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In fact, a careful microscopic derivation shows that the a full bilinear interaction between the spins is akin to the familiar Heisenberg interaction: H=∑ JSi·Sj′, where S′ has been rotated about Dij by a certain angle (Refs.). While experimentally confirmed (Ref.), and undoubtfully important in discussions of a spontaneous ferromagnetism, this observation is not essential for the lowest-order calculations of the uniform susceptibility in the absence of magnetic order-the subject of this manuscript.
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Of course, the fluctuation-dissipation theorem will still be true. However, the relationship between the uniform susceptibility and spin-spin correlation will now involve more than just the equal-time correlator (Ref.).
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Of course, the fluctuation-dissipation theorem will still be true. However, the relationship between the uniform susceptibility and spin-spin correlation will now involve more than just the equal-time correlator (Ref.).
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We might view a valence-bond solid as "exotic" if it occurs spontaneously due to quantum frustration. However, in the SS model, and experimentally in spin-dimer materials (Ref.), the valence-bond solid phase occurs because some links have a stronger interaction than others. The discussion in the introduction where we counted the valence-bond solid as an example of an exotic nonmagnetic phase was in reference to the first scenario.
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We might view a valence-bond solid as "exotic" if it occurs spontaneously due to quantum frustration. However, in the SS model, and experimentally in spin-dimer materials (Ref.), the valence-bond solid phase occurs because some links have a stronger interaction than others. The discussion in the introduction where we counted the valence-bond solid as an example of an exotic nonmagnetic phase was in reference to the first scenario.
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The experiments we are referring to (Ref.) were actually done in a magnetometer with a static field of H=1.0 T, which for spin 1/2 corresponds to an energy scale g μB H∼1.3 K. The temperature range of the experiment is from 1.7 to 400 K, so the results can be interpreted by a zero-field theory except for perhaps the very lowest temperature points.
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The experiments we are referring to (Ref.) were actually done in a magnetometer with a static field of H=1.0 T, which for spin 1/2 corresponds to an energy scale g μB H∼1.3 K. The temperature range of the experiment is from 1.7 to 400 K, so the results can be interpreted by a zero-field theory except for perhaps the very lowest temperature points.
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Measurements of the NMR relaxation rate (Ref.) determined the gap to the lowest magnetic state to be Δ1 =30 K, consistent with the value of Δ1 =35 K given in Ref.. Fitting the susceptibility data gave a slightly lower value of Δ=19 K but these and other authors (Ref.) have interpreted the ≈30 K values as the "spin gap." Therefore, we use this value for our estimate.
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Measurements of the NMR relaxation rate (Ref.) determined the gap to the lowest magnetic state to be Δ1 =30 K, consistent with the value of Δ1 =35 K given in Ref.. Fitting the susceptibility data gave a slightly lower value of Δ=19 K but these and other authors (Ref.) have interpreted the ≈30 K values as the "spin gap." Therefore, we use this value for our estimate.
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The spin gap scale is ∼Δ/g μB ∼20 T while the onset of a uniform magnetization is seen at around 18 T. We point out that these interesting field dependencies occur at fields much higher than the 1.0 T field of the magnetometer used in Ref., the results of which we interpret with our zero-field calculation.
-
The spin gap scale is ∼Δ/g μB ∼20 T while the onset of a uniform magnetization is seen at around 18 T. We point out that these interesting field dependencies occur at fields much higher than the 1.0 T field of the magnetometer used in Ref., the results of which we interpret with our zero-field calculation.
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One situation where the expansion might not work so well is if the wave function were a liquid state of the Rokhsar-Kivelson type (Ref.). In this case, the error made in keeping only leading terms might be quite large because of the cumulative effect of many small terms.
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One situation where the expansion might not work so well is if the wave function were a liquid state of the Rokhsar-Kivelson type (Ref.). In this case, the error made in keeping only leading terms might be quite large because of the cumulative effect of many small terms.
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