Investigation of Synthesizing MCM-41/ZSM-5 Composites

Journal of Physical Chemistry B

Volumn 104, Issue 13, 2000, Pages 2817-2823

  Huang, Limin ^a   Guo, Wanping ^a   Deng, Peng ^a   Xue, Zhiyuan ^a   Li, Quanzhi ^a  

^a FUDAN UNIVERSITY   (China)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 0034611711     PISSN: 15206106     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp990861y     Document Type: Article

References (29)

1. Beck, J. S.; Vartuli, C.; Roth, W. J.; Leonowicz, M. E.; Kresge, C. T.; Schmitt, K. D.; Chu, C. T-W.; Oison, D. H.; Sheppard, E. W.; McCullen, S. B.; Higgins, J. B.; Schlenker, J. L. J. Am. Chem. Soc. 1992, 114, 10834.
2. Zhao, D.; Feng, J.; Huo, Q.; Melosh, N.; Fredrickson. G. H.; Chmelka, B. F.; Stucky, G. D. Science 1998, 279, 548.
3. Davis, M. E. Nature 1993, 364, 391.
4. Sayari, A. Chem. Mater. 1996, 8, 1840.
5. Corma, A.; Fornes, V.; Navarro, M. T.; Perez-Pariente, J. J. Catal. 1994, 148, 569.
6. Branton, P. J.; Hall, P. G.; Sing, K. S. W.; Reichert, H.; Schuth, F.; Unger, K. K. J. Chem. Soc., Faraday Trans. 1994, 90, 19, 2965.
7. Kloetstra, K. R.; Zandbergen, H. W.; Jansen, J. C.; van Bekkum, H. Microporous Mater. 1996, 6, 287.
8. Kloetstra, K. R.; Jansen, J. C.; van Bekkum, H. Prepr.-Am. Chem. Soc., Div. Pet. Chem. 1996, 41, 2, 412.
9. Kloetstra, K. R.; van Bekkum, H.; Jansen, J. C. J. Chem. Soc., Chem. Commun. 1997, 2281.
10. Karlsson, A.; Stocker, M.; Schmidt, R. In Proceedings of the 12th International Zeolite Conference; MRS: Warrendale, PA, 1999; Vol. 1, p 713.
11. Karlsson, A.; Stocker, M.; Schmidt, R. Microporous Mesoporous Mater. 1999, 27, 181.
12. Huang, L.; Li, Q. In Proceedings of the 12th International Zeolite Conference; MRS: Warrendale, PA, 1999; Vol. 1, p 707.
13. Stucky, G. D.; Huo, Q. S.; Firouzi, A.; Chmelka, B. F.; Schacht, S.; Voigt-Martin, I. G.; Schuth, F. Progress in Zeolite and Microporous Materials; Studies in Surface Science and Catalysis: Chon, H., Ihm, S.-K., Uh, Y. S., Eds.; Elsevier: Amsterdam, 1997; Vol. 105, Part A. p 3.
14. Coustel, N.; Di Renzo, F.; Fajula, F.J. Chem. Soc., Chem. Commun. 1994, 967.
15. Ryoo, R.; Kim, J. M. J. Chem. Soc., Chem. Commun. 1995, 711.
16. Edler, K. J.; White, J. W. Chem. Mater. 1997, 9, 1226.
17. Ryoo, R.; Jun, S. J. Phys. Chem. B 1997, 101, 317.
18. Huang, L.; Chen, H.; Li, Q. Chinese Pat. Appl. 981109349, 1999.
19. Bagshaw, S. A.; Prouzet, E.; Pinnavaia, T. J. Science 1995, 269, 1242.
20. Ryoo, R.; Kim, J. M.; Shin, C. H.; Lee, J. Y. Progress in Zeolite and Microporous Materials; Studies in Surface Science and Catalysis; Chon, H., Ihm, S.-K., Uh, Y. S., Eds.; Elsevier: Amsterdam, 1997: Vol. 105, Part A, p 45.
21. Gregg, S. J.; Sing, K. S. W. Adsorption, Surface Area and Porosity; Academic Press: London, 1982.
22. Mikhail, R. Sh.; Brunauer, S.; Bodor, E. E. J. Coll. Interface Sci. 1968, 26, 45.
23. Lippens, B. C.; De Boer, J. H. J. Catal. 1965, 4, 319.
24. Because there are no diffraction peaks in high 10 range for mesoporous MCM-41, the ZSM-5 content in sample S2 can be deduced from the sum of three peak intensities in the 29 range of 22-24 °. First, mix MCM-41 with ZSM-5 phases according to various proportions such as 1/10, 1/7, or 1/5, and obtain their XRD profiles. Then, plot the sums of heights of three characteristic peaks in the range of 22-24 ° against the proportions of ZSM-5 to obtain a working curve. Therefore, the ZSM-5 content in sample S2 can be deduced from this working curve. Both the mechanic mixture of ZSM-5 and MCM-41 used for reference here and sample S2 have the same XRD profiles and the same Si/Al ratios.
25. Kim, J. M.; Kwak, J. H.; Jun. S.; Ryoo, R. J. Phys. Chem. 1995, 99, 16742.
26. Fraissard, J.; Ito, T. Zeolites 1988, 8, 350.
27. Chen, X.; Huang, L.; Li. Q. J. Phys. Chem. B 1997, 101, 8460.
28. Yang, P.; Zhao, D.; Margolese, D. I.; Chmelka, B. F.; Stucky, G. D Nature 1998, 395, 152.
29. Guo, W.; Huang, L.; Li, Q. J. Chem. Chin. Univ. 1999, 20, 3, 356.