functionalized polymers. Matériaux & Techniques 94 5 (2006) 305-321
43. Sun Y.J., Hu G.H., Lambla M., and Kotlar H.K. In situ compatibilization of polypropylene and poly(butylene terephthalate) polymer blends by one-step reactive extrusion. Polymer 37 (1996) 4119-4127
44. Wu S., and Chang H.-K. Diffuse interface between polymers: structure and kinetics. J Polym Sci: Polym Phys 24 (1986) 143-159
45. Fetters L.J., Lohse T.D.J., Richter D., Witten T.A., and Zirkelt A. Connection between polymer molecular weight, density, chain dimensions, and melt viscoelastic properties. Macromolecules 27 (1994) 4639
46. Lin K.K., and Chang D.H. Polymer-polymer interdiffusion during coextrusion. Polym Eng Sci 31 4 (1991) 258-268
47. Lin C.C. A mathematical model for viscosity in capillary extrusion of two-component polyblends. Polym J 11 (1979) 185-192
48. Heitmiller R.F., Naar R., and Zabusky H.H. Effect of homogeneity on viscosity in capillary extrusion of polyethylene. J Appl Polym Sci 8 (1964) 873
49. Bousmina M., Palierne J.F., and Utracki L.A. Modeling of structured polyblend flow in a laminar shear field. Polym Eng Sci 39 (1999) 1049-1059
50. Zhao R., and Macosko C.W. Slip at polymer-polymer interfaces: rheological measurements on coex- truded multilayers. J Rheol 46 (2002) 145-167
51. Lee PC, Park HE, Macosko CW, Dealy JM. Polymer-polymer interfacial slip measurements in multilayered film. Ann. Tech. Conf. (ANTEC), May 2008; Soc. of Plastics Eng'rs.im.
52. Kim H.Y., Kim H.-J., and Kim J.K. Effect of interfacial reaction and morphology on rheological properties of reactive bilayer. Polym J 38 (2006) 1165-1172
53. Koriyama H., Oyama H.T., Ougizawa T., Inoue T., Weber M., and Koch E. Studies on the reactive polysulfone-polyamide in interfacial thickness and adhesion. Polymer 40 (1999) 6381-6393
54. Patlazhan S., Schlatter G., Serra C., Bouquey M., and Muller R. Shear-induced fractal morphology of immiscible reactive polymer blends. Polymer 47 (2006) 6099-6106
55. Schmidt-Rohr K., and Spiess W. Multidimensional solid state and polymers. 2nd ed. (1996), Academic Press
56. Sheng-shu H., and Ping-Lin K. Morphological, thermal and solid-state NMR study on a novel PMMA/crosslinked silicone semi-IPN. Polymer 42 (2001) 9505-9511
57. In: Ibbet R.N. (Ed). NMR spectroscopy of polymers (1993), Chapman & Hall, London
58. Bovey F.A., and Mirau P.A. NMR of polymers (1996), Academic Press, San Diego
59. Orr C.A., Cernohous J.J., Guegan P., Hirao A., Jeon H.K., and Macosko C.W. Homogeneous reactive coupling of terminally functional polymers. Polymer 42 (2001) 8171-8178
60. Orr CA. 1997. Ph. D. thesis. University of Minnesota.
61. Montanari T. 1992. Mélanges élastomères thermoplastiques élaborés par vulcanisation dynamique. Ph. D. Université de Louis Pasteur, Strasbourg.