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Volumn 113, Issue 24, 2000, Pages 11212-11221

Dephasing of individual rotational states in liquids

Author keywords

[No Author keywords available]

Indexed keywords

CONTINUUM MECHANICS; FRICTION; LIQUIDS; MATHEMATICAL MODELS; MOLECULAR DYNAMICS; OSCILLATORS (MECHANICAL); RAMAN SCATTERING; RAMAN SPECTROSCOPY;

EID: 0034505025     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1327292     Document Type: Article
Times cited : (17)

References (91)
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    • note
    • l prescribed by the simple gas-phase expression, Eq. (3.2).
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    • note
    • We do note that the m-level degeneracy is actually split by the instantaneous asymmetry of the solvent (Refs. 7-9). Exactly why our weak coupling approach (which takes into account the individual m states only in an average sense), should lead to results so similar to those of Ref. 8 - which looks specifically at the m-state splitting - is not entirely clear.
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    • KM′(0)〉. See Ref. 7.
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    • ll′(|t-t′|). A systematic presentation of the entire development is given in J. Jang, Ph.D. thesis, Brown University, 2000.
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    • The use of this reference system is, in fact, precisely what is required by the bath average in Eq. (2.19). However, we showed in Ref. 29 that it also provides a numerically accurate way to compute the full friction.
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    • However, generalizations of INM theory have been suggested that may not turn out to be as limited. T. Keyes, J. Chem. Phys. 104, 9349 (1996).
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* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.