Polarized pump-probe measurements of electronic motion via a conical intersection

Journal of Chemical Physics

Volumn 128, Issue 14, 2008, Pages

  Farrow, Darcie A ^a,b   Qian, Wei ^a,c   Smith, Eric R ^a   Ferro, Allison A ^a,d   Jonas, David M ^a  

^a UNIVERSITY OF COLORADO   (United States)

^b SANDIA NATIONAL LABORATORIES   (United States)

^c GEORGIA INSTITUTE OF TECHNOLOGY   (United States)

^d Cutera Inc   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ANISOTROPY; POLARIZATION; WAVE PACKETS;

POLARIZATION ANISOTROPY; PROBE SPECTROSCOPY;

ULTRASHORT PULSES;

EID: 42349094547     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.2837471     Document Type: Article

References (101)

1. E. Teller, Isr. J. Chem. 7, 227 (1969).
2. H. E. Zimmerman, Acc. Chem. Res. 5, 393 (1972).
3. L. J. Butler, Annu. Rev. Phys. Chem. 49, 125 (1998).
4. J. C. Tully, in Dynamics of Molecular Collisions Part B, edited by, W. H. Miller, (Plenum, New York, 1976), Vol. 2, p. 217.
5. E. C. Kemble, The Fundamental Principles of Quantum Mechanics, 1st ed. (McGraw-Hill, New York, 1937).
6. L. D. Landau and E. M. Lifschitz, Quantum Mechanics, 3rd ed. (Pergamon, New York, 1977).
7. J. B. Delos, W. R. Thorson, and S. K. Knudson, Phys. Rev. A 1050-2947 10.1103/PhysRevA.6.709 6, 709 (1972); J. B. Delos and W. R. Thorson, Phys. Rev. A 6, 720 (1972).
8. J. v. Neumann and E. Wigner, Phys. Z. 0369-982X 30, 467 (1929); E. Teller, J. Phys. Chem. 41, 109 (1937).
9. M. Klessinger and J. Michl, Excited States and Photochemistry of Organic Molecules (VCH, New York, 1995).
10. D. R. Yarkony, J. Phys. Chem. A 105, 6277 (2001).
11. F. Bernardi, M. Olivucci, and M. A. Robb, Chem. Soc. Rev. 25, 321 (1996).
12. S. Hahn and G. Stock, J. Phys. Chem. B 104, 1146 (1999).
13. J. D. Coe and T. J. Martinez, J. Am. Chem. Soc. 127, 4560 (2005).
14. H. L. Berghout, S. Brown, R. Delgado, and F. F. Crim, J. Chem. Phys. 109, 2257 (1998).
15. A. L. Sobolewski and W. Domcke, Eur. Phys. J. D 20, 369 (2002).
16. G. A. Worth and L. S. Cederbaum, Annu. Rev. Phys. Chem. 55, 127 (2004).
17. A. Stolow, Annu. Rev. Phys. Chem. 54, 89 (2003).
18. S. A. Trushin, T. Yatsuhashi, W. Fuß, and W. E. Schmid, Chem. Phys. Lett. 0009-2614 10.1016/S0009-2614(03)00979-5 376, 282 (2003); S. Sorgues, J. M. Mestdagh, J. P. Visticot, and B. Soep, Phys. Rev. Lett. 0031-9007 10.1103/PhysRevLett.91.103001 91, 103001 (2003); A. J. Wurzer, T. Wilhelm, J. Piel, and E. Riedle, Chem. Phys. Lett. 299, 296 (1999).
19. R. R. Jones, C. S. Raman, D. W. Schumacher, and P. H. Bucksbaum, Phys. Rev. Lett. 71, 2575 (1993).
20. R. B. Bernstein and A. H. Zewail, J. Chem. Phys. 90, 829 (1989).
21. D. M. Jonas and G. R. Fleming, in Ultrafast Processes in Chemistry and Photobiology, edited by, M. A. El-Sayed, I. Tanaka, and, Y. Molin, (Blackwell Scientific, Oxford, 1995), p. 225.
22. T. S. Rose, M. J. Rosker, and A. H. Zewail, J. Chem. Phys. 91, 7415 (1989).
23. B. S. Prall, D. Y. Parkinson, N. Ishikawa, and G. R. Fleming, J. Phys. Chem. A 109, 10870 (2005).
24. H. Kano, T. Saito, and T. Kobayashi, J. Phys. Chem. A 106, 3445 (2002).
25. J. C. Tully, J. Chem. Phys. 93, 1061 (1990).
26. G. J. Atchity, S. S. Xantheas, and K. Ruedenberg, J. Chem. Phys. 95, 1862 (1991).
27. M. A. Robb and M. Olivucci, J. Photochem. Photobiol., A 144, 237 (2001).
28. L. Allen and J. H. Eberly, Optical Resonance and Two-Level Atoms (Dover, New York, 1987).
29. N. Bloembergen, Nonlinear Optics (Addison-Wesley, New York, 1992).
30. W. Demtröder, Laser Spectroscopy, 2nd ed. (Springer-Verlag, New York, 1982).
31. D. Chandler, Introduction to Modern Statistical Mechanics (Oxford University Press, New York, 1987).
32. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, New York, 1995).
33. B. Hoffman and M. A. Ratner, Mol. Phys. 35, 901 (1978).
34. C. Galli, K. Wynne, S. M. LeCours, M. J. Therien, and R. M. Hochstrasser, Chem. Phys. Lett. 206, 493 (1993).
35. R. S. Knox and D. Gülen, Photochem. Photobiol. 0031-8655 10.1111/j.1751-1097.1993.tb02252.x 57, 40 (1993); K. Wynne and R. M. Hochstrasser, J. Raman Spectrosc. 26, 561 (1995).
36. K. Wynne and R. M. Hochstrasser, Chem. Phys. 171, 179 (1993).
37. K. Wynne and R. M. Hochstrasser, Chem. Phys. 173, 539 (1993).
38. A. Albrecht Ferro and D. M. Jonas, J. Chem. Phys. 115, 6281 (2001).
39. R. S. Knox, D. Gülen, and K. E. Lotterhos, Chem. Phys. Lett. 361, 285 (2002).
40. W. Qian and D. M. Jonas, J. Chem. Phys. 119, 1611 (2003).
41. E. R. Smith, D. A. Farrow, and D. M. Jonas, J. Chem. Phys. 123, 044102 (2005).
42. E. R. Smith, D. A. Farrow, and D. M. Jonas, J. Chem. Phys. 0021-9606 10.1063/1.2090187 123, 179902 (2005); E. R. Smith, D. A. Farrow, and D. M. Jonas, J. Chem. Phys. 128, 109902 (2008).
43. H. A. Jahn and E. Teller, Proc. R. Soc. London, Ser. A 161, 220 (1937).
44. J. T. Hougen, J. Mol. Spectrosc. 13, 149 (1964).
45. G. H. Herzberg, Electronic Spectra of Polyatomic Molecules (Krieger, Malabar, FL, 1991); I. B. Bersuker, The Jahn-Teller Effect (Cambridge University Press, Cambridge, 2006).
46. D. A. Farrow, W. Qian, E. R. Smith, and D. M. Jonas, in Ultrafast Phenomena XIV, edited by, T. Kobayashi, T. Kobayashi, S. DeSilvestri, T. Okada, and, K. A. Nelson, (Springer, New York, 2005), p. 380.
47. D. M. Jonas, S. E. Bradforth, S. A. Passino, and G. R. Fleming, J. Phys. Chem. 99, 2594 (1995).
48. D. M. Jonas, M. J. Lang, Y. Nagasawa, T. Joo, and G. R. Fleming, J. Phys. Chem. 100, 12660 (1996).
49. G. R. Fleming, Chemical Applications of Ultrafast Spectroscopy (Oxford University Press, New York, 1986).
50. W. L. Clinton and B. Rice, J. Chem. Phys. 30, 542 (1959).
51. W. T. Pollard and R. A. Mathies, Annu. Rev. Phys. Chem. 43, 497 (1992).
52. R. A. Marcus, Angew. Chem. 32, 1111 (1993).
53. M. S. Child, J. Mol. Spectrosc. 0022-2852 10.1016/0022-2852(63)90181-4 10, 357 (1963); M. S. Child and F. R. S. Longuet-Higgins, Philos. Trans. R. Soc. London, Ser. A 0962-8428 10.1098/rsta.1961.0017 254, 259 (1961); M. S. Child, Philos. Trans. R. Soc. London, Ser. A 255, 31 (1962).
54. W. M. McClain, J. Chem. Phys. 55, 2789 (1971).
55. P. W. Atkins and R. S. Friedman, Molecular Quantum Mechanics, 3rd ed. (Oxford University Press, New York, 1997).
56. C. Weiss, H. Kobayashi, and M. Gouterman, J. Mol. Spectrosc. 16, 415 (1965).
57. M. B. Masthay, L. A. Findsen, B. M. Pierce, D. F. Bocian, J. S. Lindsey, and R. R. Birge, J. Chem. Phys. 84, 3901 (1986).
58. Y. Tanimura and S. Mukamel, Phys. Rev. E 47, 118 (1993).
59. Y. Gu, A. Widom, and P. M. Champion, J. Chem. Phys. 100, 2547 (1994).
60. S. Mukamel, Annu. Rev. Phys. Chem. 41, 647 (1990).
61. See EPAPS Document No. E-JCPSA6-128-011807 for information on experimental apparatus, tests for experimental artifacts, spectrally resolved pump-probe data, and models. For more information on EPAPS, see http//www.aip.org/pubservs/epaps.html.
62. M. Gouterman, J. Mol. Spectrosc. 6, 138 (1961).
63. C. Cohen-Tannoudji, B. Diu, and F. Lalöe, Quantum Mechanics (Wiley-Interscience, Paris, 1977).
64. C. Cohen-Tannoudji, J. Dupont-Roc, and G. Grynberg, Atom-Photon Interactions: Basic Processes and Applications (Wiley-Interscience, New York, 1992).
65. J. Sung and R. J. Silbey, J. Chem. Phys. 115, 9266 (2001).
66. J. Sung and R. J. Silbey, J. Chem. Phys. 122, 169901 (2005).
67. J. Sung and R. J. Silbey, J. Chem. Phys. 118, 2443 (2002).
68. M. Khalil, O. Golonzka, N. Demirdöven, C. J. Fecko, and A. Tokmakoff, Chem. Phys. Lett. 321, 231 (2000).
69. D. A. Farrow, E. R. Smith, W. Qian, and D. M. Jonas, " The polarization anisotropy of vibrational quantum beats in resonant pump-probe experiments: Diagrammatic calculations for square symmetric molecules.," J. Chem. Phys. (submitted).
70. M. Gouterman, in The Porphyrins, edited by, D. Dolphin, (Academic, New York, 1978), Vol. 3, p. 1.
71. L. D. Landau and E. M. Lifshitz, Fluid Mechanics, 2nd ed. (Pergamon, New York, 1987).
72. A. W. Albrecht, J. D. Hybl, S. M. Gallagher Faeder, and D. M. Jonas, J. Chem. Phys. 0021-9606 10.1063/1.480457 111, 10934 (1999); A. W. Albrecht, J. D. Hybl, S. M. Gallagher Faeder, and D. M. Jonas, J. Chem. Phys. 115, 5691(E) (2001).
73. A. H. Zewail, Science 242, 1645 (1988).
74. D. Braun, B. C. Titeca, and A. Ceulemans, J. Porphyr. Phthalocyanines 5, 33 (2001).
75. R. E. Clavijo, M. M. Campos Vallette, M. Saavedra, A. Alvarado, and G. Diaz, Vib. Spectrosc. 14, 79 (1997).
76. S. M. Arabei, J. P. Galaup, K. N. Solovyov, and V. F. Donyagina, Chem. Phys. 311, 307 (2005).
77. A. W. Albrecht Ferro, Ph.D. thesis, University of Colorado at Boulder, 2001.
78. P. Cong, Y. J. Yan, H. P. Deuel, and J. D. Simon, J. Chem. Phys. 0021-9606 10.1063/1.466832 100, 7855 (1994); P. Vöhringer, R. A. Westervelt, D. C. Arnett, M. J. Feldstein, and N. F. Scherer, J. Raman Spectrosc. 0377-0486 10.1002/jrs.1250260709 26, 535 (1995); T. Joo, Y. Jia, J.-Y. Yu, M. J. Lang, and G. R. Fleming, J. Chem. Phys. 104, 6089 (1996).
79. This slowing of electronic dephasing by vibrational motion may be an example of the quantum Zeno effect discussed in B. Misra and E. C. G. Sudarshan, J. Math. Phys. 18, 756 (1977).
80. G. C. Walker, E. Akesson, A. E. Johnson, N. E. Levinger, and P. F. Barbara, J. Phys. Chem. 96, 3728 (1992).
81. C. A. Mead and D. G. Truhlar, J. Chem. Phys. 77, 6090 (1982).
82. G. A. Worth and L. S. Cederbaum, Annu. Rev. Phys. Chem. 55, 127 (2004).
83. S. Sunder and H. J. Bernstein, J. Raman Spectrosc. 5, 351 (1976).
84. J. A. Cina and G. R. Fleming, J. Phys. Chem. A 108, 11196 (2004).
85. S. Mukamel and D. Abramavicius, Chem. Rev. (Washington, D.C.) 104, 2073 (2004).
86. J. P. Bergsma, P. H. Berens, K. R. Wilson, D. R. Fredkin, and E. J. Heller, J. Phys. Chem. 88, 612 (1984).
87. D. Papousek and M. R. Aliev, Molecular Vibrational-Rotational Spectra (Elsevier Scientific, New York, 1982).
88. O. V. Prezhdo and P. J. Rossky, Phys. Rev. Lett. 81, 5294 (1998).
89. C. Zhu, Y. Teranishi, and H. Nakamura, Adv. Chem. Phys. 117, 127 (2001).
90. G. Herzberg and E. Teller, Z. Phys. Chem. Abt. B 21, 410 (1933).
91. E. U. Condon, Am. J. Phys. 15, 365 (1947).
92. L. S. Cederbaum, E. Gindensperger, and I. Burghardt, Phys. Rev. Lett. 0031-9007 10.1103/PhysRevLett.94.113003 94, 113003 (2005); E. Gindensperger, I. Burghardt, and L. S. Cederbaum, J. Chem. Phys. 124, 144104 (2006).
93. E. Gindensperger, I. Burghardt, and L. S. Cederbaum, J. Chem. Phys. 124, 144103 (2006).
94. S. Mahaparta and H. Köppel, Phys. Rev. Lett. 0031-9007 10.1103/PhysRevLett.81.3116 81, 3116 (1998); H. Tamura, S. Nanbu, H. Nakamura, and T. Ishida, Chem. Phys. Lett. 0009-2614 10.1016/j.cplett.2004.11.111 401, 487 (2004); V. Vallet, Z. Lan, S. Mahapatra, A. Sobolewski, and W. Domcke, J. Chem. Phys. 123, 144307 (2005).
95. R. Kienberger, E. Goulielmakis, M. Uiberacker, Nature (London) 0028-0836 10.1038/nature02277 427, 817 (2004); A. Fohlisch, P. Feulner, F. Hennies, A. Fink, D. Menzel, D. Sanchez-Portal, P. Echenique, and W. Wurth, Nature (London) 436, 373 (2005).
96. M. S. Pshenichnikov, A. Baltuska, and D. A. Wiersma, Top. Appl. Phys. 95, 409 (2004).
97. A. T. Yeh, C. V. Shank, and J. K. McCusker, Science 289, 935 (2000).
98. M. J. Paterson, L. Blancafort, S. Wilsey, and M. A. Robb, J. Phys. Chem. A 106, 11431 (2002).
99. R. Huber, J.-E. Moser, M. Gratzel, and J. Wachtveitl, J. Phys. Chem. B 106, 6494 (2002).
100. S. Williams, R. N. Zare, and L. A. Rahn, J. Chem. Phys. 101, 1072 (1994).
101. S. J. Cyvin, J. E. Rauch, and J. C. Decius, J. Chem. Phys. 43, 4083 (1965).