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note
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At this time, we have not applied this approach in detail to 3 and 4, for which it also could be possible to take up one more MVE molecule before transferring the methyl group. However, preliminary calculations show that, as for 2 + MVE, one obtains isolated 3 and 4 together with an unbound MVE molecule.
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24
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0012418847
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5 Here it is absolutely essential not to have any other strong donors-such as THF-present, because MVE cannot replace these at the metal center.
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27
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0012376523
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note
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2C bridge which lowers the Cp-Zr-Cp angle even more.
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30
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0012452594
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note
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(d) A more detailed analysis of the potential of 9, 10, and 12 as precursors, of course, would have to include the determination of activation energies for the reactions mentioned in this subsection. This is postponed for furture work. The results mentioned here are meant to show experimentally promising trends for initiation.
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32
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