Global distribution of solid and aqueous sulfafte aerosols: Effect of the hysteresis of particle phase transitions

Journal of Geophysical Research Atmospheres

Volumn 113, Issue 11, 2008, Pages

  Wang, Jun ^a,b   Hoffmann, Andrew A ^a   Park, Rokjin J ^a,c   Jacob, Daniel J ^a   Martin, Scot T ^a  

^a HARVARD UNIVERSITY   (United States)

^b UNIVERSITY OF NEBRASKA LINCOLN   (United States)

^c Seoul National University   (South Korea)

Author keywords

[No Author keywords available]

Indexed keywords

AIR POLLUTION; ATMOSPHERIC AEROSOLS; ATMOSPHERIC HUMIDITY; BOUNDARY CONDITIONS; COMPUTER SIMULATION; HYSTERESIS; PHASE TRANSITIONS; TROPOSPHERE;

AEROSOL; BIOMASS BURNING; BOUNDARY LAYER; COMPUTER SIMULATION; CRYSTALLIZATION; NEUTRALIZATION; PHASE TRANSITION; RELATIVE HUMIDITY; SEASONAL VARIATION; SULFATE; TROPOSPHERE;

EID: 53149123681     PISSN: 01480227     EISSN: None     Source Type: Journal    
DOI: 10.1029/2007JD009367     Document Type: Article

References (51)

1. Abbatt, J. P, D., S. Benz, D. J. Cziczo, Z. Kanji, U. Lohmann, and O, Mohler (2006), Solid ammonium sulfate aerosols as ice nuclei: A pathway for cirrus cloud formation, Science, 313, 1770-1773, doi:10.1126/ science.1129726.
2. Adams, P. J., J. H. Seinfeld, and D. M. Koch (1999), Global concentrations of tropospheric sulfate, nitrate, and ammonium aerosol simulated in a general circulation model, J. Geophys. Res., 104, 13,791-13,823, doi:10.1029/1999JD900083.
3. Adams, P. J., J. H. Seinfeld, D. Koch, L. Mickley, and D. Jacob (2001), General circulation model assessment of direct radiative forcing by the sulfate-nitrate-ammonium-water inorganic aerosol system, J. Geophys. Res., 106, 1097-1111, doi:10.1029/2000JD900512.
4. Allen, D. J., R. B. Rood, A. M. Thompson, and R. D. Hidson (1996), Three-dimension 222 Rn calculations using assimilated data and a convective mixing algorithm, J. Geophys. Res., 101, 6871-6881, doi:10.1029/95JD03408.
5. Andres, R. J., and A. D. Kasgnoc (1998), A time-averaged inventory of subaerial volcanic sulfur emissions, J. Geophys. Res., 103, 25,251-25,261, doi:10.1029/98JD02091.
6. Benkovitz, C. M., M. T. Scholtz, J. Pacyna, L. Tarrason, J. Dignon, E. C. Voldner, P. A. Spiro, J. A. Logan, and T. E. Graedel (1996), Global gridded inventories of anthropogenic emissions of sulfur and nitrogen, J. Geophys. Res., 101, 29,239-29,253, doi:10.1029/96JD00126.
7. Bey, I., D. J. Jacob, R. M. Yantosca, J. A. Logan, B. Field, A. M. Fiore, Q. Li, H. Liu, L. J. Mickley, and M. Schultz (2001), Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res., 106, 23,073-23,096, doi:10.1029/2001JD000807.
8. Biskos, G., A. Malinowski, L. M. Russell, P. R. Buseck, and S. T. Martin (2006a), Nanosize effect on the deliquescence and the efflorescence of sodium chloride nanoparticles, Aerosol Sci. Technol., 40, 97-106, doi:10.1080/02786820500484396.
9. Biskos, G., D. Paulsen, L. M. Russell, P. R. Buseck, and S. T. Martin (2006b), Prompt deliquescence and efflorescence of aerosol nanoparticles, Atmos. Chem. Phys., 6, 4633-4642.
10. Bouwman, A. F., D. S. Lee, W. A. H. Asman, F. J. Dentener, K. W. Van Der Hoek, and J. G. J. Olivier (1997), A global high-resolution emission inventory for ammonia, Global Biogeochem. Cycles, 11, 561-587, doi:10.1029/97GB02266.
11. Braban, C. F., and J. P. D. Abbatt (2004), A study of the phase transition behavior of internally mixed ammonium sulfate-malonic acid aerosols, Atmos. Chem. Phys., 4, 1451-1459.
12. Chin, M., and D. J. Jacob (1996), Anthropogenic and natural contributions to tropospheric sulfate: A global model analysis, J. Geophys. Res., 101, 18,691-18,699, doi:10.1029/96JD01222.
13. Clegg, S. L., P. Brimblecombe, and A. S. Wexler (1998), Thermodynamic model of the system H+-NH4+-Na+ -SO42--NO3--Cl- -H2O at 298.15 K, J. Phys. Chem. A, 102, 2155-2171, doi:10.1021/jp973043j.
14. Colberg, C. A., B. P. Luo, H. Wernli, T. Koop, and T. Peter (2003), A novel model to predict the physical state of atmospheric H2SO4/NH3/H2O aerosol particles, Atmos. Chem. Phys., 3, 909-924.
15. Corbett, J. J., P. S. Fischbeck, and S. N. Pandis (1999), Global nitrogen and sulfur inventories for ocean-going ships, J. Geophys. Res., 104, 3457-3470, doi:10.1029/1998JD100040.
16. Dibb, J. E., R. W. Talbot, and E. M. Scheuer (2000), Composition and distribution of aerosols over the North Atlantic during the Subsonic Assessment Ozone and Nitrogen Oxide Experiment (SONEX), J. Geophys. Res., 105, 3709-3717, doi:10.1029/1999JD900424.
17. Dibb, J. E., R. W. Talbot, G. Seid, C. Jordan, E. Scheuer, E. Atlas, N. J. Blake, and D. R. Blake (2002), Airborne sampling of aerosol particles: Comparison between surface sampling at Christmas Island and P-3 sampling during PEM-Tropics B, J. Geophys. Res., 107, 8230, doi:10.1029/2001JD000408 [printed 108(D2), 2003].
18. Dibb, J. E., R. W. Talbot, E. M. Scheuer, G. Seid, M. A. Avery, and H. B. Singh (2003), Aerosol chemical composition in Asian continental outflow during the TRACE-P campaign: Comparison with PEM-West B, J. Geophys. Res., 108(D21), 8815, doi:10.1029/2002JD003111.
19. Haywood, J., and O. Boucher (2000), Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review, Rev. Geophys., 38, 513-543, doi:10.1029/1999RG000078.
20. Jaccard, C., and L. Levi (1961), Ségrégation d'impuretés dans la glace, Z. Agewandte Math. Phys., 12, 70-76, doi:10.1007/BF01601109.
21. Jacob, D. J. (2000), Heterogeneous chemistry and tropospheric ozone, Atmos. Environ., 34, 2131-2159, doi:10.1016/S1352-2310(99)00462-8.
22. Jacobson, M. Z. (2001), Global direct radiative forcing due to multicomponent anthropogenic and natural aerosols, J. Geophys. Res., 106, 1551-1568, doi:10.1029/2000JD900514.
23. Kane, S. M., F. Caloz, and M. T. Leu (2001), Heterogeneous uptake of gaseous N2O5 by (NH4)2 SO4,NH4HSO4, and H2 SO4 aerosols,J. Phys. Chem. A, 105, 6465-6470, doi:10.1021/jp010490x.
24. Lehmann, C. M. B., V. C. Bowersox, R. S. Larson, and S. M. Larson (2007), Monitoring long-term trends in sulfate and ammonium in US precipitation: Results from the National Atmospheric Deposition Program/ National Trends Network, Water Air Soil Pollut., 7, 59-66, doi:10.1007/s11267-006-9100-z.
25. Lim, H. J., A. G. Carlton, and B. J. Turpin (2005), Isoprene forms secondary organic aerosol through cloud processing: Model simulations, Environ. Sci. Technol., 39, 4441-4446, doi:10.1021/es048039h.
26. Lin, S.-J., and R. B. Rood (1996), Multidimensional flux from semi-Lagrangian transport scheme, Mon. Weather Rev., 124, 2046-2070, doi:10.1175/1520-0493(1996)124<2046:MFFSLT>2.0.CO;2.
27. Liu, H., et al. (2006), Radiative effect of clouds on tropospheric chemistry in a global three-dimensional chemical transport model, J. Geophys. Res., 111, D20303, doi:10.1029/2005JD006403.
28. Mari, C., D. J. Jacob, and P. Bechtold (2000), Transport and scavenging of soluble gases in a deep convective cloud, J. Geophys. Res., 105, 22,255-22,267, doi:10.1029/2000JD900211.
29. Martin, S. T. (1998), Phase transformations of the ternary system (NH4)2SO4-H2SO4- H2O and the implications for cirrus cloud formation, Geophys. Res. Lett., 25, 1657-1660, doi:10.1029/98GL00634.
30. Martin, S. T. (2000), Phase transitions of aqueous atmospheric particles, Chem. Rev., 100, 3403-3453, doi:10.1021/cr990034t.
31. Martin, S. T., J. H. Han, and H. M. Hung (2001), The size effect of hematite and corundum inclusions on the efflorrscence relative humidities of aqueous ammonium sulfate particles, Geophys. Res. Lett., 28, 2601-2604, doi:10.1029/2001GL013120.
32. Martin, S. T., J. C. Schlenker, A. Malinowski, H. M. Hung, and Y. Rudich (2003), Crystallization of atmospheric sulfate-nitrate-ammonium particles, Geophys. Res. Lett., 30(21), 2102, doi:10.1029/ 2003GL017930.
33. Martin, S. T., H. M. Hung, R. J. Park, D. J. Jacob, R. J. D. Spurr, K. V. Chance, and M. Chin (2004), Effects of the physical state of tropospheric ammonium-sulfate-nitrate particles on global aerosol direct radiative forcing, Atmos. Chem. Phys., 4, 183-214.
34. McKeen, S. A., T. Gierczak, J. B. Burkholder, P. O. Wennberg, T. F. Hanisco, E. R. Keim, R.-S. Gao, S. C. Liu, A. R. Ravishankara, and D. W. Fahey (1997), The photochemistry of acetone in the upper troposphere: A source of odd-hydrogen radicals, Geophys. Res. Lett., 24, 3177-3180, doi:10.1029/97GL03349.
35. Moorthi, S., and M. J. Suarez (1992), Relaxed Arakawa-Schubert. A parameterizaiton of moist convection for general circulation models, Mon. Weather Rev., 120, 978-1002, doi:10.1175/1520-0493(1992) 120<0978:RASAPO>2.0.CO;2.
36. Park, R. J., D. J. Jacob, B. D. Field, R. M. Yantosca, and M. Chin (2004), Natural and transboundary pollution influences on sulfate-nitrate-ammonium aerosols in the United States: Implications for policy, J. Geophys. Res., 109, D15204, doi:10.1029/2003JD004473.
37. Parsons, M. T., D. A. Knopf, and A. K. Bertram (2004), Deliquescence and crystallization of ammonium sulfate particles internally mixed with water-soluble organic compounds, J. Phys. Chem. A, 108, 11,600-11,609, doi:10.1021/jp0462862.
38. Parsons, M. T., J. L. Riffell, and A. K. Bertram (2006), Crystallization of aqueous inorganic-malonic acid particles: Nucleation rates, dependence on size, and dependence on the ammonium-to-sulfate ratio, J. Phys. Chem. A, 110, 8108-8115, doi:10.1021/jp057074n.
39. Pruppacher, H. R., and J. D. Klett (2003), Microphysics of Clouds and Precipitation, pp. 163-164, Springer, New York.
40. Ramaswamy, V., et al. (2001), Radiative forcing of climate change, in Climate Change 2001: The Scientific Basis - Contribution of Working Group I to the Third Assessment Report of the Intergovernmental Panel on climate Change, edited by J. T. Houghton et al., pp. 349-416, Cambridge Univ. Press, New York.
41. Schlenker, J. C., and S. T. Martin (2005), Crystallization pathways of sulfate-nitrate-ammonium aerosol particles, J. Phys. Chem. A, 109, 9980-9985, doi:10.1021/jp052973x.
42. Schultz, M. G., D. J. Jacob, J. D. Bradshaw, S. T. Sandholm, J. E. Dibb, R. W. Talbot, and H. B. Singh (2000), Chemical NO[i#x budget in the upper troposphere over the tropical south Pacific, J. Geophys. Res., 105, 6669-6679, doi:10.1029/1999JD900994.
43. Seinfeld, J. H., and S. N. Pandis (1998), Atmospheric Chemistry and Physics, John Wiley, New York.
44. Shilling, J. E., T. J. Fortin, and M. A. Tolbert (2006), Depositional ice nucleation on crystalline organic and inorganic solids, J. Geophys. Res., 111, D12204, doi:10.1029/2005JD006664.
45. Spann, J. F., and C. B. Richardson (1985), Measurement of the water cycle in mixed ammonium acid sulfate particles, Atmos. Environ., 19, 819-825, doi:10.1016/0004-6981(85)90072-1.
46. Spiro, P. A., D. J. Jacob, and J. A. Logan (1992), Global inventory of sulfur emissions with 1° × 1° resolution, J. Geophys. Res., 97, 6023-6036.
47. Streets, D. G., et al. (2003), An inventory of gaseous and primary aerosol emissions in Asia in the year 2000, J. Geophys, Res., 108(D21), 8809, doi:10.1029/2002JD003093.
48. Talbot, R. W., J. E. Dibb, and M. B. Loomis (1998), Influence of vertical transport on free tropospheric aerosols over the central USA in springtime, Geophys. Res. Lett., 25, 1367-1370, doi:10.1029/ 98GL00184.
49. Tang, I. N., and H. R. Munkelwitz (1994), Aerosol phase-transformation and growth in the atmosphere, J. Appl. Meteorol., 33, 791-796, doi:10.1175/1520-0450(1994)033<0791:APTAGI>2.0.CO;2.
50. Wang, J., and S. T. Martin (2007), Satellite characterization of urban aerosols: Importance of including hygroscopicity and mixing state in the retrieval algorithms, J. Geophys. Res., 112, D17203, doi:10.1029/ 2006JD008078.
51. Wang, J., D. J. Jacob, and S. T. Martin (2008), Sensitivity of sulfate direct climate forcing to the hysteresis of particle phase transitions, J. Geophys. Res., 113, D11207, doi:10.1029/2007JD009368.