Waiting time distribution and nonexponential relaxation in single molecule spectroscopic studies: Realization of entropic bottleneck in a simple model

Journal of Chemical Physics

Volumn 118, Issue 17, 2003, Pages 7965-7973

  Chakrabarti, Dwaipayan ^a   Bagchi, Biman ^a  

^a INDIAN INSTITUTE OF SCIENCE   (India)

Author keywords

[No Author keywords available]

Indexed keywords

COMPUTER SIMULATION; ENTROPY; MATHEMATICAL MODELS; MOLECULAR DYNAMICS; PROBABILITY; RELAXATION PROCESSES;

FINITE DISCRETE SPECE; FRACTIONAL POWER LAW DEPENDENCE; LIOUVILLE-MASTER EQUATION; SINGLE MOLECULE SPECTROSCOPY;

MOLECULAR SPECTROSCOPY;

EID: 0038176514     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1564055     Document Type: Article

References (29)

1. R. Zwanzig, J. Chem. Phys. 97, 3587 (1992).
2. H. X. Zhou and R. Zwanzig, J. Chem. Phys. 94, 6147 (1991).
3. N. Eizenberg and J. Klafter, Chem. Phys. Lett. 243, 9 (1995)
4. N. Eizenberg and J. Klafter, J. Chem. Phys. 104, 6796 (1996)
5. N. Eizenberg and J. Klafter, Physica A 249, 424 (1998).
6. A. M. Berezhkovskii, Y. A. D'yakov, J. Klafter, and V. Y. Zitzerman, Chem. Phys. Lett. 287, 442 (1998).
7. J. Wang and P. Wolynes, Chem. Phys. Lett. 212, 427 (1993).
8. D. L. Stein, R. G. Palmer, J. L. V. Hemmen, and C. R. Doering, Phys. Lett. A 136, 353 (1989).
9. C. R. Doering and J. C. Gadoua, Phys. Rev. Lett. 69, 2318 (1992).
10. B. Bagchi, G. R. Fleming, and D. W. Oxtoby, J. Chem. Phys. 78, 7375 (1983).
11. H. P. Lu, L. Xun, and X. Sunney Xie, Science 282, 1877 (1998)
12. G. K. Schenter, H. P. Lu, and X. S. Xie, J. Phys. Chem. A 103, 10477 (1999).
13. D. W. E. Moerner and M. Orrit, Science 283, 1670 (1999).
14. S. Weiss, Science 283, 1676 (1999).
15. Q. F. Xue and E. S. Yeung, Nature (London) 373, 681 (1995).
16. J. J. Macklin, J. K. Trautman, T. D. Harris, and L. E. Brus, Science 272, 255 (1996).
17. T. Ha, T. Enderle, D. S. Chemla, P. R. Selvin, and S. Weiss, Phys. Rev. Lett. 77, 3979 (1996).
18. H. P. Lu and X. S. Xie, J. Phys. Chem. B 101, 2753 (1997).
19. R. Zwanzig, Acc. Chem. Res. 23, 148 (1990).
20. L. Edman, U. Mets, and R. Rigler, Proc. Natl. Acad. Sci. U.S.A. 93, 6710 (1996).
21. A. A. Deniz, T. A. Laurence, G. S. Beligere, M. Dahan, A. B. Martin, D. S. Chemla, P. E. Dawson, P. G. Schultz, and S. Weiss, Proc. Natl. Acad. Sci. U.S.A. 97, 5179 (2000).
22. X. Zhuang, L. E. Bartley, H. P. Babcock, R. Russell, T. Ha, D. Herschlag, and S. Chu, Science 288, 2048 (2000).
23. N. G. Van Kampen, Stochastic Processes in Physics and Chemistry (Elsevier Science, B. V., 1992).
24. C. W. Gardiner, Handbook of Stochastic Methods (Springer-Verlag, Berlin, Heidelberg, 1985).
25. R. Zwanzig, A. Szabo, and B. Bagchi, Proc. Natl. Acad. Sci. U.S.A. 89, 20 (1992).
26. J. Cao, J. Chem. Phys. 114, 5137 (2001).
27. X. S. Xie (private communications).
28. A. Szabo, D. Shoup, S. H. Northrup, and J. A. McCammon, J. Chem. Phys. 77, 4484 (1982).
29. N. Agmon and J. J. Hopfield, J. Chem. Phys. 78, 6947 (1983).