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Volumn 122, Issue 15, 2000, Pages 3652-3670

Dinitrogen rearranging over a metal-oxo surface and cleaving to nitride: From the end-on to the side-on bonding mode, to the stepwise cleavage of the N≡N bonds assisted by Nb(III)-calix[4]arene

Author keywords

[No Author keywords available]

Indexed keywords

CALIXARENE; METAL COMPLEX; NITROGEN;

EID: 0034685509     PISSN: 00027863     EISSN: None     Source Type: Journal    
DOI: 10.1021/ja9943288     Document Type: Article
Times cited : (171)

References (99)
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    • A few niobium-dinitrogen compounds have been reported. See ref 3e and the following references: (a) Dilworth, J. R.; Henderson, R. A.; Hills, A.; Hughes, D. L.; Macdonald, C.; Stephens, A. N.; Walton, D. R. M. J. Chem. Soc., Dalton Trans. 1990, 1077. (b) Benin, P.; Gambarotta, S. Organometallics 1995, 14, 2159.
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    • For example: (a) Castellano, B.; Solari, E.; Floriani, C.; Scopelliti, R. Inorg. Chem. 1999, 38, 3406. (b) Giannini, L.; Solari, E.; Floriani, C.; Re, N.; Chiesi-Villa, A.; Rizzoli, C. Inorg. Chem. 1999, 38, 1439.
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    • note
    • -1, crystal dimensions 0.21 × 0.25 × 0.35 mm. For 5311 unique observed reflections [I > 2σ(I)] collected at 130 K on a MAR345 image plate diffractometer (5 > 2θ > 49°), RI = 0.126 (wR2 = 0.326).
  • 84
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    • note
    • -1, crystal dimensions 0.17 × 0.20 × 0.25 mm. For 9044 unique observed reflections [I > 2σ(I)] collected at 130 K on a Kuma KM4CCD diffractometer (5 > 2θ > 59°), R1 = 0.153 (wR2 = 0.301).
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    • note
    • A compilation of N-N bond lengths in dinitrogen complexes is reported in ref 3j.


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