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note
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This study was sponsored by the Air and Environmental Quality Division of the Department for Environment, Food and Rural Affairs through contract no. CPEA 7, by the GMR Programme of the Met Office, by a NERC/Environment Agency Advanced Fellowship (P4-F02) to one of us (DSS) and by the European Commission through contract no; EVK2-CT-2002-80019 NEPAP. The assistance and guidance provided by the referees are gratefully acknowledged.
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