Sequential self-organization of silver(I) layered materials with strong SHG by J aggregation and intercalation of organic nonlinear optical chromophores through mechanochemical synthesis

Chemistry of Materials

Volumn 19, Issue 15, 2007, Pages 3704-3711

  Cariati, Elena ^a   Macchi, Roberto ^a   Roberto, Dominique ^a   Ugo, Renato ^a   Galli, Simona ^b   Masciocchi, Norberto ^b   Sironi, Angelo ^a  

^a UNIVERSITY OF MILAN   (Italy)

^b UNIVERSITY OF INSUBRIA   (Italy)

Author keywords

[No Author keywords available]

Indexed keywords

ABSORPTION SPECTRA; HARMONIC GENERATION; NONLINEAR OPTICS;

ELECTRONIC ABSORPTION SPECTRA; MECHANOCHEMICAL APPROACH;

CHROMOPHORES;

EID: 34547676295     PISSN: 08974756     EISSN: None     Source Type: Journal    
DOI: 10.1021/cm071003e     Document Type: Article

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36. -)I interactions possess a certain degree of electrostactic character, so distances computed from van der Waals radii are somewhat overestimated.
37. Alternatively, the consecutive guest layers could be iso-oriented (leading to a "macroscopic" polarity lying in the ab plane). We do not have any direct evidence to discriminate between the two hypotheses; however, the presence of equally oriented guest layers should promote some (yet unobserved) distortion of the rhombohedral host lattice. Therefore, we propose the hypothesis of the helical domains.